!!C ====================================================================== !!C !C --- ISORROPIA CODE II !C --- SUBROUTINE ISOROPIA !C --- THIS SUBROUTINE IS THE MASTER ROUTINE FOR THE ISORROPIA !C THERMODYNAMIC EQUILIBRIUM AEROSOL MODEL (VERSION 1.1 and above) !C !C ======================== ARGUMENTS / USAGE =========================== !C !C INPUT: !C 1. [WI] !C DOUBLE PRECISION array of length [8]. !C Concentrations, expressed in moles/m3. Depending on the type of !C problem solved (specified in CNTRL(1)), WI contains either !C GAS+AEROSOL or AEROSOL only concentratios. !C WI(1) - sodium !C WI(2) - sulfate !C WI(3) - ammonium !C WI(4) - nitrate !C WI(5) - chloride !C WI(6) - calcium !C WI(7) - potassium !C WI(8) - magnesium !C !C 2. [RHI] !C DOUBLE PRECISION variable. !C Ambient relative humidity expressed on a (0,1) scale. !C !C 3. [TEMPI] !C DOUBLE PRECISION variable. !C Ambient temperature expressed in Kelvins. !C !C 4. [CNTRL] !C DOUBLE PRECISION array of length [2]. !C Parameters that control the type of problem solved. !C !C CNTRL(1): Defines the type of problem solved. !C 0 - Forward problem is solved. In this case, array WI contains !C GAS and AEROSOL concentrations together. !C 1 - Reverse problem is solved. In this case, array WI contains !C AEROSOL concentrations only. !C !C CNTRL(2): Defines the state of the aerosol !C 0 - The aerosol can have both solid+liquid phases (deliquescent) !C 1 - The aerosol is in only liquid state (metastable aerosol) !C !C OUTPUT: !C 1. [WT] !C DOUBLE PRECISION array of length [8]. !C Total concentrations (GAS+AEROSOL) of species, expressed in moles/m3. !C If the foreward probelm is solved (CNTRL(1)=0), array WT is !C identical to array WI. !C WT(1) - total sodium !C WT(2) - total sulfate !C WT(3) - total ammonium !C WT(4) - total nitrate !C WT(5) - total chloride !C WT(6) - total calcium !C WT(7) - total potassium !C WT(8) - total magnesium !C !C 2. [GAS] !C DOUBLE PRECISION array of length [03]. !C Gaseous species concentrations, expressed in moles/m3. !C GAS(1) - NH3 !C GAS(2) - HNO3 !C GAS(3) - HCl !C !C 3. [AERLIQ] !C DOUBLE PRECISION array of length [15]. !C Liquid aerosol species concentrations, expressed in moles/m3. !C AERLIQ(01) - H+(aq) !C AERLIQ(02) - Na+(aq) !C AERLIQ(03) - NH4+(aq) !C AERLIQ(04) - Cl-(aq) !C AERLIQ(05) - SO4--(aq) !C AERLIQ(06) - HSO4-(aq) !C AERLIQ(07) - NO3-(aq) !C AERLIQ(08) - H2O !C AERLIQ(09) - NH3(aq) (undissociated) !C AERLIQ(10) - HNCl(aq) (undissociated) !C AERLIQ(11) - HNO3(aq) (undissociated) !C AERLIQ(12) - OH-(aq) !C AERLIQ(13) - Ca2+(aq) !C AERLIQ(14) - K+(aq) !C AERLIQ(15) - Mg2+(aq) !C !C 4. [AERSLD] !C DOUBLE PRECISION array of length [19]. !C Solid aerosol species concentrations, expressed in moles/m3. !C AERSLD(01) - NaNO3(s) !C AERSLD(02) - NH4NO3(s) !C AERSLD(03) - NaCl(s) !C AERSLD(04) - NH4Cl(s) !C AERSLD(05) - Na2SO4(s) !C AERSLD(06) - (NH4)2SO4(s) !C AERSLD(07) - NaHSO4(s) !C AERSLD(08) - NH4HSO4(s) !C AERSLD(09) - (NH4)4H(SO4)2(s) !C AERSLD(10) - CaSO4(s) !C AERSLD(11) - Ca(NO3)2(s) !C AERSLD(12) - CaCl2(s) !C AERSLD(13) - K2SO4(s) !C AERSLD(14) - KHSO4(s) !C AERSLD(15) - KNO3(s) !C AERSLD(16) - KCl(s) !C AERSLD(17) - MgSO4(s) !C AERSLD(18) - Mg(NO3)2(s) !C AERSLD(19) - MgCl2(s) !C !C 5. [SCASI] !C CHARACTER*15 variable. !C Returns the subcase which the input corresponds to. !C !C 6. [OTHER] !C DOUBLE PRECISION array of length [9]. !C Returns solution information. !C !C OTHER(1): Shows if aerosol water exists. !C 0 - Aerosol is WET !C 1 - Aerosol is DRY !C !C OTHER(2): Aerosol Sulfate ratio, defined as (in moles/m3) : !C (total ammonia + total Na) / (total sulfate) !C !C OTHER(3): Sulfate ratio based on aerosol properties that defines !C a sulfate poor system: !C (aerosol ammonia + aerosol Na) / (aerosol sulfate) !C !C OTHER(4): Aerosol sodium ratio, defined as (in moles/m3) : !C (total Na) / (total sulfate) !C !C OTHER(5): Ionic strength of the aqueous aerosol (if it exists). !C !C OTHER(6): Total number of calls to the activity coefficient !C calculation subroutine. !C !C OTHER(7): Sulfate ratio with crustal species, defined as (in moles/m3) : !C (total ammonia + total crustal species + total Na) / (total sulfate) !C !C OTHER(8): Crustal species + sodium ratio, defined as (in moles/m3) : !C (total crustal species + total Na) / (total sulfate) !C !C OTHER(9): Crustal species ratio, defined as (in moles/m3) : !C (total crustal species) / (total sulfate) !C !C --- COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C --- GEORGIA INSTITUTE OF TECHNOLOGY !C --- WRITTEN BY ATHANASIOS NENES !C --- UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE ISOROPIA2p1 (WI, RHI, TEMPI, CNTRL, & WT, GAS, AERLIQ, AERSLD, SCASI, OTHER) INCLUDE 'module_isrpia_inc.F' PARAMETER (NCTRL=2,NOTHER=9) CHARACTER SCASI*15 DIMENSION WI(NCOMP), WT(NCOMP), GAS(NGASAQ), AERSLD(NSLDS), & AERLIQ(NIONS+NGASAQ+2), CNTRL(NCTRL), OTHER(NOTHER) !liqy character*8 date character*10 time character*5 zone integer*4 values(8) ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isoropia' ! close (unit=220) !liqy-20140513 !C !C --- PROBLEM TYPE (0=FOREWARD, 1=REVERSE) ------------------------------ !C IPROB = NINT(CNTRL(1)) !C !C --- AEROSOL STATE (0=SOLID+LIQUID, 1=METASTABLE) --------------------- !C METSTBL = NINT(CNTRL(2)) !C !C --- SOLVE FOREWARD PROBLEM ------------------------------------------** !C 50 IF (IPROB.EQ.0) THEN IF (WI(1)+WI(2)+WI(3)+WI(4)+WI(5)+WI(6)+WI(7)+WI(8) .LE. TINY) & THEN !Everything=0 CALL INIT12p1 (WI, RHI, TEMPI) !liqy ! ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling init1-f' ! close (unit=220) !liqy-20140512 ELSE IF (WI(1)+WI(4)+WI(5)+WI(6)+WI(7)+WI(8) .LE. TINY) THEN !Ca,K,Mg,Na,Cl,NO3=0 CALL ISRP1F2p1 (WI, RHI, TEMPI) !liqy ! ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp1f' ! close (unit=220) !liqy-20140512 ELSE IF (WI(1)+WI(5)+WI(6)+WI(7)+WI(8) .LE. TINY) THEN !Ca,K,Mg,Na,Cl=0 CALL ISRP2F2p1 (WI, RHI, TEMPI) !liqy ! ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp2f' ! close (unit=220) !liqy-20140512 ELSE IF (WI(6)+WI(7)+WI(8) .LE. TINY) THEN !Ca,K,Mg=0 CALL ISRP3F2p1 (WI, RHI, TEMPI) !liqy ! ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp3f' ! close (unit=220) !liqy-20140512 ELSE CALL ISRP4F2p1 (WI, RHI, TEMPI) !liqy ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp4f' ! close (unit=220) !liqy-20140513 ENDIF !C !C --- SOLVE REVERSE PROBLEM --------------------------------------------- !C ELSE IF (WI(1)+WI(2)+WI(3)+WI(4)+WI(5)+WI(6)+WI(7)+WI(8) .LE. TINY) & THEN !Everything=0 CALL INIT12p1 (WI, RHI, TEMPI) !liqy ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling init1-r' ! close (unit=220) !liqy-20140513 ELSE IF (WI(1)+WI(4)+WI(5)+WI(6)+WI(7)+WI(8) .LE. TINY) THEN !Ca,K,Mg,Na,Cl,NO3=0 CALL ISRP1R2p1 (WI, RHI, TEMPI) !liqy ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp1r' ! close (unit=220) !liqy-20140513 ELSE IF (WI(1)+WI(5)+WI(6)+WI(7)+WI(8) .LE. TINY) THEN !Ca,K,Mg,Na,Cl=0 CALL ISRP2R2p1 (WI, RHI, TEMPI) !liqy ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp2r' ! close (unit=220) !liqy-20140513 ELSE IF (WI(6)+WI(7)+WI(8) .LE. TINY) THEN !Ca,K,Mg=0 CALL ISRP3R2p1 (WI, RHI, TEMPI) !liqy ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp3r' ! close (unit=220) !liqy-20140513 ELSE CALL ISRP4R2p1 (WI, RHI, TEMPI) !liqy ! call date_and_time( date , time, zone, values ) ! open(unit=220,file='call-iso.txt',position='append') ! write(220,*) date, time, ' calling isrp4r' ! close (unit=220) !liqy-20140513 ENDIF ENDIF !C !C --- ADJUST MASS BALANCE ---------------------------------------------** !C IF (NADJ.EQ.1) CALL ADJUST2p1 (WI) !ccC !ccC *** IF METASTABLE AND NO WATER - RESOLVE AS NORMAL ******************** !ccC !!cc IF (WATER.LE.TINY .AND. METSTBL.EQ.1) THEN !cc METSTBL = 0 !cc GOTO 50 !cc ENDIF !C !C *** SAVE RESULTS TO ARRAYS (units = mole/m3) **************************** !C GAS(1) = GNH3 ! Gaseous aerosol species GAS(2) = GHNO3 GAS(3) = GHCL !C DO 10 I=1,7 ! Liquid aerosol species AERLIQ(I) = MOLAL(I) 10 CONTINUE DO 20 I=1,NGASAQ AERLIQ(7+1+I) = GASAQ(I) 20 CONTINUE AERLIQ(7+1) = WATER*1.0D3/18.0D0 AERLIQ(7+NGASAQ+2) = COH !C DO 250 I=8,10 ! Liquid aerosol species AERLIQ(I+5) = MOLAL(I) 250 CONTINUE !C AERSLD(1) = CNANO3 ! Solid aerosol species AERSLD(2) = CNH4NO3 AERSLD(3) = CNACL AERSLD(4) = CNH4CL AERSLD(5) = CNA2SO4 AERSLD(6) = CNH42S4 AERSLD(7) = CNAHSO4 AERSLD(8) = CNH4HS4 AERSLD(9) = CLC AERSLD(10) = CCASO4 AERSLD(11) = CCANO32 AERSLD(12) = CCACL2 AERSLD(13) = CK2SO4 AERSLD(14) = CKHSO4 AERSLD(15) = CKNO3 AERSLD(16) = CKCL AERSLD(17) = CMGSO4 AERSLD(18) = CMGNO32 AERSLD(19) = CMGCL2 !C IF(WATER.LE.TINY) THEN ! Dry flag OTHER(1) = 1.d0 ELSE OTHER(1) = 0.d0 ENDIF !C OTHER(2) = SULRAT ! Other stuff OTHER(3) = SULRATW OTHER(4) = SODRAT OTHER(5) = IONIC OTHER(6) = ICLACT OTHER(7) = SO4RAT OTHER(8) = CRNARAT OTHER(9) = CRRAT !C SCASI = SCASE !C WT(1) = WI(1) ! Total gas+aerosol phase WT(2) = WI(2) WT(3) = WI(3) WT(4) = WI(4) WT(5) = WI(5) WT(6) = WI(6) WT(7) = WI(7) WT(8) = WI(8) IF (IPROB.GT.0 .AND. WATER.GT.TINY) THEN WT(3) = WT(3) + GNH3 WT(4) = WT(4) + GHNO3 WT(5) = WT(5) + GHCL ENDIF !C RETURN !C !C *** END OF SUBROUTINE ISOROPIA ****************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE SETPARM !C *** THIS SUBROUTINE REDEFINES THE SOLUTION PARAMETERS OF ISORROPIA !C !C ======================== ARGUMENTS / USAGE =========================== !C !C *** NOTE: IF NEGATIVE VALUES ARE GIVEN FOR A PARAMETER, IT IS !C IGNORED AND THE CURRENT VALUE IS USED INSTEAD. !C !C INPUT: !C 1. [WFTYPI] !C INTEGER variable. !C Defines the type of weighting algorithm for the solution in Mutual !C Deliquescence Regions (MDR's): !C 0 - MDR's are assumed dry. This is equivalent to the approach !C used by SEQUILIB. !C 1 - The solution is assumed "half" dry and "half" wet throughout !C the MDR. !C 2 - The solution is a relative-humidity weighted mean of the !C dry and wet solutions (as defined in Nenes et al., 1998) !C !C 2. [IACALCI] !C INTEGER variable. !C Method of activity coefficient calculation: !C 0 - Calculate coefficients during runtime !C 1 - Use precalculated tables !C !C 3. [EPSI] !C DOUBLE PRECITION variable. !C Defines the convergence criterion for all iterative processes !C in ISORROPIA, except those for activity coefficient calculations !C (EPSACTI controls that). !C !C 4. [MAXITI] !C INTEGER variable. !C Defines the maximum number of iterations for all iterative !C processes in ISORROPIA, except for activity coefficient calculations !C (NSWEEPI controls that). !C !C 5. [NSWEEPI] !C INTEGER variable. !C Defines the maximum number of iterations for activity coefficient !C calculations. !C !C 6. [EPSACTI] !C DOUBLE PRECISION variable. !C Defines the convergence criterion for activity coefficient !C calculations. !C !C 7. [NDIV] !C INTEGER variable. !C Defines the number of subdivisions needed for the initial root !C tracking for the bisection method. Usually this parameter should !C not be altered, but is included for completeness. !C !C 8. [NADJ] !C INTEGER variable. !C Forces the solution obtained to satisfy total mass balance !C to machine precision !C 0 - No adjustment done (default) !C 1 - Do adjustment !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE SETPARM2p1 (WFTYPI, IACALCI, EPSI, MAXITI, NSWEEPI, & EPSACTI, NDIVI, NADJI) INCLUDE 'module_isrpia_inc.F' INTEGER WFTYPI !C !C *** SETUP SOLUTION PARAMETERS ***************************************** !C IF (WFTYPI .GE. 0) WFTYP = WFTYPI IF (IACALCI.GE. 0) IACALC = IACALCI IF (EPSI .GE.ZERO) EPS = EPSI IF (MAXITI .GT. 0) MAXIT = MAXITI IF (NSWEEPI.GT. 0) NSWEEP = NSWEEPI IF (EPSACTI.GE.ZERO) EPSACT = EPSACTI IF (NDIVI .GT. 0) NDIV = NDIVI IF (NADJI .GE. 0) NADJ = NADJI !C !C *** END OF SUBROUTINE SETPARM ***************************************** !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE GETPARM !C *** THIS SUBROUTINE OBTAINS THE CURRENT VAULES OF THE SOLUTION !C PARAMETERS OF ISORROPIA !C !C ======================== ARGUMENTS / USAGE =========================== !C !C *** THE PARAMETERS ARE THOSE OF SUBROUTINE SETPARM !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE GETPARM2p1 (WFTYPI, IACALCI, EPSI, MAXITI, NSWEEPI, & EPSACTI, NDIVI, NADJI) INCLUDE 'module_isrpia_inc.F' INTEGER WFTYPI !C !C *** GET SOLUTION PARAMETERS ******************************************* !C WFTYPI = WFTYP IACALCI = IACALC EPSI = EPS MAXITI = MAXIT NSWEEPI = NSWEEP EPSACTI = EPSACT NDIVI = NDIV NADJI = NADJ !C !C *** END OF SUBROUTINE GETPARM ***************************************** !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** BLOCK DATA BLKISO !C *** THIS SUBROUTINE PROVIDES INITIAL (DEFAULT) VALUES TO PROGRAM !C PARAMETERS VIA DATA STATEMENTS !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C *** ZSR RELATIONSHIP PARAMETERS MODIFIED BY DOUGLAS WALDRON !C *** OCTOBER 2003 !C *** BASED ON AIM MODEL III (http://mae.ucdavis.edu/wexler/aim) !C !C======================================================================= !C BLOCK DATA BLKISO2p1 INCLUDE 'module_isrpia_inc.F' !C !C *** DEFAULT VALUES ************************************************* !C DATA TEMP/298.0/, R/82.0567D-6/, RH/0.9D0/, EPS/1D-6/, MAXIT/100/, & TINY/1D-20/, GREAT/1D10/, ZERO/0.0D0/, ONE/1.0D0/,NSWEEP/4/, & TINY2/1D-11/,NDIV/5/ !C DATA MOLAL/NIONS*0.0D0/, MOLALR/NPAIR*0.0D0/, GAMA/NPAIR*0.1D0/, & GAMOU/NPAIR*1D10/, GAMIN/NPAIR*1D10/, CALAIN/.TRUE./, & CALAOU/.TRUE./, EPSACT/5D-2/, ICLACT/0/, & IACALC/1/, NADJ/0/, WFTYP/2/ !C DATA ERRSTK/NERRMX*0/, ERRMSG/NERRMX*' '/, NOFER/0/, & STKOFL/.FALSE./ !C DATA IPROB/0/, METSTBL/0/ !C DATA VERSION /'2.1 (07/19/09)'/ !C !C *** OTHER PARAMETERS *********************************************** !C DATA SMW/58.5,142.,85.0,132.,80.0,53.5,98.0,98.0,115.,63.0, & 36.5,120.,247.,136.1,164.,111.,174.2,136.1,101.1,74.5, & 120.3,148.3,95.2/ & IMW/ 1.0,23.0,18.0,35.5,96.0,97.0,62.0,40.1,39.1,24.3/ & WMW/23.0,98.0,17.0,63.0,36.5,40.1,39.1,24.3/ !C DATA ZZ /1,2,1,2,1,1,2,1,1,1,1,1,2,4,2,2,2,1,1,1,4,2,2/ & Z /1,1,1,1,2,1,1,2,1,2/ !C !C *** ZSR RELATIONSHIP PARAMETERS ************************************** !C !C awas= ammonium sulfate !C DATA AWAS/10*187.72,& 158.13,134.41,115.37,100.10, 87.86, 78.00, 70.00, 63.45, 58.02,& 53.46,& 49.59, 46.26, 43.37, 40.84, 38.59, 36.59, 34.79, 33.16, 31.67,& 30.31,& 29.07, 27.91, 26.84, 25.84, 24.91, 24.03, 23.21, 22.44, 21.70,& 21.01,& 20.34, 19.71, 19.11, 18.54, 17.99, 17.46, 16.95, 16.46, 15.99,& 15.54,& 15.10, 14.67, 14.26, 13.86, 13.47, 13.09, 12.72, 12.36, 12.01,& 11.67,& 11.33, 11.00, 10.68, 10.37, 10.06, 9.75, 9.45, 9.15, 8.86,& 8.57,& 8.29, 8.01, 7.73, 7.45, 7.18, 6.91, 6.64, 6.37, 6.10,& 5.83,& 5.56, 5.29, 5.02, 4.74, 4.47, 4.19, 3.91, 3.63, 3.34,& 3.05,& 2.75, 2.45, 2.14, 1.83, 1.51, 1.19, 0.87, 0.56, 0.26,& 0.1/ !C !C awsn= sodium nitrate !C DATA AWSN/10*394.54,& 338.91,293.01,254.73,222.61,195.56,172.76,153.53,137.32,123.65,& 112.08,& 102.26, 93.88, 86.68, 80.45, 75.02, 70.24, 66.02, 62.26, 58.89,& 55.85,& 53.09, 50.57, 48.26, 46.14, 44.17, 42.35, 40.65, 39.06, 37.57,& 36.17,& 34.85, 33.60, 32.42, 31.29, 30.22, 29.20, 28.22, 27.28, 26.39,& 25.52,& 24.69, 23.89, 23.12, 22.37, 21.65, 20.94, 20.26, 19.60, 18.96,& 18.33,& 17.72, 17.12, 16.53, 15.96, 15.40, 14.85, 14.31, 13.78, 13.26,& 12.75,& 12.25, 11.75, 11.26, 10.77, 10.29, 9.82, 9.35, 8.88, 8.42,& 7.97,& 7.52, 7.07, 6.62, 6.18, 5.75, 5.32, 4.89, 4.47, 4.05,& 3.64,& 3.24, 2.84, 2.45, 2.07, 1.70, 1.34, 0.99, 0.65, 0.31,& 0.1/ !C !C awsc= sodium chloride !C DATA AWSC/10*28.16,& 27.17, 26.27, 25.45, 24.69, 23.98, 23.33, 22.72, 22.14, 21.59,& 21.08,& 20.58, 20.12, 19.67, 19.24, 18.82, 18.43, 18.04, 17.67, 17.32,& 16.97,& 16.63, 16.31, 15.99, 15.68, 15.38, 15.08, 14.79, 14.51, 14.24,& 13.97,& 13.70, 13.44, 13.18, 12.93, 12.68, 12.44, 12.20, 11.96, 11.73,& 11.50,& 11.27, 11.05, 10.82, 10.60, 10.38, 10.16, 9.95, 9.74, 9.52,& 9.31,& 9.10, 8.89, 8.69, 8.48, 8.27, 8.07, 7.86, 7.65, 7.45,& 7.24,& 7.04, 6.83, 6.62, 6.42, 6.21, 6.00, 5.79, 5.58, 5.36,& 5.15,& 4.93, 4.71, 4.48, 4.26, 4.03, 3.80, 3.56, 3.32, 3.07,& 2.82,& 2.57, 2.30, 2.04, 1.76, 1.48, 1.20, 0.91, 0.61, 0.30,& 0.1/ !C !C awac= ammonium chloride !C DATA AWAC/10*1209.00,& 1067.60,949.27,848.62,761.82,686.04,619.16,559.55,505.92,457.25,& 412.69,& 371.55,333.21,297.13,262.81,229.78,197.59,165.98,135.49,108.57,& 88.29,& 74.40, 64.75, 57.69, 52.25, 47.90, 44.30, 41.27, 38.65, 36.36,& 34.34,& 32.52, 30.88, 29.39, 28.02, 26.76, 25.60, 24.51, 23.50, 22.55,& 21.65,& 20.80, 20.00, 19.24, 18.52, 17.83, 17.17, 16.54, 15.93, 15.35,& 14.79,& 14.25, 13.73, 13.22, 12.73, 12.26, 11.80, 11.35, 10.92, 10.49,& 10.08,& 9.67, 9.28, 8.89, 8.51, 8.14, 7.77, 7.42, 7.06, 6.72,& 6.37,& 6.03, 5.70, 5.37, 5.05, 4.72, 4.40, 4.08, 3.77, 3.45,& 3.14,& 2.82, 2.51, 2.20, 1.89, 1.57, 1.26, 0.94, 0.62, 0.31,& 0.1/ !C !C awss= sodium sulfate !C DATA AWSS/10*24.10,& 23.17, 22.34, 21.58, 20.90, 20.27, 19.69, 19.15, 18.64, 18.17,& 17.72,& 17.30, 16.90, 16.52, 16.16, 15.81, 15.48, 15.16, 14.85, 14.55,& 14.27,& 13.99, 13.73, 13.47, 13.21, 12.97, 12.73, 12.50, 12.27, 12.05,& 11.84,& 11.62, 11.42, 11.21, 11.01, 10.82, 10.63, 10.44, 10.25, 10.07,& 9.89,& 9.71, 9.53, 9.36, 9.19, 9.02, 8.85, 8.68, 8.51, 8.35,& 8.19,& 8.02, 7.86, 7.70, 7.54, 7.38, 7.22, 7.06, 6.90, 6.74,& 6.58,& 6.42, 6.26, 6.10, 5.94, 5.78, 5.61, 5.45, 5.28, 5.11,& 4.93,& 4.76, 4.58, 4.39, 4.20, 4.01, 3.81, 3.60, 3.39, 3.16,& 2.93,& 2.68, 2.41, 2.13, 1.83, 1.52, 1.19, 0.86, 0.54, 0.25,& 0.1/ !C !C awab= ammonium bisulfate !C DATA AWAB/10*312.84,& 271.43,237.19,208.52,184.28,163.64,145.97,130.79,117.72,106.42,& 96.64,& 88.16, 80.77, 74.33, 68.67, 63.70, 59.30, 55.39, 51.89, 48.76,& 45.93,& 43.38, 41.05, 38.92, 36.97, 35.18, 33.52, 31.98, 30.55, 29.22,& 27.98,& 26.81, 25.71, 24.67, 23.70, 22.77, 21.90, 21.06, 20.27, 19.52,& 18.80,& 18.11, 17.45, 16.82, 16.21, 15.63, 15.07, 14.53, 14.01, 13.51,& 13.02,& 12.56, 12.10, 11.66, 11.24, 10.82, 10.42, 10.04, 9.66, 9.29,& 8.93,& 8.58, 8.24, 7.91, 7.58, 7.26, 6.95, 6.65, 6.35, 6.05,& 5.76,& 5.48, 5.20, 4.92, 4.64, 4.37, 4.09, 3.82, 3.54, 3.27,& 2.99,& 2.70, 2.42, 2.12, 1.83, 1.52, 1.22, 0.90, 0.59, 0.28,& 0.1/ !C !C awsa= sulfuric acid !C DATA AWSA/34.00, 33.56, 29.22, 26.55, 24.61, 23.11, 21.89, 20.87,& 19.99, 18.45,& 17.83, 17.26, 16.73, 16.25, 15.80, 15.38, 14.98, 14.61, 14.26,& 13.93,& 13.61, 13.30, 13.01, 12.73, 12.47, 12.21, 11.96, 11.72, 11.49,& 11.26,& 11.04, 10.83, 10.62, 10.42, 10.23, 10.03, 9.85, 9.67, 9.49,& 9.31,& 9.14, 8.97, 8.81, 8.65, 8.49, 8.33, 8.18, 8.02, 7.87,& 7.73,& 7.58, 7.44, 7.29, 7.15, 7.01, 6.88, 6.74, 6.61, 6.47,& 6.34,& 6.21, 6.07, 5.94, 5.81, 5.68, 5.55, 5.43, 5.30, 5.17,& 5.04,& 4.91, 4.78, 4.65, 4.52, 4.39, 4.26, 4.13, 4.00, 3.86,& 3.73,& 3.59, 3.45, 3.31, 3.17, 3.02, 2.87, 2.71, 2.56, 2.39,& 2.22,& 2.05, 1.87, 1.68, 1.48, 1.27, 1.04, 0.80, 0.55, 0.28,& 0.1/ !C !C awlc= (NH4)3H(SO4)2 !C DATA AWLC/10*125.37,& 110.10, 97.50, 86.98, 78.08, 70.49, 63.97, 58.33, 53.43, 49.14,& 45.36,& 42.03, 39.07, 36.44, 34.08, 31.97, 30.06, 28.33, 26.76, 25.32,& 24.01,& 22.81, 21.70, 20.67, 19.71, 18.83, 18.00, 17.23, 16.50, 15.82,& 15.18,& 14.58, 14.01, 13.46, 12.95, 12.46, 11.99, 11.55, 11.13, 10.72,& 10.33,& 9.96, 9.60, 9.26, 8.93, 8.61, 8.30, 8.00, 7.72, 7.44,& 7.17,& 6.91, 6.66, 6.42, 6.19, 5.96, 5.74, 5.52, 5.31, 5.11,& 4.91,& 4.71, 4.53, 4.34, 4.16, 3.99, 3.81, 3.64, 3.48, 3.31,& 3.15,& 2.99, 2.84, 2.68, 2.53, 2.37, 2.22, 2.06, 1.91, 1.75,& 1.60,& 1.44, 1.28, 1.12, 0.95, 0.79, 0.62, 0.45, 0.29, 0.14,& 0.1/ !C !C awan= ammonium nitrate !C DATA AWAN/10*960.19,& 853.15,763.85,688.20,623.27,566.92,517.54,473.91,435.06,400.26,& 368.89,& 340.48,314.63,291.01,269.36,249.46,231.11,214.17,198.50,184.00,& 170.58,& 158.15,146.66,136.04,126.25,117.24,108.97,101.39, 94.45, 88.11,& 82.33,& 77.06, 72.25, 67.85, 63.84, 60.16, 56.78, 53.68, 50.81, 48.17,& 45.71,& 43.43, 41.31, 39.32, 37.46, 35.71, 34.06, 32.50, 31.03, 29.63,& 28.30,& 27.03, 25.82, 24.67, 23.56, 22.49, 21.47, 20.48, 19.53, 18.61,& 17.72,& 16.86, 16.02, 15.20, 14.41, 13.64, 12.89, 12.15, 11.43, 10.73,& 10.05,& 9.38, 8.73, 8.09, 7.47, 6.86, 6.27, 5.70, 5.15, 4.61,& 4.09,& 3.60, 3.12, 2.66, 2.23, 1.81, 1.41, 1.03, 0.67, 0.32,& 0.1/ !C !C awsb= sodium bisulfate !C DATA AWSB/10*55.99,& 53.79, 51.81, 49.99, 48.31, 46.75, 45.28, 43.91, 42.62, 41.39,& 40.22,& 39.10, 38.02, 36.99, 36.00, 35.04, 34.11, 33.21, 32.34, 31.49,& 30.65,& 29.84, 29.04, 28.27, 27.50, 26.75, 26.01, 25.29, 24.57, 23.87,& 23.17,& 22.49, 21.81, 21.15, 20.49, 19.84, 19.21, 18.58, 17.97, 17.37,& 16.77,& 16.19, 15.63, 15.08, 14.54, 14.01, 13.51, 13.01, 12.53, 12.07,& 11.62,& 11.19, 10.77, 10.36, 9.97, 9.59, 9.23, 8.87, 8.53, 8.20,& 7.88,& 7.57, 7.27, 6.97, 6.69, 6.41, 6.14, 5.88, 5.62, 5.36,& 5.11,& 4.87, 4.63, 4.39, 4.15, 3.92, 3.68, 3.45, 3.21, 2.98,& 2.74,& 2.49, 2.24, 1.98, 1.72, 1.44, 1.16, 0.87, 0.57, 0.28,& 0.1/ !C !C awpc= potassium chloride !C DATA AWPC/172.62, 165.75, 159.10, 152.67, 146.46, 140.45, 134.64,& 129.03, 123.61, 118.38, 113.34, 108.48, 103.79, 99.27,& 94.93, 90.74, 86.71, 82.84, 79.11, 75.53, 72.09, 68.79,& 65.63, 62.59, 59.68, 56.90, 54.23, 51.68, 49.24, 46.91,& 44.68, 42.56, 40.53, 38.60, 36.76, 35.00, 33.33, 31.75,& 30.24, 28.81, 27.45, 26.16, 24.94, 23.78, 22.68, 21.64,& 20.66, 19.74, 18.86, 18.03, 17.25, 16.51, 15.82, 15.16,& 14.54, 13.96, 13.41, 12.89, 12.40, 11.94, 11.50, 11.08,& 10.69, 10.32, 9.96, 9.62, 9.30, 8.99, 8.69, 8.40, 8.12,& 7.85, 7.59, 7.33, 7.08, 6.83, 6.58, 6.33, 6.08, 5.84,& 5.59, 5.34, 5.09, 4.83, 4.57, 4.31, 4.04, 3.76, 3.48,& 3.19, 2.90, 2.60, 2.29, 1.98, 1.66, 1.33, 0.99, 0.65,& 0.30, 0.1/ !C !C awps= potassium sulfate !C DATA AWPS/1014.82, 969.72, 926.16, 884.11, 843.54, 804.41, 766.68,& 730.32, 695.30, 661.58, 629.14, 597.93, 567.92, 539.09,& 511.41, 484.83, 459.34, 434.89, 411.47, 389.04, 367.58,& 347.05, 327.43, 308.69, 290.80, 273.73, 257.47, 241.98,& 227.24, 213.22, 199.90, 187.26, 175.27, 163.91, 153.15,& 142.97, 133.36, 124.28, 115.73, 107.66, 100.08, 92.95,& 86.26, 79.99, 74.12, 68.63, 63.50, 58.73, 54.27, 50.14,& 46.30, 42.74, 39.44, 36.40, 33.59, 31.00, 28.63, 26.45,& 24.45, 22.62, 20.95, 19.43, 18.05, 16.79, 15.64, 14.61,& 13.66, 12.81, 12.03, 11.33, 10.68, 10.09, 9.55, 9.06,& 8.60, 8.17, 7.76, 7.38, 7.02, 6.66, 6.32, 5.98, 5.65,& 5.31, 4.98, 4.64, 4.31, 3.96, 3.62, 3.27, 2.92, 2.57,& 2.22, 1.87, 1.53, 1.20, 0.87, 0.57, 0.28, 0.1/ !C !C awpn= potassium nitrate !C DATA AWPN/44*1000.00, 953.05, 881.09, 813.39,& 749.78, 690.09, 634.14, 581.77, 532.83, 487.16, 444.61,& 405.02, 368.26, 334.18, 302.64, 273.51, 246.67, 221.97,& 199.31, 178.56, 159.60, 142.33, 126.63, 112.40, 99.54,& 87.96, 77.55, 68.24, 59.92, 52.53, 45.98, 40.2, 35.11,& 30.65, 26.75, 23.35, 20.40, 17.85, 15.63, 13.72, 12.06,& 10.61, 9.35, 8.24, 7.25, 6.37, 5.56, 4.82, 4.12, 3.47,& 2.86, 2.28, 1.74, 1.24, 0.79, 0.40, 0.1/ !C !C awpb= potassium bisulfate !C DATA AWPB/10*55.99,& 53.79, 51.81, 49.99, 48.31, 46.75, 45.28, 43.91, 42.62, 41.39,& 40.22,& 39.10, 38.02, 36.99, 36.00, 35.04, 34.11, 33.21, 32.34, 31.49,& 30.65,& 29.84, 29.04, 28.27, 27.50, 26.75, 26.01, 25.29, 24.57, 23.87,& 23.17,& 22.49, 21.81, 21.15, 20.49, 19.84, 19.21, 18.58, 17.97, 17.37,& 16.77,& 16.19, 15.63, 15.08, 14.54, 14.01, 13.51, 13.01, 12.53, 12.07,& 11.62,& 11.19, 10.77, 10.36, 9.97, 9.59, 9.23, 8.87, 8.53, 8.20,& 7.88,& 7.57, 7.27, 6.97, 6.69, 6.41, 6.14, 5.88, 5.62, 5.36,& 5.11,& 4.87, 4.63, 4.39, 4.15, 3.92, 3.68, 3.45, 3.21, 2.98,& 2.74,& 2.49, 2.24, 1.98, 1.72, 1.44, 1.16, 0.87, 0.57, 0.28,& 0.1/ !C !C awcc= calcium chloride !C DATA AWCC/19.9, 19.0, 18.15, 17.35, 16.6, 15.89, 15.22, 14.58,& 13.99, 13.43, 12.90, 12.41, 11.94, 11.50, 11.09, 10.7,& 10.34, 9.99, 9.67, 9.37, 9.09, 8.83, 8.57, 8.34, 8.12,& 7.91, 7.71, 7.53, 7.35, 7.19, 7.03, 6.88, 6.74, 6.6,& 6.47, 6.35, 6.23, 6.12, 6.01, 5.90, 5.80, 5.70, 5.61,& 5.51, 5.42, 5.33, 5.24, 5.16, 5.07, 4.99, 4.91, 4.82,& 4.74, 4.66, 4.58, 4.50, 4.42, 4.34, 4.26, 4.19, 4.11,& 4.03, 3.95, 3.87, 3.79, 3.72, 3.64, 3.56, 3.48, 3.41,& 3.33, 3.25, 3.17, 3.09, 3.01, 2.93, 2.85, 2.76, 2.68,& 2.59, 2.50, 2.41, 2.32, 2.23, 2.13, 2.03, 1.93, 1.82,& 1.71, 1.59, 1.47, 1.35, 1.22, 1.07, 0.93, 0.77, 0.61,& 0.44, 0.25, 0.1/ !C !C awcn= calcium nitrate !C DATA AWCN/32.89, 31.46, 30.12, 28.84, 27.64, 26.51, 25.44, 24.44,& 23.49, 22.59, 21.75, 20.96, 20.22, 19.51, 18.85, 18.23,& 17.64, 17.09, 16.56, 16.07, 15.61, 15.17, 14.75, 14.36,& 13.99, 13.63, 13.3, 12.98, 12.68, 12.39, 12.11, 11.84,& 11.59, 11.35, 11.11, 10.88, 10.66, 10.45, 10.24, 10.04,& 9.84, 9.65, 9.46, 9.28, 9.1, 8.92, 8.74, 8.57, 8.4,& 8.23, 8.06, 7.9, 7.73, 7.57, 7.41, 7.25, 7.1,6.94, 6.79,& 6.63, 6.48, 6.33, 6.18, 6.03, 5.89, 5.74, 5.60, 5.46,& 5.32, 5.17, 5.04, 4.9, 4.76, 4.62, 4.49, 4.35, 4.22,& 4.08, 3.94, 3.80, 3.66, 3.52, 3.38, 3.23, 3.08, 2.93,& 2.77, 2.60, 2.43, 2.25, 2.07, 1.87, 1.67, 1.45, 1.22,& 0.97, 0.72, 0.44, 0.14, 0.1/ !C !C awmc= magnesium chloride !C DATA AWMC/11.24, 10.99, 10.74, 10.5, 10.26, 10.03, 9.81, 9.59,& 9.38, 9.18, 8.98, 8.79, 8.60, 8.42, 8.25, 8.07, 7.91,& 7.75, 7.59, 7.44, 7.29, 7.15, 7.01, 6.88, 6.75, 6.62,& 6.5, 6.38, 6.27, 6.16, 6.05, 5.94, 5.85, 5.75, 5.65,& 5.56, 5.47, 5.38, 5.30, 5.22, 5.14, 5.06, 4.98, 4.91,& 4.84, 4.77, 4.7, 4.63, 4.57, 4.5, 4.44, 4.37, 4.31,& 4.25, 4.19, 4.13, 4.07, 4.01, 3.95, 3.89, 3.83, 3.77,& 3.71, 3.65, 3.58, 3.52, 3.46, 3.39, 3.33, 3.26, 3.19,& 3.12, 3.05, 2.98, 2.9, 2.82, 2.75, 2.67, 2.58, 2.49,& 2.41, 2.32, 2.22, 2.13, 2.03, 1.92, 1.82, 1.71, 1.60,& 1.48, 1.36, 1.24, 1.11, 0.98, 0.84, 0.70, 0.56, 0.41,& 0.25, 0.1/ !C !C awmn= magnesium nitrate !C DATA AWMN/12.00, 11.84, 11.68, 11.52, 11.36, 11.2, 11.04, 10.88,& 10.72, 10.56, 10.40, 10.25, 10.09, 9.93, 9.78, 9.63,& 9.47, 9.32, 9.17, 9.02, 8.87, 8.72, 8.58, 8.43, 8.29,& 8.15, 8.01, 7.87, 7.73, 7.59, 7.46, 7.33, 7.2, 7.07,& 6.94, 6.82, 6.69, 6.57, 6.45, 6.33, 6.21, 6.01, 5.98,& 5.87, 5.76, 5.65, 5.55, 5.44, 5.34, 5.24, 5.14, 5.04,& 4.94, 4.84, 4.75, 4.66, 4.56, 4.47, 4.38, 4.29, 4.21,& 4.12, 4.03, 3.95, 3.86, 3.78, 3.69, 3.61, 3.53, 3.45,& 3.36, 3.28, 3.19, 3.11, 3.03, 2.94, 2.85, 2.76, 2.67,& 2.58, 2.49, 2.39, 2.3, 2.2, 2.1, 1.99, 1.88, 1.77, 1.66,& 1.54, 1.42, 1.29, 1.16, 1.02, 0.88, 0.73, 0.58, 0.42,& 0.25, 0.1/ !C !C awmn= magnesium sulfate !C DATA AWMS/0.93, 2.5, 3.94, 5.25, 6.45, 7.54, 8.52, 9.40, 10.19,& 10.89, 11.50, 12.04, 12.51, 12.90, 13.23, 13.50, 13.72,& 13.88, 13.99, 14.07, 14.1, 14.09, 14.05, 13.98, 13.88,& 13.75, 13.6, 13.43, 13.25, 13.05, 12.83, 12.61, 12.37,& 12.13, 11.88, 11.63, 11.37, 11.12, 10.86, 10.60, 10.35,& 10.09, 9.85, 9.6, 9.36, 9.13, 8.9, 8.68, 8.47, 8.26,& 8.07, 7.87, 7.69, 7.52, 7.35, 7.19, 7.03, 6.89, 6.75,& 6.62, 6.49, 6.37, 6.26, 6.15, 6.04, 5.94, 5.84, 5.75,& 5.65, 5.56, 5.47, 5.38, 5.29, 5.20, 5.11, 5.01, 4.92,& 4.82, 4.71, 4.60, 4.49, 4.36, 4.24, 4.10, 3.96, 3.81,& 3.65, 3.48, 3.30, 3.11, 2.92, 2.71, 2.49, 2.26, 2.02,& 1.76, 1.50, 1.22, 0.94, 0.64/ !C !C *** ZSR RELATIONSHIP PARAMETERS ************************************** !C !C awas= ammonium sulfate !C !C DATA AWAS/33*100.,30,30,30,29.54,28.25,27.06,25.94, !C & 24.89,23.90,22.97,22.10,21.27,20.48,19.73,19.02,18.34,17.69, !C & 17.07,16.48,15.91,15.37,14.85,14.34,13.86,13.39,12.94,12.50, !C & 12.08,11.67,11.27,10.88,10.51,10.14, 9.79, 9.44, 9.10, 8.78, !C & 8.45, 8.14, 7.83, 7.53, 7.23, 6.94, 6.65, 6.36, 6.08, 5.81, !C & 5.53, 5.26, 4.99, 4.72, 4.46, 4.19, 3.92, 3.65, 3.38, 3.11, !C & 2.83, 2.54, 2.25, 1.95, 1.63, 1.31, 0.97, 0.63, 0.30, 0.001/ !C !C awsn= sodium nitrate !C !C DATA AWSN/ 9*1.e5,685.59, !C & 451.00,336.46,268.48,223.41,191.28, !C & 167.20,148.46,133.44,121.12,110.83, !C & 102.09,94.57,88.03,82.29,77.20,72.65,68.56,64.87,61.51,58.44, !C & 55.62,53.03,50.63,48.40,46.32,44.39,42.57,40.87,39.27,37.76, !C & 36.33,34.98,33.70,32.48,31.32,30.21,29.16,28.14,27.18,26.25, !C & 25.35,24.50,23.67,22.87,22.11,21.36,20.65,19.95,19.28,18.62, !C & 17.99,17.37,16.77,16.18,15.61,15.05,14.51,13.98,13.45,12.94, !C & 12.44,11.94,11.46,10.98,10.51,10.04, 9.58, 9.12, 8.67, 8.22, !C & 7.77, 7.32, 6.88, 6.43, 5.98, 5.53, 5.07, 4.61, 4.15, 3.69, !C & 3.22, 2.76, 2.31, 1.87, 1.47, 1.10, 0.77, 0.48, 0.23, 0.001/ !C !C awsc= sodium chloride !C !C DATA AWSC/ !C & 100., 100., 100., 100., 100., 100., 100., 100., 100., 100., !C & 100., 100., 100., 100., 100., 100., 100., 100., 100.,16.34, !C & 16.28,16.22,16.15,16.09,16.02,15.95,15.88,15.80,15.72,15.64, !C & 15.55,15.45,15.36,15.25,15.14,15.02,14.89,14.75,14.60,14.43, !C & 14.25,14.04,13.81,13.55,13.25,12.92,12.56,12.19,11.82,11.47, !C & 11.13,10.82,10.53,10.26,10.00, 9.76, 9.53, 9.30, 9.09, 8.88, !C & 8.67, 8.48, 8.28, 8.09, 7.90, 7.72, 7.54, 7.36, 7.17, 6.99, !C & 6.81, 6.63, 6.45, 6.27, 6.09, 5.91, 5.72, 5.53, 5.34, 5.14, !C & 4.94, 4.74, 4.53, 4.31, 4.09, 3.86, 3.62, 3.37, 3.12, 2.85, !C & 2.58, 2.30, 2.01, 1.72, 1.44, 1.16, 0.89, 0.64, 0.40, 0.18/ !C !C awac= ammonium chloride !C !C DATA AWAC/ !C & 100., 100., 100., 100., 100., 100., 100., 100., 100., 100., !C & 100., 100., 100., 100., 100., 100., 100., 100., 100.,31.45, !C & 31.30,31.14,30.98,30.82,30.65,30.48,30.30,30.11,29.92,29.71, !C & 29.50,29.29,29.06,28.82,28.57,28.30,28.03,27.78,27.78,27.77, !C & 27.77,27.43,27.07,26.67,26.21,25.73,25.18,24.56,23.84,23.01, !C & 22.05,20.97,19.85,18.77,17.78,16.89,16.10,15.39,14.74,14.14, !C & 13.59,13.06,12.56,12.09,11.65,11.22,10.81,10.42,10.03, 9.66, !C & 9.30, 8.94, 8.59, 8.25, 7.92, 7.59, 7.27, 6.95, 6.63, 6.32, !C & 6.01, 5.70, 5.39, 5.08, 4.78, 4.47, 4.17, 3.86, 3.56, 3.25, !C & 2.94, 2.62, 2.30, 1.98, 1.65, 1.32, 0.97, 0.62, 0.26, 0.13/ !C !C awss= sodium sulfate !C !C DATA AWSS/34*1.e5,23*14.30,14.21,12.53,11.47, !C & 10.66,10.01, 9.46, 8.99, 8.57, 8.19, 7.85, 7.54, 7.25, 6.98, !C & 6.74, 6.50, 6.29, 6.08, 5.88, 5.70, 5.52, 5.36, 5.20, 5.04, !C & 4.90, 4.75, 4.54, 4.34, 4.14, 3.93, 3.71, 3.49, 3.26, 3.02, !C & 2.76, 2.49, 2.20, 1.89, 1.55, 1.18, 0.82, 0.49, 0.22, 0.001/ !C !C awab= ammonium bisulfate !C !C DATA AWAB/356.45,296.51,253.21,220.47,194.85, !C & 174.24,157.31,143.16,131.15,120.82, !C & 111.86,103.99,97.04,90.86,85.31,80.31,75.78,71.66,67.90,64.44, !C & 61.25,58.31,55.58,53.04,50.68,48.47,46.40,44.46,42.63,40.91, !C & 39.29,37.75,36.30,34.92,33.61,32.36,31.18,30.04,28.96,27.93, !C & 26.94,25.99,25.08,24.21,23.37,22.57,21.79,21.05,20.32,19.63, !C & 18.96,18.31,17.68,17.07,16.49,15.92,15.36,14.83,14.31,13.80, !C & 13.31,12.83,12.36,11.91,11.46,11.03,10.61,10.20, 9.80, 9.41, !C & 9.02, 8.64, 8.28, 7.91, 7.56, 7.21, 6.87, 6.54, 6.21, 5.88, !C & 5.56, 5.25, 4.94, 4.63, 4.33, 4.03, 3.73, 3.44, 3.14, 2.85, !C & 2.57, 2.28, 1.99, 1.71, 1.42, 1.14, 0.86, 0.57, 0.29, 0.001/ !C !C awsa= sulfuric acid !C !C DATA AWSA/ !C & 34.0,33.56,29.22,26.55,24.61,23.11,21.89,20.87,19.99, !C & 19.21,18.51,17.87,17.29,16.76,16.26,15.8,15.37,14.95,14.56, !C & 14.20,13.85,13.53,13.22,12.93,12.66,12.40,12.14,11.90,11.67, !C & 11.44,11.22,11.01,10.8,10.60,10.4,10.2,10.01,9.83,9.65,9.47, !C & 9.3,9.13,8.96,8.81,8.64,8.48,8.33,8.17,8.02,7.87,7.72,7.58, !C & 7.44,7.30,7.16,7.02,6.88,6.75,6.61,6.48,6.35,6.21,6.08,5.95, !C & 5.82,5.69,5.56,5.44,5.31,5.18,5.05,4.92,4.79,4.66,4.53,4.40, !C & 4.27,4.14,4.,3.87,3.73,3.6,3.46,3.31,3.17,3.02,2.87,2.72, !C & 2.56,2.4,2.23,2.05,1.87,1.68,1.48,1.27,1.05,0.807,0.552,0.281/ !C !C awlc= (NH4)3H(SO4)2 !C !C DATA AWLC/34*1.e5,17.0,16.5,15.94,15.31,14.71,14.14, !C & 13.60,13.08,12.59,12.12,11.68,11.25,10.84,10.44,10.07, 9.71, !C & 9.36, 9.02, 8.70, 8.39, 8.09, 7.80, 7.52, 7.25, 6.99, 6.73, !C & 6.49, 6.25, 6.02, 5.79, 5.57, 5.36, 5.15, 4.95, 4.76, 4.56, !C & 4.38, 4.20, 4.02, 3.84, 3.67, 3.51, 3.34, 3.18, 3.02, 2.87, !C & 2.72, 2.57, 2.42, 2.28, 2.13, 1.99, 1.85, 1.71, 1.57, 1.43, !C & 1.30, 1.16, 1.02, 0.89, 0.75, 0.61, 0.46, 0.32, 0.16, 0.001/ !C !C awan= ammonium nitrate !C !C DATA AWAN/31*1.e5, !C & 97.17,92.28,87.66,83.15,78.87,74.84,70.98,67.46,64.11, !C & 60.98,58.07,55.37,52.85,50.43,48.24,46.19,44.26,42.40,40.70, !C & 39.10,37.54,36.10,34.69,33.35,32.11,30.89,29.71,28.58,27.46, !C & 26.42,25.37,24.33,23.89,22.42,21.48,20.56,19.65,18.76,17.91, !C & 17.05,16.23,15.40,14.61,13.82,13.03,12.30,11.55,10.83,10.14, !C & 9.44, 8.79, 8.13, 7.51, 6.91, 6.32, 5.75, 5.18, 4.65, 4.14, !C & 3.65, 3.16, 2.71, 2.26, 1.83, 1.42, 1.03, 0.66, 0.30, 0.001/ !C !C awsb= sodium bisulfate !C !C DATA AWSB/173.72,156.88,142.80,130.85,120.57, !C & 111.64,103.80,96.88,90.71,85.18, !C & 80.20,75.69,71.58,67.82,64.37,61.19,58.26,55.53,53.00,50.64, !C & 48.44,46.37,44.44,42.61,40.90,39.27,37.74,36.29,34.91,33.61, !C & 32.36,31.18,30.05,28.97,27.94,26.95,26.00,25.10,24.23,23.39, !C & 22.59,21.81,21.07,20.35,19.65,18.98,18.34,17.71,17.11,16.52, !C & 15.95,15.40,14.87,14.35,13.85,13.36,12.88,12.42,11.97,11.53, !C & 11.10,10.69,10.28, 9.88, 9.49, 9.12, 8.75, 8.38, 8.03, 7.68, !C & 7.34, 7.01, 6.69, 6.37, 6.06, 5.75, 5.45, 5.15, 4.86, 4.58, !C & 4.30, 4.02, 3.76, 3.49, 3.23, 2.98, 2.73, 2.48, 2.24, 2.01, !C & 1.78, 1.56, 1.34, 1.13, 0.92, 0.73, 0.53, 0.35, 0.17, 0.001/ !C !C *** END OF BLOCK DATA SUBPROGRAM ************************************* !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE INIT1 !C *** THIS SUBROUTINE INITIALIZES ALL GLOBAL VARIABLES FOR AMMONIUM !C SULFATE AEROSOL SYSTEMS (SUBROUTINE ISRP1) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE INIT12p1 (WI, RHI, TEMPI) INCLUDE 'module_isrpia_inc.F' DIMENSION WI(NCOMP) REAL IC,GII,GI0,XX,LN10 PARAMETER (LN10=2.3025851) !C !C *** SAVE INPUT VARIABLES IN COMMON BLOCK ****************************** !C IF (IPROB.EQ.0) THEN ! FORWARD CALCULATION DO 10 I=1,NCOMP W(I) = MAX(WI(I), TINY) 10 CONTINUE ELSE DO 15 I=1,NCOMP ! REVERSE CALCULATION WAER(I) = MAX(WI(I), TINY) W(I) = ZERO 15 CONTINUE ENDIF RH = RHI TEMP = TEMPI !C !C *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !C XK1 = 1.015e-2 ! HSO4(aq) <==> H(aq) + SO4(aq) XK21 = 57.639 ! NH3(g) <==> NH3(aq) XK22 = 1.805e-5 ! NH3(aq) <==> NH4(aq) + OH(aq) XK7 = 1.817 ! (NH4)2SO4(s) <==> 2*NH4(aq) + SO4(aq) XK12 = 1.382e2 ! NH4HSO4(s) <==> NH4(aq) + HSO4(aq) XK13 = 29.268 ! (NH4)3H(SO4)2(s) <==> 3*NH4(aq) + HSO4(aq) + SO4(aq) XKW = 1.010e-14 ! H2O <==> H(aq) + OH(aq) !C IF (INT(TEMP) .NE. 298) THEN ! FOR T != 298K or 298.15K T0 = 298.15 T0T = T0/TEMP COEF= 1.0+LOG(T0T)-T0T XK1 = XK1 *EXP( 8.85*(T0T-1.0) + 25.140*COEF) XK21= XK21*EXP( 13.79*(T0T-1.0) - 5.393*COEF) XK22= XK22*EXP( -1.50*(T0T-1.0) + 26.920*COEF) XK7 = XK7 *EXP( -2.65*(T0T-1.0) + 38.570*COEF) XK12= XK12*EXP( -2.87*(T0T-1.0) + 15.830*COEF) XK13= XK13*EXP( -5.19*(T0T-1.0) + 54.400*COEF) XKW = XKW *EXP(-22.52*(T0T-1.0) + 26.920*COEF) ENDIF XK2 = XK21*XK22 !C !C *** CALCULATE DELIQUESCENCE RELATIVE HUMIDITIES (UNICOMPONENT) ******** !C DRH2SO4 = 0.0000D0 DRNH42S4 = 0.7997D0 DRNH4HS4 = 0.4000D0 DRLC = 0.6900D0 IF (INT(TEMP) .NE. 298) THEN T0 = 298.15d0 TCF = 1.0/TEMP - 1.0/T0 DRNH42S4 = DRNH42S4*EXP( 80.*TCF) DRNH4HS4 = DRNH4HS4*EXP(384.*TCF) DRLC = DRLC *EXP(186.*TCF) ENDIF !C !C *** CALCULATE MUTUAL DELIQUESCENCE RELATIVE HUMIDITIES **************** !C DRMLCAB = 0.3780D0 ! (NH4)3H(SO4)2 & NH4HSO4 DRMLCAS = 0.6900D0 ! (NH4)3H(SO4)2 & (NH4)2SO4 !!CCC IF (INT(TEMP) .NE. 298) THEN ! For the time being. !CCC T0 = 298.15d0 !CCC TCF = 1.0/TEMP - 1.0/T0 !CCC DRMLCAB = DRMLCAB*EXP(507.506*TCF) !CCC DRMLCAS = DRMLCAS*EXP(133.865*TCF) !CCC ENDIF !C !C *** LIQUID PHASE ****************************************************** !C CHNO3 = ZERO CHCL = ZERO CH2SO4 = ZERO COH = ZERO WATER = TINY !C DO 20 I=1,NPAIR MOLALR(I)=ZERO GAMA(I) =0.1 GAMIN(I) =GREAT GAMOU(I) =GREAT M0(I) =1d5 20 CONTINUE !C DO 30 I=1,NPAIR GAMA(I) = 0.1d0 30 CONTINUE !C DO 40 I=1,NIONS MOLAL(I)=ZERO 40 CONTINUE COH = ZERO !C DO 50 I=1,NGASAQ GASAQ(I)=ZERO 50 CONTINUE !C !C *** SOLID PHASE ******************************************************* !C CNH42S4= ZERO CNH4HS4= ZERO CNACL = ZERO CNA2SO4= ZERO CNANO3 = ZERO CNH4NO3= ZERO CNH4CL = ZERO CNAHSO4= ZERO CLC = ZERO CCASO4 = ZERO CCANO32= ZERO CCACL2 = ZERO CK2SO4 = ZERO CKHSO4 = ZERO CKNO3 = ZERO CKCL = ZERO CMGSO4 = ZERO CMGNO32= ZERO CMGCL2 = ZERO !C !C *** GAS PHASE ********************************************************* !C GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO !C !C *** CALCULATE ZSR PARAMETERS ****************************************** !C IRH = MIN (INT(RH*NZSR+0.5),NZSR) ! Position in ZSR arrays IRH = MAX (IRH, 1) !C !C M0(01) = AWSC(IRH) ! NACl !C IF (M0(01) .LT. 100.0) THEN !C IC = M0(01) !C CALL KMTAB(IC,298.0, GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(01) = M0(01)*EXP(LN10*(GI0-GII)) !C ENDIF !CC !C M0(02) = AWSS(IRH) ! (NA)2SO4 !C IF (M0(02) .LT. 100.0) THEN !C IC = 3.0*M0(02) !C CALL KMTAB(IC,298.0, XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(02) = M0(02)*EXP(LN10*(GI0-GII)) !C ENDIF !CC !C M0(03) = AWSN(IRH) ! NANO3 !C IF (M0(03) .LT. 100.0) THEN !C IC = M0(03) !C CALL KMTAB(IC,298.0, XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(03) = M0(03)*EXP(LN10*(GI0-GII)) !C ENDIF !CC M0(04) = AWAS(IRH) ! (NH4)2SO4 !CC IF (M0(04) .LT. 100.0) THEN !CC IC = 3.0*M0(04) !C !C CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(04) = M0(04)*EXP(LN10*(GI0-GII)) !CC ENDIF !C !C M0(05) = AWAN(IRH) ! NH4NO3 !C IF (M0(05) .LT. 100.0) THEN !C IC = M0(05) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(05) = M0(05)*EXP(LN10*(GI0-GII)) !C ENDIF !CC !C M0(06) = AWAC(IRH) ! NH4CL !C IF (M0(06) .LT. 100.0) THEN !C IC = M0(06) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(06) = M0(06)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(07) = AWSA(IRH) ! 2H-SO4 !CC IF (M0(07) .LT. 100.0) THEN !CC IC = 3.0*M0(07) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(07) = M0(07)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(08) = AWSA(IRH) ! H-HSO4 !CCC IF (M0(08) .LT. 100.0) THEN ! These are redundant, because M0(8) is not used !CCC IC = M0(08) !CCC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCCCCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX) !CCC M0(08) = M0(08)*EXP(LN10*(GI0-GII)) !CCC ENDIF !C M0(09) = AWAB(IRH) ! NH4HSO4 !CC IF (M0(09) .LT. 100.0) THEN !CC IC = M0(09) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(09) = M0(09)*EXP(LN10*(GI0-GII)) !CC ENDIF !C !C M0(12) = AWSB(IRH) ! NAHSO4 !C IF (M0(12) .LT. 100.0) THEN !C IC = M0(12) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GI0, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GII, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(12) = M0(12)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(13) = AWLC(IRH) ! (NH4)3H(SO4)2 !CC IF (M0(13) .LT. 100.0) THEN !CC IC = 4.0*M0(13) !CC CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC G130 = 0.2*(3.0*GI0+2.0*GII) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC G13I = 0.2*(3.0*GI0+2.0*GII) !CC M0(13) = M0(13)*EXP(LN10*SNGL(G130-G13I)) !CC ENDIF !C !C *** OTHER INITIALIZATIONS ********************************************* !C ICLACT = 0 CALAOU = .TRUE. CALAIN = .TRUE. FRST = .TRUE. !liqy ! SCASE = '??' SCASE = 'xx' !liqy-20140513 SULRATW = 2.D0 SODRAT = ZERO CRNARAT = ZERO CRRAT = ZERO NOFER = 0 STKOFL =.FALSE. DO 60 I=1,NERRMX ERRSTK(I) =-999 ERRMSG(I) = 'MESSAGE N/A' 60 CONTINUE !C !C *** END OF SUBROUTINE INIT1 ******************************************* !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE INIT2 !C *** THIS SUBROUTINE INITIALIZES ALL GLOBAL VARIABLES FOR AMMONIUM, !C NITRATE, SULFATE AEROSOL SYSTEMS (SUBROUTINE ISRP2) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE INIT22p1 (WI, RHI, TEMPI) INCLUDE 'module_isrpia_inc.F' DIMENSION WI(NCOMP) REAL IC,GII,GI0,XX,LN10 PARAMETER (LN10=2.3025851) !C !C *** SAVE INPUT VARIABLES IN COMMON BLOCK ****************************** !C IF (IPROB.EQ.0) THEN ! FORWARD CALCULATION DO 10 I=1,NCOMP W(I) = MAX(WI(I), TINY) 10 CONTINUE ELSE DO 15 I=1,NCOMP ! REVERSE CALCULATION WAER(I) = MAX(WI(I), TINY) W(I) = ZERO 15 CONTINUE ENDIF RH = RHI TEMP = TEMPI !C !C *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !C XK1 = 1.015e-2 ! HSO4(aq) <==> H(aq) + SO4(aq) XK21 = 57.639 ! NH3(g) <==> NH3(aq) XK22 = 1.805e-5 ! NH3(aq) <==> NH4(aq) + OH(aq) XK4 = 2.511e6 ! HNO3(g) <==> H(aq) + NO3(aq) ! ISORR !CCC XK4 = 3.638e6 ! HNO3(g) <==> H(aq) + NO3(aq) ! SEQUIL XK41 = 2.100e5 ! HNO3(g) <==> HNO3(aq) XK7 = 1.817 ! (NH4)2SO4(s) <==> 2*NH4(aq) + SO4(aq) XK10 = 5.746e-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! ISORR !CCC XK10 = 2.985e-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! SEQUIL XK12 = 1.382e2 ! NH4HSO4(s) <==> NH4(aq) + HSO4(aq) XK13 = 29.268 ! (NH4)3H(SO4)2(s) <==> 3*NH4(aq) + HSO4(aq) + SO4(aq) XKW = 1.010e-14 ! H2O <==> H(aq) + OH(aq) !C IF (INT(TEMP) .NE. 298) THEN ! FOR T != 298K or 298.15K T0 = 298.15D0 T0T = T0/TEMP COEF= 1.0+LOG(T0T)-T0T XK1 = XK1 *EXP( 8.85*(T0T-1.0) + 25.140*COEF) XK21= XK21*EXP( 13.79*(T0T-1.0) - 5.393*COEF) XK22= XK22*EXP( -1.50*(T0T-1.0) + 26.920*COEF) XK4 = XK4 *EXP( 29.17*(T0T-1.0) + 16.830*COEF) !ISORR !CCC XK4 = XK4 *EXP( 29.47*(T0T-1.0) + 16.840*COEF) ! SEQUIL XK41= XK41*EXP( 29.17*(T0T-1.0) + 16.830*COEF) XK7 = XK7 *EXP( -2.65*(T0T-1.0) + 38.570*COEF) XK10= XK10*EXP(-74.38*(T0T-1.0) + 6.120*COEF) ! ISORR !CCC XK10= XK10*EXP(-75.11*(T0T-1.0) + 13.460*COEF) ! SEQUIL XK12= XK12*EXP( -2.87*(T0T-1.0) + 15.830*COEF) XK13= XK13*EXP( -5.19*(T0T-1.0) + 54.400*COEF) XKW = XKW *EXP(-22.52*(T0T-1.0) + 26.920*COEF) ENDIF XK2 = XK21*XK22 XK42 = XK4/XK41 !C !C *** CALCULATE DELIQUESCENCE RELATIVE HUMIDITIES (UNICOMPONENT) ******** !C DRH2SO4 = ZERO DRNH42S4 = 0.7997D0 DRNH4HS4 = 0.4000D0 DRNH4NO3 = 0.6183D0 DRLC = 0.6900D0 IF (INT(TEMP) .NE. 298) THEN T0 = 298.15D0 TCF = 1.0/TEMP - 1.0/T0 DRNH4NO3 = DRNH4NO3*EXP(852.*TCF) DRNH42S4 = DRNH42S4*EXP( 80.*TCF) DRNH4HS4 = DRNH4HS4*EXP(384.*TCF) DRLC = DRLC *EXP(186.*TCF) DRNH4NO3 = MIN (DRNH4NO3,DRNH42S4) ! ADJUST FOR DRH CROSSOVER AT T<271K ENDIF !C !C *** CALCULATE MUTUAL DELIQUESCENCE RELATIVE HUMIDITIES **************** !C DRMLCAB = 0.3780D0 ! (NH4)3H(SO4)2 & NH4HSO4 DRMLCAS = 0.6900D0 ! (NH4)3H(SO4)2 & (NH4)2SO4 DRMASAN = 0.6000D0 ! (NH4)2SO4 & NH4NO3 !CCC IF (INT(TEMP) .NE. 298) THEN ! For the time being !CCC T0 = 298.15d0 !CCC TCF = 1.0/TEMP - 1.0/T0 !CCC DRMLCAB = DRMLCAB*EXP( 507.506*TCF) !CCC DRMLCAS = DRMLCAS*EXP( 133.865*TCF) !CCC DRMASAN = DRMASAN*EXP(1269.068*TCF) !CCC ENDIF !C !C *** LIQUID PHASE ****************************************************** !C CHNO3 = ZERO CHCL = ZERO CH2SO4 = ZERO COH = ZERO WATER = TINY !C DO 20 I=1,NPAIR MOLALR(I)=ZERO GAMA(I) =0.1 GAMIN(I) =GREAT GAMOU(I) =GREAT M0(I) =1d5 20 CONTINUE !C DO 30 I=1,NPAIR GAMA(I) = 0.1d0 30 CONTINUE !C DO 40 I=1,NIONS MOLAL(I)=ZERO 40 CONTINUE COH = ZERO !C DO 50 I=1,NGASAQ GASAQ(I)=ZERO 50 CONTINUE !C !C *** SOLID PHASE ****************************************************** !C CNH42S4= ZERO CNH4HS4= ZERO CNACL = ZERO CNA2SO4= ZERO CNANO3 = ZERO CNH4NO3= ZERO CNH4CL = ZERO CNAHSO4= ZERO CLC = ZERO CCASO4 = ZERO CCANO32= ZERO CCACL2 = ZERO CK2SO4 = ZERO CKHSO4 = ZERO CKNO3 = ZERO CKCL = ZERO CMGSO4 = ZERO CMGNO32= ZERO CMGCL2 = ZERO !C !C *** GAS PHASE ******************************************************** !C GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO !C !C *** CALCULATE ZSR PARAMETERS ***************************************** !C IRH = MIN (INT(RH*NZSR+0.5),NZSR) ! Position in ZSR arrays IRH = MAX (IRH, 1) !C !C M0(01) = AWSC(IRH) ! NACl !C IF (M0(01) .LT. 100.0) THEN !C IC = M0(01) !C CALL KMTAB(IC,298.0, GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(01) = M0(01)*EXP(LN10*(GI0-GII)) !C ENDIF !CC !C M0(02) = AWSS(IRH) ! (NA)2SO4 !C IF (M0(02) .LT. 100.0) THEN !C IC = 3.0*M0(02) !C CALL KMTAB(IC,298.0, XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(02) = M0(02)*EXP(LN10*(GI0-GII)) !C ENDIF !CCC !C M0(03) = AWSN(IRH) ! NANO3 !C IF (M0(03) .LT. 100.0) THEN !C IC = M0(03) !C CALL KMTAB(IC,298.0, XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(03) = M0(03)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(04) = AWAS(IRH) ! (NH4)2SO4 !CC IF (M0(04) .LT. 100.0) THEN !CC IC = 3.0*M0(04) !CC CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(04) = M0(04)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(05) = AWAN(IRH) ! NH4NO3 !CC IF (M0(05) .LT. 100.0) THEN !CC IC = M0(05) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(05) = M0(05)*EXP(LN10*(GI0-GII)) !CC ENDIF !C !C M0(06) = AWAC(IRH) ! NH4CL !C IF (M0(06) .LT. 100.0) THEN !C IC = M0(06) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(06) = M0(06)*EXP(LN10*(GI0-GII)) !C ENDIF !CC M0(07) = AWSA(IRH) ! 2H-SO4 !CC IF (M0(07) .LT. 100.0) THEN !CC IC = 3.0*M0(07) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(07) = M0(07)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(08) = AWSA(IRH) ! H-HSO4 !CCC IF (M0(08) .LT. 100.0) THEN ! These are redundant, because M0(8) is not used !CCC IC = M0(08) !CCC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCCCCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX) !CCC M0(08) = M0(08)*EXP(LN10*(GI0-GII)) !CCC ENDIF !C M0(09) = AWAB(IRH) ! NH4HSO4 !CC IF (M0(09) .LT. 100.0) THEN !CC IC = M0(09) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(09) = M0(09)*EXP(LN10*(GI0-GII)) !CC ENDIF !C !C M0(12) = AWSB(IRH) ! NAHSO4 !C IF (M0(12) .LT. 100.0) THEN !C IC = M0(12) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GI0, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GII, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(12) = M0(12)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(13) = AWLC(IRH) ! (NH4)3H(SO4)2 !C IF (M0(13) .LT. 100.0) THEN !C IC = 4.0*M0(13) !C CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C G130 = 0.2*(3.0*GI0+2.0*GII) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C G13I = 0.2*(3.0*GI0+2.0*GII) !C M0(13) = M0(13)*EXP(LN10*SNGL(G130-G13I)) !C ENDIF !C !C *** OTHER INITIALIZATIONS ********************************************* !C ICLACT = 0 CALAOU = .TRUE. CALAIN = .TRUE. FRST = .TRUE. !liqy ! SCASE = '??' SCASE = 'xx' !liqy-20140513 SULRATW = 2.D0 SODRAT = ZERO CRNARAT = ZERO CRRAT = ZERO NOFER = 0 STKOFL =.FALSE. DO 60 I=1,NERRMX ERRSTK(I) =-999 ERRMSG(I) = 'MESSAGE N/A' 60 CONTINUE !C !C *** END OF SUBROUTINE INIT2 ******************************************* !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE ISOINIT3 !C *** THIS SUBROUTINE INITIALIZES ALL GLOBAL VARIABLES FOR AMMONIUM, !C SODIUM, CHLORIDE, NITRATE, SULFATE AEROSOL SYSTEMS (SUBROUTINE !C ISRP3) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE ISOINIT32p1 (WI, RHI, TEMPI) INCLUDE 'module_isrpia_inc.F' DIMENSION WI(NCOMP) REAL IC,GII,GI0,XX,LN10 PARAMETER (LN10=2.3025851) !C !C *** SAVE INPUT VARIABLES IN COMMON BLOCK ****************************** !C IF (IPROB.EQ.0) THEN ! FORWARD CALCULATION DO 10 I=1,NCOMP W(I) = MAX(WI(I), TINY) 10 CONTINUE ELSE DO 15 I=1,NCOMP ! REVERSE CALCULATION WAER(I) = MAX(WI(I), TINY) W(I) = ZERO 15 CONTINUE ENDIF RH = RHI TEMP = TEMPI !C !C *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !C XK1 = 1.015D-2 ! HSO4(aq) <==> H(aq) + SO4(aq) XK21 = 57.639D0 ! NH3(g) <==> NH3(aq) XK22 = 1.805D-5 ! NH3(aq) <==> NH4(aq) + OH(aq) XK3 = 1.971D6 ! HCL(g) <==> H(aq) + CL(aq) XK31 = 2.500e3 ! HCL(g) <==> HCL(aq) XK4 = 2.511e6 ! HNO3(g) <==> H(aq) + NO3(aq) ! ISORR !CCC XK4 = 3.638e6 ! HNO3(g) <==> H(aq) + NO3(aq) ! SEQUIL XK41 = 2.100e5 ! HNO3(g) <==> HNO3(aq) XK5 = 0.4799D0 ! NA2SO4(s) <==> 2*NA(aq) + SO4(aq) XK6 = 1.086D-16 ! NH4CL(s) <==> NH3(g) + HCL(g) XK7 = 1.817D0 ! (NH4)2SO4(s) <==> 2*NH4(aq) + SO4(aq) XK8 = 37.661D0 ! NACL(s) <==> NA(aq) + CL(aq) XK10 = 5.746D-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! ISORR !CCC XK10 = 2.985e-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! SEQUIL XK11 = 2.413D4 ! NAHSO4(s) <==> NA(aq) + HSO4(aq) XK12 = 1.382D2 ! NH4HSO4(s) <==> NH4(aq) + HSO4(aq) XK13 = 29.268D0 ! (NH4)3H(SO4)2(s) <==> 3*NH4(aq) + HSO4(aq) + SO4(aq) XK14 = 22.05D0 ! NH4CL(s) <==> NH4(aq) + CL(aq) XKW = 1.010D-14 ! H2O <==> H(aq) + OH(aq) XK9 = 11.977D0 ! NANO3(s) <==> NA(aq) + NO3(aq) !C IF (INT(TEMP) .NE. 298) THEN ! FOR T != 298K or 298.15K T0 = 298.15D0 T0T = T0/TEMP COEF= 1.0+LOG(T0T)-T0T XK1 = XK1 *EXP( 8.85*(T0T-1.0) + 25.140*COEF) XK21= XK21*EXP( 13.79*(T0T-1.0) - 5.393*COEF) XK22= XK22*EXP( -1.50*(T0T-1.0) + 26.920*COEF) XK3 = XK3 *EXP( 30.20*(T0T-1.0) + 19.910*COEF) XK31= XK31*EXP( 30.20*(T0T-1.0) + 19.910*COEF) XK4 = XK4 *EXP( 29.17*(T0T-1.0) + 16.830*COEF) !ISORR !CCC XK4 = XK4 *EXP( 29.47*(T0T-1.0) + 16.840*COEF) ! SEQUIL XK41= XK41*EXP( 29.17*(T0T-1.0) + 16.830*COEF) XK5 = XK5 *EXP( 0.98*(T0T-1.0) + 39.500*COEF) XK6 = XK6 *EXP(-71.00*(T0T-1.0) + 2.400*COEF) XK7 = XK7 *EXP( -2.65*(T0T-1.0) + 38.570*COEF) XK8 = XK8 *EXP( -1.56*(T0T-1.0) + 16.900*COEF) XK9 = XK9 *EXP( -8.22*(T0T-1.0) + 16.010*COEF) XK10= XK10*EXP(-74.38*(T0T-1.0) + 6.120*COEF) ! ISORR !CCC XK10= XK10*EXP(-75.11*(T0T-1.0) + 13.460*COEF) ! SEQUIL XK11= XK11*EXP( 0.79*(T0T-1.0) + 14.746*COEF) XK12= XK12*EXP( -2.87*(T0T-1.0) + 15.830*COEF) XK13= XK13*EXP( -5.19*(T0T-1.0) + 54.400*COEF) XK14= XK14*EXP( 24.55*(T0T-1.0) + 16.900*COEF) XKW = XKW *EXP(-22.52*(T0T-1.0) + 26.920*COEF) ENDIF XK2 = XK21*XK22 XK42 = XK4/XK41 XK32 = XK3/XK31 !C !C *** CALCULATE DELIQUESCENCE RELATIVE HUMIDITIES (UNICOMPONENT) ******** !C DRH2SO4 = ZERO DRNH42S4 = 0.7997D0 DRNH4HS4 = 0.4000D0 DRLC = 0.6900D0 DRNACL = 0.7528D0 DRNANO3 = 0.7379D0 DRNH4CL = 0.7710D0 DRNH4NO3 = 0.6183D0 DRNA2SO4 = 0.9300D0 DRNAHSO4 = 0.5200D0 IF (INT(TEMP) .NE. 298) THEN T0 = 298.15D0 TCF = 1.0/TEMP - 1.0/T0 DRNACL = DRNACL *EXP( 25.*TCF) DRNANO3 = DRNANO3 *EXP(304.*TCF) DRNA2SO4 = DRNA2SO4*EXP( 80.*TCF) DRNH4NO3 = DRNH4NO3*EXP(852.*TCF) DRNH42S4 = DRNH42S4*EXP( 80.*TCF) DRNH4HS4 = DRNH4HS4*EXP(384.*TCF) DRLC = DRLC *EXP(186.*TCF) DRNH4CL = DRNH4Cl *EXP(239.*TCF) DRNAHSO4 = DRNAHSO4*EXP(-45.*TCF) !C !C *** ADJUST FOR DRH "CROSSOVER" AT LOW TEMPERATURES !C DRNH4NO3 = MIN (DRNH4NO3, DRNH4CL, DRNH42S4, DRNANO3, DRNACL) DRNANO3 = MIN (DRNANO3, DRNACL) DRNH4CL = MIN (DRNH4Cl, DRNH42S4) !C ENDIF !C !C *** CALCULATE MUTUAL DELIQUESCENCE RELATIVE HUMIDITIES **************** !C DRMLCAB = 0.378D0 ! (NH4)3H(SO4)2 & NH4HSO4 DRMLCAS = 0.690D0 ! (NH4)3H(SO4)2 & (NH4)2SO4 DRMASAN = 0.600D0 ! (NH4)2SO4 & NH4NO3 DRMG1 = 0.460D0 ! (NH4)2SO4, NH4NO3, NA2SO4, NH4CL DRMG2 = 0.691D0 ! (NH4)2SO4, NA2SO4, NH4CL DRMG3 = 0.697D0 ! (NH4)2SO4, NA2SO4 DRMH1 = 0.240D0 ! NA2SO4, NANO3, NACL, NH4NO3, NH4CL DRMH2 = 0.596D0 ! NA2SO4, NANO3, NACL, NH4CL DRMI1 = 0.240D0 ! LC, NAHSO4, NH4HSO4, NA2SO4, (NH4)2SO4 DRMI2 = 0.363D0 ! LC, NAHSO4, NA2SO4, (NH4)2SO4 - NO DATA - DRMI3 = 0.610D0 ! LC, NA2SO4, (NH4)2SO4 DRMQ1 = 0.494D0 ! (NH4)2SO4, NH4NO3, NA2SO4 DRMR1 = 0.663D0 ! NA2SO4, NANO3, NACL DRMR2 = 0.735D0 ! NA2SO4, NACL DRMR3 = 0.673D0 ! NANO3, NACL DRMR4 = 0.694D0 ! NA2SO4, NACL, NH4CL DRMR5 = 0.731D0 ! NA2SO4, NH4CL DRMR6 = 0.596D0 ! NA2SO4, NANO3, NH4CL DRMR7 = 0.380D0 ! NA2SO4, NANO3, NACL, NH4NO3 DRMR8 = 0.380D0 ! NA2SO4, NACL, NH4NO3 DRMR9 = 0.494D0 ! NA2SO4, NH4NO3 DRMR10 = 0.476D0 ! NA2SO4, NANO3, NH4NO3 DRMR11 = 0.340D0 ! NA2SO4, NACL, NH4NO3, NH4CL DRMR12 = 0.460D0 ! NA2SO4, NH4NO3, NH4CL DRMR13 = 0.438D0 ! NA2SO4, NANO3, NH4NO3, NH4CL !CCC IF (INT(TEMP) .NE. 298) THEN !CCC T0 = 298.15d0 !CCC TCF = 1.0/TEMP - 1.0/T0 !CCC DRMLCAB = DRMLCAB*EXP( 507.506*TCF) !CCC DRMLCAS = DRMLCAS*EXP( 133.865*TCF) !CCC DRMASAN = DRMASAN*EXP(1269.068*TCF) !CCC DRMG1 = DRMG1 *EXP( 572.207*TCF) !CCC DRMG2 = DRMG2 *EXP( 58.166*TCF) !CCC DRMG3 = DRMG3 *EXP( 22.253*TCF) !CCC DRMH1 = DRMH1 *EXP(2116.542*TCF) !CCC DRMH2 = DRMH2 *EXP( 650.549*TCF) !CCC DRMI1 = DRMI1 *EXP( 565.743*TCF) !CCC DRMI2 = DRMI2 *EXP( 91.745*TCF) !CCC DRMI3 = DRMI3 *EXP( 161.272*TCF) !CCC DRMQ1 = DRMQ1 *EXP(1616.621*TCF) !CCC DRMR1 = DRMR1 *EXP( 292.564*TCF) !CCC DRMR2 = DRMR2 *EXP( 14.587*TCF) !CCC DRMR3 = DRMR3 *EXP( 307.907*TCF) !CCC DRMR4 = DRMR4 *EXP( 97.605*TCF) !CCC DRMR5 = DRMR5 *EXP( 98.523*TCF) !CCC DRMR6 = DRMR6 *EXP( 465.500*TCF) !CCC DRMR7 = DRMR7 *EXP( 324.425*TCF) !CCC DRMR8 = DRMR8 *EXP(2660.184*TCF) !CCC DRMR9 = DRMR9 *EXP(1617.178*TCF) !CCC DRMR10 = DRMR10 *EXP(1745.226*TCF) !CCC DRMR11 = DRMR11 *EXP(3691.328*TCF) !CCC DRMR12 = DRMR12 *EXP(1836.842*TCF) !CCC DRMR13 = DRMR13 *EXP(1967.938*TCF) !CCC ENDIF !C !C *** LIQUID PHASE ****************************************************** !C CHNO3 = ZERO CHCL = ZERO CH2SO4 = ZERO COH = ZERO WATER = TINY !C DO 20 I=1,NPAIR MOLALR(I)=ZERO GAMA(I) =0.1 GAMIN(I) =GREAT GAMOU(I) =GREAT M0(I) =1d5 20 CONTINUE !C DO 30 I=1,NPAIR GAMA(I) = 0.1d0 30 CONTINUE !C DO 40 I=1,NIONS MOLAL(I)=ZERO 40 CONTINUE COH = ZERO !C DO 50 I=1,NGASAQ GASAQ(I)=ZERO 50 CONTINUE !C !C *** SOLID PHASE ******************************************************* !C CNH42S4= ZERO CNH4HS4= ZERO CNACL = ZERO CNA2SO4= ZERO CNANO3 = ZERO CNH4NO3= ZERO CNH4CL = ZERO CNAHSO4= ZERO CLC = ZERO CCASO4 = ZERO CCANO32= ZERO CCACL2 = ZERO CK2SO4 = ZERO CKHSO4 = ZERO CKNO3 = ZERO CKCL = ZERO CMGSO4 = ZERO CMGNO32= ZERO CMGCL2 = ZERO !C !C *** GAS PHASE ********************************************************* !C GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO !C !C *** CALCULATE ZSR PARAMETERS ****************************************** !C IRH = MIN (INT(RH*NZSR+0.5),NZSR) ! Position in ZSR arrays IRH = MAX (IRH, 1) !C M0(01) = AWSC(IRH) ! NACl !CC IF (M0(01) .LT. 100.0) THEN !CC IC = M0(01) !CC CALL KMTAB(IC,298.0, GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(01) = M0(01)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(02) = AWSS(IRH) ! (NA)2SO4 !CC IF (M0(02) .LT. 100.0) THEN !CC IC = 3.0*M0(02) !CC CALL KMTAB(IC,298.0, XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(02) = M0(02)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(03) = AWSN(IRH) ! NANO3 !CC IF (M0(03) .LT. 100.0) THEN !CC IC = M0(03) !CC CALL KMTAB(IC,298.0, XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C !C M0(03) = M0(03)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(04) = AWAS(IRH) ! (NH4)2SO4 !CC IF (M0(04) .LT. 100.0) THEN !CC IC = 3.0*M0(04) !CC CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(04) = M0(04)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(05) = AWAN(IRH) ! NH4NO3 !CC IF (M0(05) .LT. 100.0) THEN !CC IC = M0(05) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(05) = M0(05)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(06) = AWAC(IRH) ! NH4CL !CC IF (M0(06) .LT. 100.0) THEN !CC IC = M0(06) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(06) = M0(06)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(07) = AWSA(IRH) ! 2H-SO4 !CC IF (M0(07) .LT. 100.0) THEN !CC IC = 3.0*M0(07) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(07) = M0(07)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(08) = AWSA(IRH) ! H-HSO4 !CCC IF (M0(08) .LT. 100.0) THEN ! These are redundant, because M0(8) is not used !CCC IC = M0(08) !CCC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCCCCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX) !CCC M0(08) = M0(08)*EXP(LN10*(GI0-GII)) !CCC ENDIF !C M0(09) = AWAB(IRH) ! NH4HSO4 !CC IF (M0(09) .LT. 100.0) THEN !CC IC = M0(09) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(09) = M0(09)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(12) = AWSB(IRH) ! NAHSO4 !CC IF (M0(12) .LT. 100.0) THEN !CC IC = M0(12) !CC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GI0, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GII, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC M0(12) = M0(12)*EXP(LN10*(GI0-GII)) !CC ENDIF !C M0(13) = AWLC(IRH) ! (NH4)3H(SO4)2 !CC IF (M0(13) .LT. 100.0) THEN !CC IC = 4.0*M0(13) !CC CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC G130 = 0.2*(3.0*GI0+2.0*GII) !CC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !CC & XX,XX,XX,XX,XX,XX,XX,XX,XX) !CC G13I = 0.2*(3.0*GI0+2.0*GII) !CC M0(13) = M0(13)*EXP(LN10*SNGL(G130-G13I)) !CC ENDIF !C !C *** OTHER INITIALIZATIONS ********************************************* !C ICLACT = 0 CALAOU = .TRUE. CALAIN = .TRUE. FRST = .TRUE. !liqy ! SCASE = '??' SCASE = 'xx' !liqy-20140513 SULRATW = 2.D0 CRNARAT = ZERO CRRAT = ZERO NOFER = 0 STKOFL =.FALSE. DO 60 I=1,NERRMX ERRSTK(I) =-999 ERRMSG(I) = 'MESSAGE N/A' 60 CONTINUE !C !C *** END OF SUBROUTINE ISOINIT3 ******************************************* !C END !C======================================================================= !C !C *** ISORROPIA CODE II !C *** SUBROUTINE INIT4 !C *** THIS SUBROUTINE INITIALIZES ALL GLOBAL VARIABLES FOR AMMONIUM, !C SODIUM, CHLORIDE, NITRATE, SULFATE, CALCIUM, POTASSIUM, MAGNESIUM !C AEROSOL SYSTEMS (SUBROUTINE ISRP4) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY CHRISTOS FOUNTOUKIS AND ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE INIT42p1 (WI, RHI, TEMPI) INCLUDE 'module_isrpia_inc.F' DIMENSION WI(NCOMP) REAL IC,GII,GI0,XX,LN10 PARAMETER (LN10=2.3025851) !C !C *** SAVE INPUT VARIABLES IN COMMON BLOCK ****************************** !C IF (IPROB.EQ.0) THEN ! FORWARD CALCULATION DO 10 I=1,NCOMP W(I) = MAX(WI(I), TINY) 10 CONTINUE ELSE DO 15 I=1,NCOMP ! REVERSE CALCULATION WAER(I) = MAX(WI(I), TINY) W(I) = ZERO 15 CONTINUE ENDIF RH = RHI TEMP = TEMPI !C !C *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !C XK1 = 1.015D-2 ! HSO4(aq) <==> H(aq) + SO4(aq) XK21 = 57.639D0 ! NH3(g) <==> NH3(aq) XK22 = 1.805D-5 ! NH3(aq) <==> NH4(aq) + OH(aq) XK3 = 1.971D6 ! HCL(g) <==> H(aq) + CL(aq) XK31 = 2.500e3 ! HCL(g) <==> HCL(aq) XK4 = 2.511e6 ! HNO3(g) <==> H(aq) + NO3(aq) ! ISORR !C XK4 = 3.638e6 ! HNO3(g) <==> H(aq) + NO3(aq) ! SEQUIL XK41 = 2.100e5 ! HNO3(g) <==> HNO3(aq) XK5 = 0.4799D0 ! NA2SO4(s) <==> 2*NA(aq) + SO4(aq) XK6 = 1.086D-16 ! NH4CL(s) <==> NH3(g) + HCL(g) XK7 = 1.817D0 ! (NH4)2SO4(s) <==> 2*NH4(aq) + SO4(aq) XK8 = 37.661D0 ! NACL(s) <==> NA(aq) + CL(aq) !C XK10 = 5.746D-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! ISORR XK10 = 4.199D-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! (Mozurkewich, 1993) !C XK10 = 2.985e-17 ! NH4NO3(s) <==> NH3(g) + HNO3(g) ! SEQUIL XK11 = 2.413D4 ! NAHSO4(s) <==> NA(aq) + HSO4(aq) XK12 = 1.382D2 ! NH4HSO4(s) <==> NH4(aq) + HSO4(aq) XK13 = 29.268D0 ! (NH4)3H(SO4)2(s) <==> 3*NH4(aq) + HSO4(aq) + SO4(aq) XK14 = 22.05D0 ! NH4CL(s) <==> NH4(aq) + CL(aq) XKW = 1.010D-14 ! H2O <==> H(aq) + OH(aq) XK9 = 11.977D0 ! NANO3(s) <==> NA(aq) + NO3(aq) !CCC XK15 = 6.067D5 ! CA(NO3)2(s) <==> CA(aq) + 2NO3(aq) XK16 = 7.974D11 ! CACL2(s) <==> CA(aq) + 2CL(aq) XK17 = 1.569D-2 ! K2SO4(s) <==> 2K(aq) + SO4(aq) XK18 = 24.016 ! KHSO4(s) <==> K(aq) + HSO4(aq) XK19 = 0.872 ! KNO3(s) <==> K(aq) + NO3(aq) XK20 = 8.680 ! KCL(s) <==> K(aq) + CL(aq) XK23 = 1.079D5 ! MGS04(s) <==> MG(aq) + SO4(aq) XK24 = 2.507D15 ! MG(NO3)2(s) <==> MG(aq) + 2NO3(aq) XK25 = 9.557D21 ! MGCL2(s) <==> MG(aq) + 2CL(aq) !C XK26 = 4.299D-7 ! CO2(aq) + H2O <==> HCO3(aq) + H(aq) !C XK27 = 4.678D-11 ! HCO3(aq) <==> CO3(aq) + H(aq) !C IF (INT(TEMP) .NE. 298) THEN ! FOR T != 298K or 298.15K T0 = 298.15D0 T0T = T0/TEMP COEF= 1.0+LOG(T0T)-T0T XK1 = XK1 *EXP( 8.85*(T0T-1.0) + 25.140*COEF) XK21= XK21*EXP( 13.79*(T0T-1.0) - 5.393*COEF) XK22= XK22*EXP( -1.50*(T0T-1.0) + 26.920*COEF) XK3 = XK3 *EXP( 30.20*(T0T-1.0) + 19.910*COEF) XK31= XK31*EXP( 30.20*(T0T-1.0) + 19.910*COEF) XK4 = XK4 *EXP( 29.17*(T0T-1.0) + 16.830*COEF) !ISORR !C XK4 = XK4 *EXP( 29.47*(T0T-1.0) + 16.840*COEF) ! SEQUIL XK41= XK41*EXP( 29.17*(T0T-1.0) + 16.830*COEF) XK5 = XK5 *EXP( 0.98*(T0T-1.0) + 39.500*COEF) XK6 = XK6 *EXP(-71.00*(T0T-1.0) + 2.400*COEF) XK7 = XK7 *EXP( -2.65*(T0T-1.0) + 38.570*COEF) XK8 = XK8 *EXP( -1.56*(T0T-1.0) + 16.900*COEF) XK9 = XK9 *EXP( -8.22*(T0T-1.0) + 16.010*COEF) !C XK10= XK10*EXP(-74.38*(T0T-1.0) + 6.120*COEF) ! ISORR XK10= XK10*EXP(-74.7351*(T0T-1.0) + 6.025*COEF) ! (Mozurkewich, 1993) !C XK10= XK10*EXP(-75.11*(T0T-1.0) + 13.460*COEF) ! SEQUIL XK11= XK11*EXP( 0.79*(T0T-1.0) + 14.746*COEF) XK12= XK12*EXP( -2.87*(T0T-1.0) + 15.830*COEF) XK13= XK13*EXP( -5.19*(T0T-1.0) + 54.400*COEF) XK14= XK14*EXP( 24.55*(T0T-1.0) + 16.900*COEF) XKW = XKW *EXP(-22.52*(T0T-1.0) + 26.920*COEF) !CCC !C XK15= XK15 *EXP( .0*(T0T-1.0) + .0*COEF) !C XK16= XK16 *EXP( .0*(T0T-1.0) + .0*COEF) XK17= XK17 *EXP(-9.585*(T0T-1.0) + 45.81*COEF) XK18= XK18 *EXP(-8.423*(T0T-1.0) + 17.96*COEF) XK19= XK19 *EXP(-14.08*(T0T-1.0) + 19.39*COEF) XK20= XK20 *EXP(-6.902*(T0T-1.0) + 19.95*COEF) !C XK23= XK23 *EXP( .0*(T0T-1.0) + .0*COEF) !C XK24= XK24 *EXP( .0*(T0T-1.0) + .0*COEF) !C XK25= XK25 *EXP( .0*(T0T-1.0) + .0*COEF) !C XK26= XK26 *EXP(-3.0821*(T0T-1.0) + 31.8139*COEF) !C XK27= XK27 *EXP(-5.9908*(T0T-1.0) + 38.844*COEF) ENDIF XK2 = XK21*XK22 XK42 = XK4/XK41 XK32 = XK3/XK31 !C !C *** CALCULATE DELIQUESCENCE RELATIVE HUMIDITIES (UNICOMPONENT) ******** !C DRH2SO4 = ZERO DRNH42S4 = 0.7997D0 DRNH4HS4 = 0.4000D0 DRLC = 0.6900D0 DRNACL = 0.7528D0 DRNANO3 = 0.7379D0 DRNH4CL = 0.7710D0 DRNH4NO3 = 0.6183D0 DRNA2SO4 = 0.9300D0 DRNAHSO4 = 0.5200D0 DRCANO32 = 0.4906D0 DRCACL2 = 0.2830D0 DRK2SO4 = 0.9750D0 DRKHSO4 = 0.8600D0 DRKNO3 = 0.9248D0 DRKCL = 0.8426D0 DRMGSO4 = 0.8613D0 DRMGNO32 = 0.5400D0 DRMGCL2 = 0.3284D0 IF (INT(TEMP) .NE. 298) THEN T0 = 298.15D0 TCF = 1.0/TEMP - 1.0/T0 DRNACL = DRNACL *EXP( 25.*TCF) DRNANO3 = DRNANO3 *EXP(304.*TCF) DRNA2SO4 = DRNA2SO4*EXP( 80.*TCF) DRNH4NO3 = DRNH4NO3*EXP(852.*TCF) DRNH42S4 = DRNH42S4*EXP( 80.*TCF) DRNH4HS4 = DRNH4HS4*EXP(384.*TCF) DRLC = DRLC *EXP(186.*TCF) DRNH4CL = DRNH4Cl *EXP(239.*TCF) DRNAHSO4 = DRNAHSO4*EXP(-45.*TCF) !C DRCANO32 = DRCANO32*EXP(-430.5*TCF) DRCANO32 = DRCANO32*EXP(509.4*TCF) ! KELLY & WEXLER (2005) FOR CANO32.4H20 !C DRCACL2 = DRCACL2 *EXP(-1121.*TCF) DRCACL2 = DRCACL2 *EXP(551.1*TCF) ! KELLY & WEXLER (2005) FOR CACL2.6H20 DRK2SO4 = DRK2SO4 *EXP(35.6*TCF) !C DRKHSO4 = DRKHSO4 *EXP( 0.*TCF) !C DRKNO3 = DRKNO3 *EXP( 0.*TCF) DRKCL = DRKCL *EXP(159.*TCF) DRMGSO4 = DRMGSO4 *EXP(-714.45*TCF) DRMGNO32 = DRMGNO32*EXP(230.2*TCF) ! KELLY & WEXLER (2005) FOR MGNO32.6H20 !C DRMGCL2 = DRMGCL2 *EXP(-1860.*TCF) DRMGCL2 = DRMGCL2 *EXP(42.23*TCF) ! KELLY & WEXLER (2005) FOR MGCL2.6H20 !C ENDIF !C !C *** CALCULATE MUTUAL DELIQUESCENCE RELATIVE HUMIDITIES **************** !C DRMLCAB = 0.378D0 ! (NH4)3H(SO4)2 & NH4HSO4 DRMLCAS = 0.690D0 ! (NH4)3H(SO4)2 & (NH4)2SO4 DRMASAN = 0.600D0 ! (NH4)2SO4 & NH4NO3 DRMG1 = 0.460D0 ! (NH4)2SO4, NH4NO3, NA2SO4, NH4CL DRMG2 = 0.691D0 ! (NH4)2SO4, NA2SO4, NH4CL DRMG3 = 0.697D0 ! (NH4)2SO4, NA2SO4 DRMH1 = 0.240D0 ! NA2SO4, NANO3, NACL, NH4NO3, NH4CL DRMH2 = 0.596D0 ! NA2SO4, NANO3, NACL, NH4CL DRMI1 = 0.240D0 ! LC, NAHSO4, NH4HSO4, NA2SO4, (NH4)2SO4 DRMI2 = 0.363D0 ! LC, NAHSO4, NA2SO4, (NH4)2SO4 - NO DATA - DRMI3 = 0.610D0 ! LC, NA2SO4, (NH4)2SO4 DRMQ1 = 0.494D0 ! (NH4)2SO4, NH4NO3, NA2SO4 DRMR1 = 0.663D0 ! NA2SO4, NANO3, NACL DRMR2 = 0.735D0 ! NA2SO4, NACL DRMR3 = 0.673D0 ! NANO3, NACL DRMR4 = 0.694D0 ! NA2SO4, NACL, NH4CL DRMR5 = 0.731D0 ! NA2SO4, NH4CL DRMR6 = 0.596D0 ! NA2SO4, NANO3, NH4CL DRMR7 = 0.380D0 ! NA2SO4, NANO3, NACL, NH4NO3 DRMR8 = 0.380D0 ! NA2SO4, NACL, NH4NO3 DRMR9 = 0.494D0 ! NA2SO4, NH4NO3 DRMR10 = 0.476D0 ! NA2SO4, NANO3, NH4NO3 DRMR11 = 0.340D0 ! NA2SO4, NACL, NH4NO3, NH4CL DRMR12 = 0.460D0 ! NA2SO4, NH4NO3, NH4CL DRMR13 = 0.438D0 ! NA2SO4, NANO3, NH4NO3, NH4CL !C DRMO1 = 0.460D0 ! (NH4)2SO4, NH4NO3, NH4Cl, NA2SO4, K2SO4, MGSO4 DRMO2 = 0.691D0 ! (NH4)2SO4, NH4Cl, NA2SO4, K2SO4, MGSO4 DRMO3 = 0.697D0 ! (NH4)2SO4, NA2SO4, K2SO4, MGSO4 DRML1 = 0.240D0 ! K2SO4, MGSO4, KHSO4, NH4HSO4, NAHSO4, (NH4)2SO4, NA2SO4, LC DRML2 = 0.363D0 ! K2SO4, MGSO4, KHSO4, NAHSO4, (NH4)2SO4, NA2SO4, LC DRML3 = 0.610D0 ! K2SO4, MGSO4, KHSO4, (NH4)2SO4, NA2SO4, LC DRMM1 = 0.240D0 ! K2SO4, NA2SO4, MGSO4, NH4CL, NACL, NANO3, NH4NO3 DRMM2 = 0.596D0 ! K2SO4, NA2SO4, MGSO4, NH4CL, NACL, NANO3 DRMP1 = 0.200D0 ! CA(NO3)2, CACL2, K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, MGCL2, NANO3, NACL, NH4NO3, NH4CL DRMP2 = 0.240D0 ! CA(NO3)2, K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, MGCL2, NANO3, NACL, NH4NO3, NH4CL DRMP3 = 0.240D0 ! CA(NO3)2, K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, NANO3, NACL, NH4NO3, NH4CL DRMP4 = 0.240D0 ! K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, NANO3, NACL, NH4NO3, NH4CL DRMP5 = 0.240D0 ! K2SO4, KNO3, KCL, MGSO4, NANO3, NACL, NH4NO3, NH4CL !CC DRMV1 = 0.494D0 ! (NH4)2SO4, NH4NO3, NA2SO4, K2SO4, MGSO4 !CC !CC !C DRMO1 = 0.1D0 ! (NH4)2SO4, NH4NO3, NH4Cl, NA2SO4, K2SO4, MGSO4 !C DRMO2 = 0.1D0 ! (NH4)2SO4, NH4Cl, NA2SO4, K2SO4, MGSO4 !C DRMO3 = 0.1D0 ! (NH4)2SO4, NA2SO4, K2SO4, MGSO4 !C DRML1 = 0.1D0 ! K2SO4, MGSO4, KHSO4, NH4HSO4, NAHSO4, (NH4)2SO4, NA2SO4, LC !C DRML2 = 0.1D0 ! K2SO4, MGSO4, KHSO4, NAHSO4, (NH4)2SO4, NA2SO4, LC !C DRML3 = 0.1D0 ! K2SO4, MGSO4, KHSO4, (NH4)2SO4, NA2SO4, LC !C DRMM1 = 0.1D0 ! K2SO4, NA2SO4, MGSO4, NH4CL, NACL, NANO3, NH4NO3 !C DRMM2 = 0.1D0 ! K2SO4, NA2SO4, MGSO4, NH4CL, NACL, NANO3 !C DRMP1 = 0.1D0 ! CA(NO3)2, CACL2, K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, MGCL2, NANO3, NACL, NH4NO3, NH4CL !C DRMP2 = 0.1D0 ! CA(NO3)2, K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, MGCL2, NANO3, NACL, NH4NO3, NH4CL !C DRMP3 = 0.1D0 ! CA(NO3)2, K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, NANO3, NACL, NH4NO3, NH4CL !C DRMP4 = 0.1D0 ! K2SO4, KNO3, KCL, MGSO4, MG(NO3)2, NANO3, NACL, NH4NO3, NH4CL !C DRMP5 = 0.1D0 ! K2SO4, KNO3, KCL, MGSO4, NANO3, NACL, NH4NO3, NH4CL !CC !C DRMV1 = 0.1D0 ! (NH4)2SO4, NH4NO3, NA2SO4, K2SO4, MGSO4 !C !CCC IF (INT(TEMP) .NE. 298) THEN !CCC T0 = 298.15d0 !CCC TCF = 1.0/TEMP - 1.0/T0 !CCC DRMLCAB = DRMLCAB*EXP( 507.506*TCF) !CCC DRMLCAS = DRMLCAS*EXP( 133.865*TCF) !CCC DRMASAN = DRMASAN*EXP(1269.068*TCF) !CCC DRMG1 = DRMG1 *EXP( 572.207*TCF) !CCC DRMG2 = DRMG2 *EXP( 58.166*TCF) !CCC DRMG3 = DRMG3 *EXP( 22.253*TCF) !CCC DRMH1 = DRMH1 *EXP(2116.542*TCF) !CCC DRMH2 = DRMH2 *EXP( 650.549*TCF) !CCC DRMI1 = DRMI1 *EXP( 565.743*TCF) !CCC DRMI2 = DRMI2 *EXP( 91.745*TCF) !CCC DRMI3 = DRMI3 *EXP( 161.272*TCF) !CCC DRMQ1 = DRMQ1 *EXP(1616.621*TCF) !CCC DRMR1 = DRMR1 *EXP( 292.564*TCF) !CCC DRMR2 = DRMR2 *EXP( 14.587*TCF) !CCC DRMR3 = DRMR3 *EXP( 307.907*TCF) !CCC DRMR4 = DRMR4 *EXP( 97.605*TCF) !CCC DRMR5 = DRMR5 *EXP( 98.523*TCF) !CCC DRMR6 = DRMR6 *EXP( 465.500*TCF) !CCC DRMR7 = DRMR7 *EXP( 324.425*TCF) !CCC DRMR8 = DRMR8 *EXP(2660.184*TCF) !CCC DRMR9 = DRMR9 *EXP(1617.178*TCF) !CCC DRMR10 = DRMR10 *EXP(1745.226*TCF) !CCC DRMR11 = DRMR11 *EXP(3691.328*TCF) !CCC DRMR12 = DRMR12 *EXP(1836.842*TCF) !CCC DRMR13 = DRMR13 *EXP(1967.938*TCF) !CCC ENDIF !C !C *** LIQUID PHASE ****************************************************** !C CHNO3 = ZERO CHCL = ZERO CH2SO4 = ZERO COH = ZERO WATER = TINY !C DO 20 I=1,NPAIR MOLALR(I)=ZERO GAMA(I) =0.1 GAMIN(I) =GREAT GAMOU(I) =GREAT M0(I) =1d5 20 CONTINUE !C DO 30 I=1,NPAIR GAMA(I) = 0.1d0 30 CONTINUE !C DO 40 I=1,NIONS MOLAL(I)=ZERO 40 CONTINUE COH = ZERO !C DO 50 I=1,NGASAQ GASAQ(I)=ZERO 50 CONTINUE !C !C *** SOLID PHASE ******************************************************* !C CNH42S4= ZERO CNH4HS4= ZERO CNACL = ZERO CNA2SO4= ZERO CNANO3 = ZERO CNH4NO3= ZERO CNH4CL = ZERO CNAHSO4= ZERO CLC = ZERO CCASO4 = ZERO CCANO32= ZERO CCACL2 = ZERO CK2SO4 = ZERO CKHSO4 = ZERO CKNO3 = ZERO CKCL = ZERO CMGSO4 = ZERO CMGNO32= ZERO CMGCL2 = ZERO !C !C *** GAS PHASE ********************************************************* !C GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO !C !C *** CALCULATE ZSR PARAMETERS ****************************************** !C IRH = MIN (INT(RH*NZSR+0.5),NZSR) ! Position in ZSR arrays IRH = MAX (IRH, 1) !C M0(01) = AWSC(IRH) ! NACl !C IF (M0(01) .LT. 100.0) THEN !C IC = M0(01) !C CALL KMTAB(IC,298.0, GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(01) = M0(01)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(02) = AWSS(IRH) ! (NA)2SO4 !C IF (M0(02) .LT. 100.0) THEN !C IC = 3.0*M0(02) !C CALL KMTAB(IC,298.0, XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(02) = M0(02)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(03) = AWSN(IRH) ! NANO3 !C IF (M0(03) .LT. 100.0) THEN !C IC = M0(03) !C CALL KMTAB(IC,298.0, XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(03) = M0(03)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(04) = AWAS(IRH) ! (NH4)2SO4 !C IF (M0(04) .LT. 100.0) THEN !C IC = 3.0*M0(04) !C CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(04) = M0(04)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(05) = AWAN(IRH) ! NH4NO3 !C IF (M0(05) .LT. 100.0) THEN !C IC = M0(05) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(05) = M0(05)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(06) = AWAC(IRH) ! NH4CL !C IF (M0(06) .LT. 100.0) THEN !C IC = M0(06) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(06) = M0(06)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(07) = AWSA(IRH) ! 2H-SO4 !C IF (M0(07) .LT. 100.0) THEN !C IC = 3.0*M0(07) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(07) = M0(07)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(08) = AWSA(IRH) ! H-HSO4 !CCC IF (M0(08) .LT. 100.0) THEN ! These are redundant, because M0(8) is not used !CCC IC = M0(08) !CCC CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX,XX) !CCCCCC CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX,XX) !CCC M0(08) = M0(08)*EXP(LN10*(GI0-GII)) !CCC ENDIF !C M0(09) = AWAB(IRH) ! NH4HSO4 !C IF (M0(09) .LT. 100.0) THEN !C IC = M0(09) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,GI0,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,GII,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(09) = M0(09)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(12) = AWSB(IRH) ! NAHSO4 !C IF (M0(12) .LT. 100.0) THEN !C IC = M0(12) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GI0, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,GII, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(12) = M0(12)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(13) = AWLC(IRH) ! (NH4)3H(SO4)2 !C IF (M0(13) .LT. 100.0) THEN !C IC = 4.0*M0(13) !C CALL KMTAB(IC,298.0, XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C G130 = 0.2*(3.0*GI0+2.0*GII) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,GI0,XX,XX,XX,XX,GII,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,XX) !C G13I = 0.2*(3.0*GI0+2.0*GII) !C M0(13) = M0(13)*EXP(LN10*SNGL(G130-G13I)) !C ENDIF !C M0(15) = AWCN(IRH) ! CA(NO3)2 !C IF (M0(15) .LT. 100.0) THEN !C IC = M0(15) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & GI0,XX,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & GII,XX,XX,XX,XX,XX,XX,XX,XX) !C M0(15) = M0(15)*EXP(LN10*(GI0-GII)) !C ENDIF !CC M0(16) = AWCC(IRH) ! CACl2 !C IF (M0(16) .LT. 100.0) THEN !C IC = M0(16) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,GI0,XX,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,GII,XX,XX,XX,XX,XX,XX,XX) !C M0(16) = M0(16)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(17) = AWPS(IRH) ! K2SO4 !C IF (M0(17) .LT. 100.0) THEN !C IC = M0(17) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,GI0,XX,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,GII,XX,XX,XX,XX,XX,XX) !C M0(17) = M0(17)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(18) = AWPB(IRH) ! KHSO4 !C IF (M0(18) .LT. 100.0) THEN !C IC = M0(18) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,GI0,XX,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,GII,XX,XX,XX,XX,XX) !C M0(18) = M0(18)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(19) = AWPN(IRH) ! KNO3 !C IF (M0(19) .LT. 100.0) THEN !C IC = M0(19) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,GI0,XX,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,GII,XX,XX,XX,XX) !C M0(19) = M0(19)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(20) = AWPC(IRH) ! KCl !C IF (M0(20) .LT. 100.0) THEN !C IC = M0(20) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,GI0,XX,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,GII,XX,XX,XX) !C M0(20) = M0(20)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(21) = AWMS(IRH) ! MGSO4 !C IF (M0(21) .LT. 100.0) THEN !C IC = M0(21) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,GI0,XX,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,GII,XX,XX) !C M0(21) = M0(21)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(22) = AWMN(IRH) ! MG(NO3)2 !C IF (M0(22) .LT. 100.0) THEN !C IC = M0(22) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,GI0,XX) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,GII,XX) !C M0(22) = M0(22)*EXP(LN10*(GI0-GII)) !C ENDIF !C M0(23) = AWMC(IRH) ! MGCL2 !C IF (M0(23) .LT. 100.0) THEN !C IC = M0(23) !C CALL KMTAB(IC,298.0, XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,GI0) !C CALL KMTAB(IC,SNGL(TEMP),XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX,XX, !C & XX,XX,XX,XX,XX,XX,XX,XX,GII) !C M0(23) = M0(23)*EXP(LN10*(GI0-GII)) !C ENDIF !C !C *** OTHER INITIALIZATIONS ********************************************* !C ICLACT = 0 CALAOU = .TRUE. CALAIN = .TRUE. FRST = .TRUE. !liqy ! SCASE = '??' SCASE = 'xx' !liqy-20140513 SULRATW = 2.D0 SO4RAT = 2.D0 CRNARAT = 2.D0 CRRAT = 2.D0 NOFER = 0 STKOFL =.FALSE. DO 60 I=1,NERRMX ERRSTK(I) =-999 ERRMSG(I) = 'MESSAGE N/A' 60 CONTINUE !C !C *** END OF SUBROUTINE INIT4 ******************************************* !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE ADJUST !C *** ADJUSTS FOR MASS BALANCE BETWEEN VOLATILE SPECIES AND SULFATE !C FIRST CALCULATE THE EXCESS OF EACH PRECURSOR, AND IF IT EXISTS, THEN !C ADJUST SEQUENTIALY AEROSOL PHASE SPECIES WHICH CONTAIN THE EXCESS !C PRECURSOR. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE ADJUST2p1 (WI) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION WI(*) !C !C *** FOR AMMONIUM ***************************************************** !C IF (IPROB.EQ.0) THEN ! Calculate excess (solution - input) EXNH4 = GNH3 + MOLAL(3) + CNH4CL + CNH4NO3 + CNH4HS4 & + 2D0*CNH42S4 + 3D0*CLC & -WI(3) ELSE EXNH4 = MOLAL(3) + CNH4CL + CNH4NO3 + CNH4HS4 + 2D0*CNH42S4 & + 3D0*CLC & -WI(3) ENDIF EXNH4 = MAX(EXNH4,ZERO) IF (EXNH4.LT.TINY) GOTO 20 ! No excess NH4, go to next precursor !C IF (MOLAL(3).GT.EXNH4) THEN ! Adjust aqueous phase NH4 MOLAL(3) = MOLAL(3) - EXNH4 GOTO 20 ELSE EXNH4 = EXNH4 - MOLAL(3) MOLAL(3) = ZERO ENDIF !C IF (CNH4CL.GT.EXNH4) THEN ! Adjust NH4Cl(s) CNH4CL = CNH4CL - EXNH4 ! more solid than excess GHCL = GHCL + EXNH4 ! evaporate Cl to gas phase GOTO 20 ELSE ! less solid than excess GHCL = GHCL + CNH4CL ! evaporate into gas phase EXNH4 = EXNH4 - CNH4CL ! reduce excess CNH4CL = ZERO ! zero salt concentration ENDIF !C IF (CNH4NO3.GT.EXNH4) THEN ! Adjust NH4NO3(s) CNH4NO3 = CNH4NO3- EXNH4 ! more solid than excess GHNO3 = GHNO3 + EXNH4 ! evaporate NO3 to gas phase GOTO 20 ELSE ! less solid than excess GHNO3 = GHNO3 + CNH4NO3! evaporate into gas phase EXNH4 = EXNH4 - CNH4NO3! reduce excess CNH4NO3 = ZERO ! zero salt concentration ENDIF !C IF (CLC.GT.3d0*EXNH4) THEN ! Adjust (NH4)3H(SO4)2(s) CLC = CLC - EXNH4/3d0 ! more solid than excess GOTO 20 ELSE ! less solid than excess EXNH4 = EXNH4 - 3d0*CLC ! reduce excess CLC = ZERO ! zero salt concentration ENDIF !C IF (CNH4HS4.GT.EXNH4) THEN ! Adjust NH4HSO4(s) CNH4HS4 = CNH4HS4- EXNH4 ! more solid than excess GOTO 20 ELSE ! less solid than excess EXNH4 = EXNH4 - CNH4HS4! reduce excess CNH4HS4 = ZERO ! zero salt concentration ENDIF !C IF (CNH42S4.GT.EXNH4) THEN ! Adjust (NH4)2SO4(s) CNH42S4 = CNH42S4- EXNH4 ! more solid than excess GOTO 20 ELSE ! less solid than excess EXNH4 = EXNH4 - CNH42S4! reduce excess CNH42S4 = ZERO ! zero salt concentration ENDIF !C !C *** FOR NITRATE ****************************************************** !C 20 IF (IPROB.EQ.0) THEN ! Calculate excess (solution - input) EXNO3 = GHNO3 + MOLAL(7) + CNH4NO3 & -WI(4) ELSE EXNO3 = MOLAL(7) + CNH4NO3 & -WI(4) ENDIF EXNO3 = MAX(EXNO3,ZERO) IF (EXNO3.LT.TINY) GOTO 30 ! No excess NO3, go to next precursor !C IF (MOLAL(7).GT.EXNO3) THEN ! Adjust aqueous phase NO3 MOLAL(7) = MOLAL(7) - EXNO3 GOTO 30 ELSE EXNO3 = EXNO3 - MOLAL(7) MOLAL(7) = ZERO ENDIF !C IF (CNH4NO3.GT.EXNO3) THEN ! Adjust NH4NO3(s) CNH4NO3 = CNH4NO3- EXNO3 ! more solid than excess GNH3 = GNH3 + EXNO3 ! evaporate NO3 to gas phase GOTO 30 ELSE ! less solid than excess GNH3 = GNH3 + CNH4NO3! evaporate into gas phase EXNO3 = EXNO3 - CNH4NO3! reduce excess CNH4NO3 = ZERO ! zero salt concentration ENDIF !C !C *** FOR CHLORIDE ***************************************************** !C 30 IF (IPROB.EQ.0) THEN ! Calculate excess (solution - input) EXCl = GHCL + MOLAL(4) + CNH4CL & -WI(5) ELSE EXCl = MOLAL(4) + CNH4CL & -WI(5) ENDIF EXCl = MAX(EXCl,ZERO) IF (EXCl.LT.TINY) GOTO 40 ! No excess Cl, go to next precursor !C IF (MOLAL(4).GT.EXCL) THEN ! Adjust aqueous phase Cl MOLAL(4) = MOLAL(4) - EXCL GOTO 40 ELSE EXCL = EXCL - MOLAL(4) MOLAL(4) = ZERO ENDIF !C IF (CNH4CL.GT.EXCL) THEN ! Adjust NH4Cl(s) CNH4CL = CNH4CL - EXCL ! more solid than excess GHCL = GHCL + EXCL ! evaporate Cl to gas phase GOTO 40 ELSE ! less solid than excess GHCL = GHCL + CNH4CL ! evaporate into gas phase EXCL = EXCL - CNH4CL ! reduce excess CNH4CL = ZERO ! zero salt concentration ENDIF !C !C *** FOR SULFATE ****************************************************** !C 40 EXS4 = MOLAL(5) + MOLAL(6) + 2.d0*CLC + CNH42S4 + CNH4HS4 + & CNA2SO4 + CNAHSO4 - WI(2) EXS4 = MAX(EXS4,ZERO) ! Calculate excess (solution - input) IF (EXS4.LT.TINY) GOTO 50 ! No excess SO4, return !C IF (MOLAL(6).GT.EXS4) THEN ! Adjust aqueous phase HSO4 MOLAL(6) = MOLAL(6) - EXS4 GOTO 50 ELSE EXS4 = EXS4 - MOLAL(6) MOLAL(6) = ZERO ENDIF !C IF (MOLAL(5).GT.EXS4) THEN ! Adjust aqueous phase SO4 MOLAL(5) = MOLAL(5) - EXS4 GOTO 50 ELSE EXS4 = EXS4 - MOLAL(5) MOLAL(5) = ZERO ENDIF !C IF (CLC.GT.2d0*EXS4) THEN ! Adjust (NH4)3H(SO4)2(s) CLC = CLC - EXS4/2d0 ! more solid than excess GNH3 = GNH3 +1.5d0*EXS4! evaporate NH3 to gas phase GOTO 50 ELSE ! less solid than excess GNH3 = GNH3 + 1.5d0*CLC! evaporate NH3 to gas phase EXS4 = EXS4 - 2d0*CLC ! reduce excess CLC = ZERO ! zero salt concentration ENDIF !C IF (CNH4HS4.GT.EXS4) THEN ! Adjust NH4HSO4(s) CNH4HS4 = CNH4HS4 - EXS4 ! more solid than excess GNH3 = GNH3 + EXS4 ! evaporate NH3 to gas phase GOTO 50 ELSE ! less solid than excess GNH3 = GNH3 + CNH4HS4 ! evaporate NH3 to gas phase EXS4 = EXS4 - CNH4HS4 ! reduce excess CNH4HS4 = ZERO ! zero salt concentration ENDIF !C IF (CNH42S4.GT.EXS4) THEN ! Adjust (NH4)2SO4(s) CNH42S4 = CNH42S4- EXS4 ! more solid than excess GNH3 = GNH3 + 2.d0*EXS4! evaporate NH3 to gas phase GOTO 50 ELSE ! less solid than excess GNH3 = GNH3+2.d0*CNH42S4 ! evaporate NH3 to gas phase EXS4 = EXS4 - CNH42S4 ! reduce excess CNH42S4 = ZERO ! zero salt concentration ENDIF !C !C *** RETURN ********************************************************** !C 50 RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** FUNCTION GETASR !C *** CALCULATES THE LIMITING NH4+/SO4 RATIO OF A SULFATE POOR SYSTEM !C (i.e. SULFATE RATIO = 2.0) FOR GIVEN SO4 LEVEL AND RH !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C DOUBLE PRECISION FUNCTION GETASR2p1 (SO4I, RHI) PARAMETER (NSO4S=14, NRHS=20, NASRD=NSO4S*NRHS) COMMON /ASRC2p1/ ASRAT(NASRD), ASSO4(NSO4S) DOUBLE PRECISION SO4I, RHI !CCC !CCC *** SOLVE USING FULL COMPUTATIONS, NOT LOOK-UP TABLES ************** !CCC !CCC W(2) = WAER(2) !CCC W(3) = WAER(2)*2.0001D0 !CCC CALL CALCA2 !CCC SULRATW = MOLAL(3)/WAER(2) !CCC CALL INIT1 (WI, RHI, TEMPI) ! Re-initialize COMMON BLOCK !C !C *** CALCULATE INDICES ************************************************ !C RAT = SO4I/1.E-9 A1 = INT(ALOG10(RAT)) ! Magnitude of RAT IA1 = INT(RAT/2.5/10.0**A1) !C INDS = 4.0*A1 + MIN(IA1,4) INDS = MIN(MAX(0, INDS), NSO4S-1) + 1 ! SO4 component of IPOS !C INDR = INT(99.0-RHI*100.0) + 1 INDR = MIN(MAX(1, INDR), NRHS) ! RH component of IPOS !C !C *** GET VALUE AND RETURN ********************************************* !C INDSL = INDS INDSH = MIN(INDSL+1, NSO4S) IPOSL = (INDSL-1)*NRHS + INDR ! Low position in array IPOSH = (INDSH-1)*NRHS + INDR ! High position in array !C WF = (SO4I-ASSO4(INDSL))/(ASSO4(INDSH)-ASSO4(INDSL) + 1e-7) WF = MIN(MAX(WF, 0.0), 1.0) !C GETASR2p1 = WF*ASRAT(IPOSH) + (1.0-WF)*ASRAT(IPOSL) !C !C *** END OF FUNCTION GETASR ******************************************* !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** BLOCK DATA AERSR !C *** CONTAINS DATA FOR AEROSOL SULFATE RATIO ARRAY NEEDED IN FUNCTION !C GETASR !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C BLOCK DATA AERSR2p1 PARAMETER (NSO4S=14, NRHS=20, NASRD=NSO4S*NRHS) COMMON /ASRC2p1/ ASRAT(NASRD), ASSO4(NSO4S) !C DATA ASSO4/1.0E-9, 2.5E-9, 5.0E-9, 7.5E-9, 1.0E-8, & 2.5E-8, 5.0E-8, 7.5E-8, 1.0E-7, 2.5E-7, & 5.0E-7, 7.5E-7, 1.0E-6, 5.0E-6/ !C DATA (ASRAT(I), I=1,100)/& 1.020464, 0.9998130, 0.9960167, 0.9984423, 1.004004,& 1.010885, 1.018356, 1.026726, 1.034268, 1.043846,& 1.052933, 1.062230, 1.062213, 1.080050, 1.088350,& 1.096603, 1.104289, 1.111745, 1.094662, 1.121594,& 1.268909, 1.242444, 1.233815, 1.232088, 1.234020,& 1.238068, 1.243455, 1.250636, 1.258734, 1.267543,& 1.276948, 1.286642, 1.293337, 1.305592, 1.314726,& 1.323463, 1.333258, 1.343604, 1.344793, 1.355571,& 1.431463, 1.405204, 1.395791, 1.393190, 1.394403,& 1.398107, 1.403811, 1.411744, 1.420560, 1.429990,& 1.439742, 1.449507, 1.458986, 1.468403, 1.477394,& 1.487373, 1.495385, 1.503854, 1.512281, 1.520394,& 1.514464, 1.489699, 1.480686, 1.478187, 1.479446,& 1.483310, 1.489316, 1.497517, 1.506501, 1.515816,& 1.524724, 1.533950, 1.542758, 1.551730, 1.559587,& 1.568343, 1.575610, 1.583140, 1.590440, 1.596481,& 1.567743, 1.544426, 1.535928, 1.533645, 1.535016,& 1.539003, 1.545124, 1.553283, 1.561886, 1.570530,& 1.579234, 1.587813, 1.595956, 1.603901, 1.611349,& 1.618833, 1.625819, 1.632543, 1.639032, 1.645276/ DATA (ASRAT(I), I=101,200)/& 1.707390, 1.689553, 1.683198, 1.681810, 1.683490,& 1.687477, 1.693148, 1.700084, 1.706917, 1.713507,& 1.719952, 1.726190, 1.731985, 1.737544, 1.742673,& 1.747756, 1.752431, 1.756890, 1.761141, 1.765190,& 1.785657, 1.771851, 1.767063, 1.766229, 1.767901,& 1.771455, 1.776223, 1.781769, 1.787065, 1.792081,& 1.796922, 1.801561, 1.805832, 1.809896, 1.813622,& 1.817292, 1.820651, 1.823841, 1.826871, 1.829745,& 1.822215, 1.810497, 1.806496, 1.805898, 1.807480,& 1.810684, 1.814860, 1.819613, 1.824093, 1.828306,& 1.832352, 1.836209, 1.839748, 1.843105, 1.846175,& 1.849192, 1.851948, 1.854574, 1.857038, 1.859387,& 1.844588, 1.834208, 1.830701, 1.830233, 1.831727,& 1.834665, 1.838429, 1.842658, 1.846615, 1.850321,& 1.853869, 1.857243, 1.860332, 1.863257, 1.865928,& 1.868550, 1.870942, 1.873208, 1.875355, 1.877389,& 1.899556, 1.892637, 1.890367, 1.890165, 1.891317,& 1.893436, 1.896036, 1.898872, 1.901485, 1.903908,& 1.906212, 1.908391, 1.910375, 1.912248, 1.913952,& 1.915621, 1.917140, 1.918576, 1.919934, 1.921220/ DATA (ASRAT(I), I=201,280)/& 1.928264, 1.923245, 1.921625, 1.921523, 1.922421,& 1.924016, 1.925931, 1.927991, 1.929875, 1.931614,& 1.933262, 1.934816, 1.936229, 1.937560, 1.938769,& 1.939951, 1.941026, 1.942042, 1.943003, 1.943911,& 1.941205, 1.937060, 1.935734, 1.935666, 1.936430,& 1.937769, 1.939359, 1.941061, 1.942612, 1.944041,& 1.945393, 1.946666, 1.947823, 1.948911, 1.949900,& 1.950866, 1.951744, 1.952574, 1.953358, 1.954099,& 1.948985, 1.945372, 1.944221, 1.944171, 1.944850,& 1.946027, 1.947419, 1.948902, 1.950251, 1.951494,& 1.952668, 1.953773, 1.954776, 1.955719, 1.956576,& 1.957413, 1.958174, 1.958892, 1.959571, 1.960213,& 1.977193, 1.975540, 1.975023, 1.975015, 1.975346,& 1.975903, 1.976547, 1.977225, 1.977838, 1.978401,& 1.978930, 1.979428, 1.979879, 1.980302, 1.980686,& 1.981060, 1.981401, 1.981722, 1.982025, 1.982312/ !C !C *** END OF BLOCK DATA AERSR ****************************************** !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCHA !C *** CALCULATES CHLORIDES SPECIATION !C !C HYDROCHLORIC ACID IN THE LIQUID PHASE IS ASSUMED A MINOR SPECIES, !C AND DOES NOT SIGNIFICANTLY PERTURB THE HSO4-SO4 EQUILIBRIUM. THE !C HYDROCHLORIC ACID DISSOLVED IS CALCULATED FROM THE !C HCL(G) <-> (H+) + (CL-) !C EQUILIBRIUM, USING THE (H+) FROM THE SULFATES. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCHA2p1 INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION KAPA !CC CHARACTER ERRINF*40 !C !C *** CALCULATE HCL DISSOLUTION ***************************************** !C X = W(5) DELT = 0.0d0 IF (WATER.GT.TINY) THEN KAPA = MOLAL(1) ALFA = XK3*R*TEMP*(WATER/GAMA(11))**2.0 DIAK = SQRT( (KAPA+ALFA)**2.0 + 4.0*ALFA*X) DELT = 0.5*(-(KAPA+ALFA) + DIAK) !CC IF (DELT/KAPA.GT.0.1d0) THEN !CC WRITE (ERRINF,'(1PE10.3)') DELT/KAPA*100.0 !CC CALL PUSHERR (0033, ERRINF) !CC ENDIF ENDIF !C !C *** CALCULATE HCL SPECIATION IN THE GAS PHASE ************************* !C GHCL = MAX(X-DELT, 0.0d0) ! GAS HCL !C !C *** CALCULATE HCL SPECIATION IN THE LIQUID PHASE ********************** !C MOLAL(4) = DELT ! CL- MOLAL(1) = MOLAL(1) + DELT ! H+ !C RETURN !C !C *** END OF SUBROUTINE CALCHA ****************************************** !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCHAP !C *** CALCULATES CHLORIDES SPECIATION !C !C HYDROCHLORIC ACID IN THE LIQUID PHASE IS ASSUMED A MINOR SPECIES, !C THAT DOES NOT SIGNIFICANTLY PERTURB THE HSO4-SO4 EQUILIBRIUM. !C THE HYDROCHLORIC ACID DISSOLVED IS CALCULATED FROM THE !C HCL(G) -> HCL(AQ) AND HCL(AQ) -> (H+) + (CL-) !C EQUILIBRIA, USING (H+) FROM THE SULFATES. !C !C THIS IS THE VERSION USED BY THE INVERSE PROBLEM SOVER !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCHAP2p1 INCLUDE 'module_isrpia_inc.F' !C !C *** IS THERE A LIQUID PHASE? ****************************************** !C IF (WATER.LE.TINY) RETURN !C !C *** CALCULATE HCL SPECIATION IN THE GAS PHASE ************************* !C CALL CALCCLAQ2p1 (MOLAL(4), MOLAL(1), DELT) ALFA = XK3*R*TEMP*(WATER/GAMA(11))**2.0 GASAQ(3) = DELT MOLAL(1) = MOLAL(1) - DELT MOLAL(4) = MOLAL(4) - DELT GHCL = MOLAL(1)*MOLAL(4)/ALFA !C RETURN !C !C *** END OF SUBROUTINE CALCHAP ***************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNA !C *** CALCULATES NITRATES SPECIATION !C !C NITRIC ACID IN THE LIQUID PHASE IS ASSUMED A MINOR SPECIES, THAT !C DOES NOT SIGNIFICANTLY PERTURB THE HSO4-SO4 EQUILIBRIUM. THE NITRIC !C ACID DISSOLVED IS CALCULATED FROM THE HNO3(G) -> (H+) + (NO3-) !C EQUILIBRIUM, USING THE (H+) FROM THE SULFATES. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNA2p1 INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION KAPA !CC CHARACTER ERRINF*40 !C !C *** CALCULATE HNO3 DISSOLUTION **************************************** !C X = W(4) DELT = 0.0d0 IF (WATER.GT.TINY) THEN KAPA = MOLAL(1) ALFA = XK4*R*TEMP*(WATER/GAMA(10))**2.0 DIAK = SQRT( (KAPA+ALFA)**2.0 + 4.0*ALFA*X) DELT = 0.5*(-(KAPA+ALFA) + DIAK) !CC IF (DELT/KAPA.GT.0.1d0) THEN !CC WRITE (ERRINF,'(1PE10.3)') DELT/KAPA*100.0 !CC CALL PUSHERR (0019, ERRINF) ! WARNING ERROR: NO SOLUTION !CC ENDIF ENDIF !C !C *** CALCULATE HNO3 SPECIATION IN THE GAS PHASE ************************ !C GHNO3 = MAX(X-DELT, 0.0d0) ! GAS HNO3 !C !C *** CALCULATE HNO3 SPECIATION IN THE LIQUID PHASE ********************* !C MOLAL(7) = DELT ! NO3- MOLAL(1) = MOLAL(1) + DELT ! H+ !C RETURN !C !C *** END OF SUBROUTINE CALCNA ****************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNAP !C *** CALCULATES NITRATES SPECIATION !C !C NITRIC ACID IN THE LIQUID PHASE IS ASSUMED A MINOR SPECIES, THAT !C DOES NOT SIGNIFICANTLY PERTURB THE HSO4-SO4 EQUILIBRIUM. THE NITRIC !C ACID DISSOLVED IS CALCULATED FROM THE HNO3(G) -> HNO3(AQ) AND !C HNO3(AQ) -> (H+) + (CL-) EQUILIBRIA, USING (H+) FROM THE SULFATES. !C !C THIS IS THE VERSION USED BY THE INVERSE PROBLEM SOVER !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNAP2p1 INCLUDE 'module_isrpia_inc.F' !C !C *** IS THERE A LIQUID PHASE? ****************************************** !C IF (WATER.LE.TINY) RETURN !C !C *** CALCULATE HNO3 SPECIATION IN THE GAS PHASE ************************ !C CALL CALCNIAQ2p1 (MOLAL(7), MOLAL(1), DELT) ALFA = XK4*R*TEMP*(WATER/GAMA(10))**2.0 GASAQ(3) = DELT MOLAL(1) = MOLAL(1) - DELT MOLAL(7) = MOLAL(7) - DELT GHNO3 = MOLAL(1)*MOLAL(7)/ALFA write (*,*) ALFA, MOLAL(1), MOLAL(7), GHNO3, DELT !C RETURN !C !C *** END OF SUBROUTINE CALCNAP ***************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNH3 !C *** CALCULATES AMMONIA IN GAS PHASE !C !C AMMONIA IN THE GAS PHASE IS ASSUMED A MINOR SPECIES, THAT !C DOES NOT SIGNIFICANTLY PERTURB THE AEROSOL EQUILIBRIUM. !C AMMONIA GAS IS CALCULATED FROM THE NH3(g) + (H+)(l) <==> (NH4+)(l) !C EQUILIBRIUM, USING (H+), (NH4+) FROM THE AEROSOL SOLUTION. !C !C THIS IS THE VERSION USED BY THE DIRECT PROBLEM !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNH32p1 INCLUDE 'module_isrpia_inc.F' !C !C *** IS THERE A LIQUID PHASE? ****************************************** !C IF (WATER.LE.TINY) RETURN !C !C *** CALCULATE NH3 SUBLIMATION ***************************************** !C A1 = (XK2/XKW)*R*TEMP*(GAMA(10)/GAMA(5))**2.0 CHI1 = MOLAL(3) CHI2 = MOLAL(1) !C BB =(CHI2 + ONE/A1) ! a=1; b!=1; c!=1 CC =-CHI1/A1 DIAK = SQRT(BB*BB - 4.D0*CC) ! Always > 0 PSI = 0.5*(-BB + DIAK) ! One positive root PSI = MAX(TINY, MIN(PSI,CHI1))! Constrict in acceptible range !C !C *** CALCULATE NH3 SPECIATION IN THE GAS PHASE ************************* !C GNH3 = PSI ! GAS HNO3 !C !C *** CALCULATE NH3 AFFECT IN THE LIQUID PHASE ************************** !C MOLAL(3) = CHI1 - PSI ! NH4+ MOLAL(1) = CHI2 + PSI ! H+ !C RETURN !C !C *** END OF SUBROUTINE CALCNH3 ***************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNH3P !C *** CALCULATES AMMONIA IN GAS PHASE !C !C AMMONIA GAS IS CALCULATED FROM THE NH3(g) + (H+)(l) <==> (NH4+)(l) !C EQUILIBRIUM, USING (H+), (NH4+) FROM THE AEROSOL SOLUTION. !C !C THIS IS THE VERSION USED BY THE INVERSE PROBLEM SOLVER !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNH3P2p1 INCLUDE 'module_isrpia_inc.F' !C !C *** IS THERE A LIQUID PHASE? ****************************************** !C IF (WATER.LE.TINY) RETURN !C !C *** CALCULATE NH3 GAS PHASE CONCENTRATION ***************************** !C A1 = (XK2/XKW)*R*TEMP*(GAMA(10)/GAMA(5))**2.0 GNH3 = MOLAL(3)/MOLAL(1)/A1 !C RETURN !C !C *** END OF SUBROUTINE CALCNH3P **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNHA !C !C THIS SUBROUTINE CALCULATES THE DISSOLUTION OF HCL, HNO3 AT !C THE PRESENCE OF (H,SO4). HCL, HNO3 ARE CONSIDERED MINOR SPECIES, !C THAT DO NOT SIGNIFICANTLY AFFECT THE EQUILIBRIUM POINT. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNHA2p1 INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION M1, M2, M3 CHARACTER ERRINF*40 !C !C *** SPECIAL CASE; WATER=ZERO ****************************************** !C IF (WATER.LE.TINY) THEN GOTO 55 !C !C *** SPECIAL CASE; HCL=HNO3=ZERO *************************************** !C ELSEIF (W(5).LE.TINY .AND. W(4).LE.TINY) THEN GOTO 60 !C !C *** SPECIAL CASE; HCL=ZERO ******************************************** !C ELSE IF (W(5).LE.TINY) THEN CALL CALCNA2p1 ! CALL HNO3 DISSOLUTION ROUTINE GOTO 60 !C !C *** SPECIAL CASE; HNO3=ZERO ******************************************* !C ELSE IF (W(4).LE.TINY) THEN CALL CALCHA2p1 ! CALL HCL DISSOLUTION ROUTINE GOTO 60 ENDIF !C !C *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !C A3 = XK4*R*TEMP*(WATER/GAMA(10))**2.0 ! HNO3 A4 = XK3*R*TEMP*(WATER/GAMA(11))**2.0 ! HCL !C !C *** CALCULATE CUBIC EQUATION COEFFICIENTS ***************************** !C DELCL = ZERO DELNO = ZERO !C OMEGA = MOLAL(1) ! H+ CHI3 = W(4) ! HNO3 CHI4 = W(5) ! HCL !C C1 = A3*CHI3 C2 = A4*CHI4 C3 = A3 - A4 !C M1 = (C1 + C2 + (OMEGA+A4)*C3)/C3 M2 = ((OMEGA+A4)*C2 - A4*C3*CHI4)/C3 M3 =-A4*C2*CHI4/C3 !C !C *** CALCULATE ROOTS *************************************************** !C CALL POLY32p1 (M1, M2, M3, DELCL, ISLV) ! HCL DISSOLUTION IF (ISLV.NE.0) THEN DELCL = TINY ! TINY AMOUNTS OF HCL ASSUMED WHEN NO ROOT WRITE (ERRINF,'(1PE7.1)') TINY CALL PUSHERR2p1 (0022, ERRINF) ! WARNING ERROR: NO SOLUTION ENDIF DELCL = MIN(DELCL, CHI4) !C DELNO = C1*DELCL/(C2 + C3*DELCL) DELNO = MIN(DELNO, CHI3) !C IF (DELCL.LT.ZERO .OR. DELNO.LT.ZERO .OR. & DELCL.GT.CHI4 .OR. DELNO.GT.CHI3 ) THEN DELCL = TINY ! TINY AMOUNTS OF HCL ASSUMED WHEN NO ROOT DELNO = TINY WRITE (ERRINF,'(1PE7.1)') TINY CALL PUSHERR2p1 (0022, ERRINF) ! WARNING ERROR: NO SOLUTION ENDIF !CCC !CCC *** COMPARE DELTA TO TOTAL H+ ; ESTIMATE EFFECT TO HSO4 *************** !CCC !CC IF ((DELCL+DELNO)/MOLAL(1).GT.0.1d0) THEN !CC WRITE (ERRINF,'(1PE10.3)') (DELCL+DELNO)/MOLAL(1)*100.0 !CC CALL PUSHERR (0021, ERRINF) !CC ENDIF !C !C *** EFFECT ON LIQUID PHASE ******************************************** !C 50 MOLAL(1) = MOLAL(1) + (DELNO+DELCL) ! H+ CHANGE MOLAL(4) = MOLAL(4) + DELCL ! CL- CHANGE MOLAL(7) = MOLAL(7) + DELNO ! NO3- CHANGE !C !C *** EFFECT ON GAS PHASE *********************************************** !C 55 GHCL = MAX(W(5) - MOLAL(4), TINY) GHNO3 = MAX(W(4) - MOLAL(7), TINY) !C 60 RETURN !C !C *** END OF SUBROUTINE CALCNHA ***************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNHP !C !C THIS SUBROUTINE CALCULATES THE GAS PHASE NITRIC AND HYDROCHLORIC !C ACID. CONCENTRATIONS ARE CALCULATED FROM THE DISSOLUTION !C EQUILIBRIA, USING (H+), (Cl-), (NO3-) IN THE AEROSOL PHASE. !C !C THIS IS THE VERSION USED BY THE INVERSE PROBLEM SOLVER !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNHP2p1 INCLUDE 'module_isrpia_inc.F' !C !C *** IS THERE A LIQUID PHASE? ****************************************** !C IF (WATER.LE.TINY) RETURN !C !C *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !C A3 = XK3*R*TEMP*(WATER/GAMA(11))**2.0 A4 = XK4*R*TEMP*(WATER/GAMA(10))**2.0 MOLAL(1) = MOLAL(1) + WAER(4) + WAER(5) ! H+ increases because NO3, Cl are added. !C !C *** CALCULATE CONCENTRATIONS ****************************************** !C *** ASSUME THAT 'DELT' FROM HNO3 >> 'DELT' FROM HCL !C CALL CALCNIAQ2p1 (WAER(4), MOLAL(1)+MOLAL(7)+MOLAL(4), DELT) MOLAL(1) = MOLAL(1) - DELT MOLAL(7) = WAER(4) - DELT ! NO3- = Waer(4) minus any turned into (HNO3aq) GASAQ(3) = DELT !C CALL CALCCLAQ2p1 (WAER(5), MOLAL(1)+MOLAL(7)+MOLAL(4), DELT) MOLAL(1) = MOLAL(1) - DELT MOLAL(4) = WAER(5) - DELT ! Cl- = Waer(4) minus any turned into (HNO3aq) GASAQ(2) = DELT !C GHNO3 = MOLAL(1)*MOLAL(7)/A4 GHCL = MOLAL(1)*MOLAL(4)/A3 !C RETURN !C !C *** END OF SUBROUTINE CALCNHP ***************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE II !C *** SUBROUTINE CALCHCO3 !C *** CORRECTS FOR H+ WHEN CRUSTALS ARE IN EXCESS !C !C CARBONATES ARE IN EXCESS, HCO3- IS ASSUMED A MINOR SPECIES, !C THE H+ CONCENTRATION IS CALCULATED FROM THE !C CO2(aq) + H2O <-> (HCO3-) + (H+) !C HCO3- <-> (H+) + (CO3--) EQUILIBRIUM. !C THE CO3-- CONCENTRATION IS ASSUMED NEGLIGIBLE WITH RESPECT TO HCO3- !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY CHRISTOS FOUNTOUKIS AND ATHANASIOS NENES !C !C======================================================================= !C !C SUBROUTINE CALCHCO3 !C INCLUDE 'module_isrpia_inc.F' !C DOUBLE PRECISION KAPA !CCC CHARACTER ERRINF*40 !CC !CC *** SPECIAL CASE; WATER=ZERO ****************************************** !CC !C IF (WATER.LE.TINY) THEN !C GOTO 521 !C ENDIF !CC !CC *** CALCULATE CO2 DISSOLUTION ***************************************** !CC !C REST = 2.D0*W(2) + W(4) + W(5) !CC !C DELT = 0.0d0 !CC DELT2 = 0.0d0 !C IF (W(1)+W(6)+W(7)+W(8).GT.REST) THEN !C KAPA = MOLAL(1) !CC !CC *** CALCULATE EQUILIBRIUM CONSTANTS *********************************** !CC !C ALFA = XK26*RH*(WATER/1.0) ! CO2(aq) + H2O !CC ALFA2 = XK27*(WATER/1.0) ! HCO3- !CC !CC *** CALCULATE CUBIC EQUATION COEFFICIENTS ***************************** !CC !C X = W(1)+W(6)+W(7)+W(8) - REST ! EXCESS OF CRUSTALS EQUALS HCO3- !CC !C BB =-(KAPA + X + ALFA) !C CC = KAPA*X !C DD = BB*BB - 4.D0*CC !CC !C IF (DD.GE.ZERO) THEN !C SQDD = SQRT(DD) !C DELT = 0.5*(-BB - SQDD) !C ELSE !C DELT = ZERO !C ENDIF !C !C ENDIF !CC !CC *** CALCULATE H+ ***************************************************** !CC !C MOLAL(1) = KAPA - DELT ! H+ !CC !C521 RETURN !CC !CC *** END OF SUBROUTINE CALCHCO3 *************************************** !CC !C END !CC !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCAMAQ !C *** THIS SUBROUTINE CALCULATES THE NH3(aq) GENERATED FROM (H,NH4+). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCAMAQ2p1 (NH4I, OHI, DELT) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION NH4I !CC CHARACTER ERRINF*40 !C !C *** EQUILIBRIUM CONSTANTS !C A22 = XK22/XKW/WATER*(GAMA(8)/GAMA(9))**2. ! GAMA(NH3) ASSUMED 1 AKW = XKW *RH*WATER*WATER !C !C *** FIND ROOT !C OM1 = NH4I OM2 = OHI BB =-(OM1+OM2+A22*AKW) CC = OM1*OM2 DD = SQRT(BB*BB-4.D0*CC) DEL1 = 0.5D0*(-BB - DD) DEL2 = 0.5D0*(-BB + DD) !C !C *** GET APPROPRIATE ROOT. !C IF (DEL1.LT.ZERO) THEN IF (DEL2.GT.NH4I .OR. DEL2.GT.OHI) THEN DELT = ZERO ELSE DELT = DEL2 ENDIF ELSE DELT = DEL1 ENDIF !CC !CC *** COMPARE DELTA TO TOTAL NH4+ ; ESTIMATE EFFECT ********************* !CC !CC IF (DELTA/HYD.GT.0.1d0) THEN !CC WRITE (ERRINF,'(1PE10.3)') DELTA/HYD*100.0 !CC CALL PUSHERR (0020, ERRINF) !CC ENDIF !C RETURN !C !C *** END OF SUBROUTINE CALCAMAQ **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCAMAQ2 !C !C THIS SUBROUTINE CALCULATES THE NH3(aq) GENERATED FROM (H,NH4+). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCAMAQ22p1 (GGNH3, NH4I, OHI, NH3AQ) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION NH4I, NH3AQ !C !C *** EQUILIBRIUM CONSTANTS !C A22 = XK22/XKW/WATER*(GAMA(8)/GAMA(9))**2. ! GAMA(NH3) ASSUMED 1 AKW = XKW *RH*WATER*WATER !C !C *** FIND ROOT !C ALF1 = NH4I - GGNH3 ALF2 = GGNH3 BB = ALF1 + A22*AKW CC =-A22*AKW*ALF2 DEL = 0.5D0*(-BB + SQRT(BB*BB-4.D0*CC)) !C !C *** ADJUST CONCENTRATIONS !C NH4I = ALF1 + DEL OHI = DEL IF (OHI.LE.TINY) OHI = SQRT(AKW) ! If solution is neutral. NH3AQ = ALF2 - DEL !C RETURN !C !C *** END OF SUBROUTINE CALCAMAQ2 **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCCLAQ !C !C THIS SUBROUTINE CALCULATES THE HCL(aq) GENERATED FROM (H+,CL-). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCCLAQ2p1 (CLI, HI, DELT) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION CLI !C !C *** EQUILIBRIUM CONSTANTS !C A32 = XK32*WATER/(GAMA(11))**2. ! GAMA(HCL) ASSUMED 1 !C !C *** FIND ROOT !C OM1 = CLI OM2 = HI BB =-(OM1+OM2+A32) CC = OM1*OM2 DD = SQRT(BB*BB-4.D0*CC) DEL1 = 0.5D0*(-BB - DD) DEL2 = 0.5D0*(-BB + DD) !C !C *** GET APPROPRIATE ROOT. !C IF (DEL1.LT.ZERO) THEN IF (DEL2.LT.ZERO .OR. DEL2.GT.CLI .OR. DEL2.GT.HI) THEN DELT = ZERO ELSE DELT = DEL2 ENDIF ELSE DELT = DEL1 ENDIF !C RETURN !C !C *** END OF SUBROUTINE CALCCLAQ **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCCLAQ2 !C !C THIS SUBROUTINE CALCULATES THE HCL(aq) GENERATED FROM (H+,CL-). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCCLAQ22p1 (GGCL, CLI, HI, CLAQ) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION CLI !C !C *** EQUILIBRIUM CONSTANTS !C A32 = XK32*WATER/(GAMA(11))**2. ! GAMA(HCL) ASSUMED 1 AKW = XKW *RH*WATER*WATER !C !C *** FIND ROOT !C ALF1 = CLI - GGCL ALF2 = GGCL COEF = (ALF1+A32) DEL1 = 0.5*(-COEF + SQRT(COEF*COEF+4.D0*A32*ALF2)) !C !C *** CORRECT CONCENTRATIONS !C CLI = ALF1 + DEL1 HI = DEL1 IF (HI.LE.TINY) HI = SQRT(AKW) ! If solution is neutral. CLAQ = ALF2 - DEL1 !C RETURN !C !C *** END OF SUBROUTINE CALCCLAQ2 **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNIAQ !C !C THIS SUBROUTINE CALCULATES THE HNO3(aq) GENERATED FROM (H,NO3-). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNIAQ2p1 (NO3I, HI, DELT) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION NO3I, HI, DELT !C !C *** EQUILIBRIUM CONSTANTS !C A42 = XK42*WATER/(GAMA(10))**2. ! GAMA(HNO3) ASSUMED 1 !C !C *** FIND ROOT !C OM1 = NO3I OM2 = HI BB =-(OM1+OM2+A42) CC = OM1*OM2 DD = SQRT(BB*BB-4.D0*CC) DEL1 = 0.5D0*(-BB - DD) DEL2 = 0.5D0*(-BB + DD) !C !C *** GET APPROPRIATE ROOT. !C IF (DEL1.LT.ZERO .OR. DEL1.GT.HI .OR. DEL1.GT.NO3I) THEN ! print *, DELT DELT = ZERO ELSE DELT = DEL1 RETURN ENDIF !C IF (DEL2.LT.ZERO .OR. DEL2.GT.NO3I .OR. DEL2.GT.HI) THEN DELT = ZERO ELSE DELT = DEL2 ENDIF !C RETURN !C !C *** END OF SUBROUTINE CALCNIAQ **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCNIAQ2 !C !C THIS SUBROUTINE CALCULATES THE UNDISSOCIATED HNO3(aq) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCNIAQ22p1 (GGNO3, NO3I, HI, NO3AQ) INCLUDE 'module_isrpia_inc.F' DOUBLE PRECISION NO3I, NO3AQ !C !C *** EQUILIBRIUM CONSTANTS !C A42 = XK42*WATER/(GAMA(10))**2. ! GAMA(HNO3) ASSUMED 1 AKW = XKW *RH*WATER*WATER !C !C *** FIND ROOT !C ALF1 = NO3I - GGNO3 ALF2 = GGNO3 ALF3 = HI !C BB = ALF3 + ALF1 + A42 CC = ALF3*ALF1 - A42*ALF2 DEL1 = 0.5*(-BB + SQRT(BB*BB-4.D0*CC)) !C !C *** CORRECT CONCENTRATIONS !C NO3I = ALF1 + DEL1 HI = ALF3 + DEL1 IF (HI.LE.TINY) HI = SQRT(AKW) ! If solution is neutral. NO3AQ = ALF2 - DEL1 !C RETURN !C !C *** END OF SUBROUTINE CALCNIAQ2 **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCMR !C *** THIS SUBROUTINE CALCULATES: !C 1. ION PAIR CONCENTRATIONS (FROM [MOLAR] ARRAY) !C 2. WATER CONTENT OF LIQUID AEROSOL PHASE (FROM ZSR CORRELATION) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCMR2p1 INCLUDE 'module_isrpia_inc.F' COMMON /SOLUT2p1/ CHI1, CHI2, CHI3, CHI4, CHI5, CHI6, CHI7, CHI8,& CHI9, CHI10, CHI11, CHI12, CHI13, CHI14, CHI15,& CHI16, CHI17, PSI1, PSI2, PSI3, PSI4, PSI5, PSI6,& PSI7, PSI8, PSI9, PSI10, PSI11, PSI12, PSI13,& PSI14, PSI15, PSI16, PSI17, A1, A2, A3, A4, A5, A6,& A7, A8, A9, A10, A11, A12, A13, A14, A15, A16, A17 !C CHARACTER SC*1 !C !C *** CALCULATE ION PAIR CONCENTRATIONS ACCORDING TO SPECIFIC CASE **** !C SC =SCASE(1:1) ! SULRAT & SODRAT case !C !C *** NH4-SO4 SYSTEM ; SULFATE POOR CASE !C IF (SC.EQ.'A') THEN MOLALR(4) = MOLAL(5)+MOLAL(6) ! (NH4)2SO4 - CORRECT FOR SO4 TO HSO4 !C !C *** NH4-SO4 SYSTEM ; SULFATE RICH CASE ; NO FREE ACID !C ELSE IF (SC.EQ.'B') THEN SO4I = MOLAL(5)-MOLAL(1) ! CORRECT FOR HSO4 DISSOCIATION HSO4I = MOLAL(6)+MOLAL(1) IF (SO4I.LT.HSO4I) THEN MOLALR(13) = SO4I ! [LC] = [SO4] MOLALR(9) = MAX(HSO4I-SO4I, ZERO) ! NH4HSO4 ELSE MOLALR(13) = HSO4I ! [LC] = [HSO4] MOLALR(4) = MAX(SO4I-HSO4I, ZERO) ! (NH4)2SO4 ENDIF !C !C *** NH4-SO4 SYSTEM ; SULFATE RICH CASE ; FREE ACID !C ELSE IF (SC.EQ.'C') THEN MOLALR(4) = MOLAL(3) ! NH4HSO4 MOLALR(7) = MAX(W(2)-W(3), ZERO) ! H2SO4 !C !C *** NH4-SO4-NO3 SYSTEM ; SULFATE POOR CASE !C ELSE IF (SC.EQ.'D') THEN MOLALR(4) = MOLAL(5) + MOLAL(6) ! (NH4)2SO4 AML5 = MOLAL(3)-2.D0*MOLALR(4) ! "free" NH4 MOLALR(5) = MAX(MIN(AML5,MOLAL(7)), ZERO)! NH4NO3 = MIN("free", NO3) !C !C *** NH4-SO4-NO3 SYSTEM ; SULFATE RICH CASE ; NO FREE ACID !C ELSE IF (SC.EQ.'E') THEN SO4I = MAX(MOLAL(5)-MOLAL(1),ZERO) ! FROM HSO4 DISSOCIATION HSO4I = MOLAL(6)+MOLAL(1) IF (SO4I.LT.HSO4I) THEN MOLALR(13) = SO4I ! [LC] = [SO4] MOLALR(9) = MAX(HSO4I-SO4I, ZERO) ! NH4HSO4 ELSE MOLALR(13) = HSO4I ! [LC] = [HSO4] MOLALR(4) = MAX(SO4I-HSO4I, ZERO) ! (NH4)2SO4 ENDIF !C !C *** NH4-SO4-NO3 SYSTEM ; SULFATE RICH CASE ; FREE ACID !C ELSE IF (SC.EQ.'F') THEN MOLALR(4) = MOLAL(3) ! NH4HSO4 MOLALR(7) = MAX(MOLAL(5)+MOLAL(6)-MOLAL(3),ZERO) ! H2SO4 !C !C *** NA-NH4-SO4-NO3-CL SYSTEM ; SULFATE POOR ; SODIUM POOR CASE !C ELSE IF (SC.EQ.'G') THEN MOLALR(2) = 0.5D0*MOLAL(2) ! NA2SO4 TOTS4 = MOLAL(5)+MOLAL(6) ! Total SO4 MOLALR(4) = MAX(TOTS4 - MOLALR(2), ZERO) ! (NH4)2SO4 FRNH4 = MAX(MOLAL(3) - 2.D0*MOLALR(4), ZERO) MOLALR(5) = MIN(MOLAL(7),FRNH4) ! NH4NO3 FRNH4 = MAX(FRNH4 - MOLALR(5), ZERO) MOLALR(6) = MIN(MOLAL(4), FRNH4) ! NH4CL !C !C *** NA-NH4-SO4-NO3-CL SYSTEM ; SULFATE POOR ; SODIUM RICH CASE !C *** RETREIVE DISSOLVED SALTS DIRECTLY FROM COMMON BLOCK /SOLUT/ !C ELSE IF (SC.EQ.'H') THEN MOLALR(1) = PSI7 ! NACL MOLALR(2) = PSI1 ! NA2SO4 MOLALR(3) = PSI8 ! NANO3 MOLALR(4) = ZERO ! (NH4)2SO4 FRNO3 = MAX(MOLAL(7) - MOLALR(3), ZERO) ! "FREE" NO3 FRCL = MAX(MOLAL(4) - MOLALR(1), ZERO) ! "FREE" CL MOLALR(5) = MIN(MOLAL(3),FRNO3) ! NH4NO3 FRNH4 = MAX(MOLAL(3) - MOLALR(5), ZERO) ! "FREE" NH3 MOLALR(6) = MIN(FRCL, FRNH4) ! NH4CL !C !C *** NA-NH4-SO4-NO3-CL SYSTEM ; SULFATE RICH CASE ; NO FREE ACID !C *** RETREIVE DISSOLVED SALTS DIRECTLY FROM COMMON BLOCK /SOLUT/ !C ELSE IF (SC.EQ.'I') THEN MOLALR(04) = PSI5 ! (NH4)2SO4 MOLALR(02) = PSI4 ! NA2SO4 MOLALR(09) = PSI1 ! NH4HSO4 MOLALR(12) = PSI3 ! NAHSO4 MOLALR(13) = PSI2 ! LC !C !C *** NA-NH4-SO4-NO3-CL SYSTEM ; SULFATE RICH CASE ; FREE ACID !C ELSE IF (SC.EQ.'J') THEN MOLALR(09) = MOLAL(3) ! NH4HSO4 MOLALR(12) = MOLAL(2) ! NAHSO4 MOLALR(07) = MOLAL(5)+MOLAL(6)-MOLAL(3)-MOLAL(2) ! H2SO4 MOLALR(07) = MAX(MOLALR(07),ZERO) !C !C *** NA-NH4-SO4-NO3-CL-CA-K-MG SYSTEM ; SULFATE POOR ; CR+NA POOR CASE !C ELSE IF (SC.EQ.'O') THEN MOLALR(2) = 0.5D0*MOLAL(2) ! NA2SO4 TOTS4 = MOLAL(5)+MOLAL(6) ! Total SO4 MOLALR(17)= 0.5*MOLAL(9) ! K2SO4 MOLALR(21)= MOLAL(10) ! MGSO4 MOLALR(4) = MAX(TOTS4 - MOLALR(2) - MOLALR(17) & - MOLALR(21), ZERO) ! (NH4)2SO4 FRNH4 = MAX(MOLAL(3) - 2.D0*MOLALR(4), ZERO) MOLALR(5) = MIN(MOLAL(7),FRNH4) ! NH4NO3 FRNH4 = MAX(FRNH4 - MOLALR(5), ZERO) MOLALR(6) = MIN(MOLAL(4), FRNH4) ! NH4CL !C !C *** NA-NH4-SO4-NO3-CL-CA-K-MG SYSTEM ; SULFATE POOR ; CR+NA RICH; CR POOR CASE !C *** RETREIVE DISSOLVED SALTS DIRECTLY FROM COMMON BLOCK /SOLUT/ !C ELSE IF (SC.EQ.'M') THEN MOLALR(1) = PSI7 ! NACL MOLALR(2) = PSI1 ! NA2SO4 MOLALR(3) = PSI8 ! NANO3 MOLALR(4) = ZERO ! (NH4)2SO4 FRNO3 = MAX(MOLAL(7) - MOLALR(3), ZERO) ! "FREE" NO3 FRCL = MAX(MOLAL(4) - MOLALR(1), ZERO) ! "FREE" CL MOLALR(5) = MIN(MOLAL(3),FRNO3) ! NH4NO3 FRNH4 = MAX(MOLAL(3) - MOLALR(5), ZERO) ! "FREE" NH3 MOLALR(6) = MIN(FRCL, FRNH4) ! NH4CL MOLALR(17)= PSI9 ! K2SO4 MOLALR(21)= PSI10 ! MGSO4 !C !C *** NA-NH4-SO4-NO3-CL-CA-K-MG SYSTEM ; SULFATE POOR ; CR+NA RICH; CR RICH CASE !C *** RETREIVE DISSOLVED SALTS DIRECTLY FROM COMMON BLOCK /SOLUT/ !C ELSE IF (SC.EQ.'P') THEN MOLALR(1) = PSI7 ! NACL MOLALR(3) = PSI8 ! NANO3 MOLALR(15)= PSI12 ! CANO32 MOLALR(16)= PSI17 ! CACL2 MOLALR(19)= PSI13 ! KNO3 MOLALR(20)= PSI14 ! KCL MOLALR(22)= PSI15 ! MGNO32 MOLALR(23)= PSI16 ! MGCL2 FRNO3 = MAX(MOLAL(7)-MOLALR(3)-2.D0*MOLALR(15) & -MOLALR(19)-2.D0*MOLALR(22), ZERO) ! "FREE" NO3 FRCL = MAX(MOLAL(4)-MOLALR(1)-2.D0*MOLALR(16) & -MOLALR(20)-2.D0*MOLALR(23), ZERO) ! "FREE" CL MOLALR(5) = MIN(MOLAL(3),FRNO3) ! NH4NO3 FRNH4 = MAX(MOLAL(3) - MOLALR(5), ZERO) ! "FREE" NH3 MOLALR(6) = MIN(FRCL, FRNH4) ! NH4CL MOLALR(17)= PSI9 ! K2SO4 MOLALR(21)= PSI10 ! MGSO4 !C !C *** NA-NH4-SO4-NO3-CL-CA-K-MG SYSTEM ; SULFATE RICH CASE ; NO FREE ACID !C ELSE IF (SC.EQ.'L') THEN MOLALR(04) = PSI5 ! (NH4)2SO4 MOLALR(02) = PSI4 ! NA2SO4 MOLALR(09) = PSI1 ! NH4HSO4 MOLALR(12) = PSI3 ! NAHSO4 MOLALR(13) = PSI2 ! LC MOLALR(17) = PSI6 ! K2SO4 MOLALR(21) = PSI7 ! MGSO4 MOLALR(18) = PSI8 ! KHSO4 !C !C *** NA-NH4-SO4-NO3-CL-CA-K-MG SYSTEM ; SULFATE SUPER RICH CASE ; FREE ACID !C ELSE IF (SC.EQ.'K') THEN MOLALR(09) = MOLAL(3) ! NH4HSO4 MOLALR(12) = MOLAL(2) ! NAHSO4 MOLALR(14) = MOLAL(8) ! CASO4 MOLALR(18) = MOLAL(9) ! KHSO4 MOLALR(21) = MOLAL(10) ! MGSO4 MOLALR(07) = MOLAL(5)+MOLAL(6)-MOLAL(3) & -MOLAL(2)-MOLAL(8)-MOLAL(9)-MOLAL(10) ! H2SO4 MOLALR(07) = MAX(MOLALR(07),ZERO) !C !C ======= REVERSE PROBLEMS =========================================== !C !C *** NH4-SO4-NO3 SYSTEM ; SULFATE POOR CASE !C ELSE IF (SC.EQ.'N') THEN MOLALR(4) = MOLAL(5) + MOLAL(6) ! (NH4)2SO4 AML5 = WAER(3)-2.D0*MOLALR(4) ! "free" NH4 MOLALR(5) = MAX(MIN(AML5,WAER(4)), ZERO) ! NH4NO3 = MIN("free", NO3) !C !C *** NH4-SO4-NO3-NA-CL SYSTEM ; SULFATE POOR, SODIUM POOR CASE !C ELSE IF (SC.EQ.'Q') THEN MOLALR(2) = PSI1 ! NA2SO4 MOLALR(4) = PSI6 ! (NH4)2SO4 MOLALR(5) = PSI5 ! NH4NO3 MOLALR(6) = PSI4 ! NH4CL !C !C *** NH4-SO4-NO3-NA-CL SYSTEM ; SULFATE POOR, SODIUM RICH CASE !C ELSE IF (SC.EQ.'R') THEN MOLALR(1) = PSI3 ! NACL MOLALR(2) = PSI1 ! NA2SO4 MOLALR(3) = PSI2 ! NANO3 MOLALR(4) = ZERO ! (NH4)2SO4 MOLALR(5) = PSI5 ! NH4NO3 MOLALR(6) = PSI4 ! NH4CL !C !C *** NH4-SO4-NO3-NA-CL-CA-K-MG SYSTEM ; SULFATE POOR, CRUSTAL&SODIUM POOR CASE !C ELSE IF (SC.EQ.'V') THEN MOLALR(2) = PSI1 ! NA2SO4 MOLALR(4) = PSI6 ! (NH4)2SO4 MOLALR(5) = PSI5 ! NH4NO3 MOLALR(6) = PSI4 ! NH4CL MOLALR(17)= PSI7 ! K2SO4 MOLALR(21)= PSI8 ! MGSO4 !C !C *** NH4-SO4-NO3-NA-CL-CA-K-MG SYSTEM ; SULFATE POOR, CRUSTAL&SODIUM RICH, CRUSTAL POOR CASE !C ELSE IF (SC.EQ.'U') THEN MOLALR(1) = PSI3 ! NACL MOLALR(2) = PSI1 ! NA2SO4 MOLALR(3) = PSI2 ! NANO3 MOLALR(5) = PSI5 ! NH4NO3 MOLALR(6) = PSI4 ! NH4CL MOLALR(17)= PSI7 ! K2SO4 MOLALR(21)= PSI8 ! MGSO4 !C !C *** NH4-SO4-NO3-NA-CL-CA-K-MG SYSTEM ; SULFATE POOR, CRUSTAL&SODIUM RICH, CRUSTAL RICH CASE !C ELSE IF (SC.EQ.'W') THEN MOLALR(1) = PSI7 ! NACL MOLALR(3) = PSI8 ! NANO3 MOLALR(5) = PSI6 ! NH4NO3 MOLALR(6) = PSI5 ! NH4CL MOLALR(15)= PSI12 ! CANO32 MOLALR(16)= PSI17 ! CACL2 MOLALR(17)= PSI9 ! K2SO4 MOLALR(19)= PSI13 ! KNO3 MOLALR(20)= PSI14 ! KCL MOLALR(21)= PSI10 ! MGSO4 MOLALR(22)= PSI15 ! MGNO32 MOLALR(23)= PSI16 ! MGCL2 !C !C *** UNKNOWN CASE !C !C ELSE !C CALL PUSHERR (1001, ' ') ! FATAL ERROR: CASE NOT SUPPORTED ENDIF !C !C *** CALCULATE WATER CONTENT ; ZSR CORRELATION *********************** !C WATER = ZERO DO 10 I=1,NPAIR WATER = WATER + MOLALR(I)/M0(I) 10 CONTINUE WATER = MAX(WATER, TINY) !C RETURN !C !C *** END OF SUBROUTINE CALCMR ****************************************** !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCMDRH !C !C THIS IS THE CASE WHERE THE RELATIVE HUMIDITY IS IN THE MUTUAL !C DRH REGION. THE SOLUTION IS ASSUMED TO BE THE SUM OF TWO WEIGHTED !C SOLUTIONS ; THE 'DRY' SOLUTION (SUBROUTINE DRYCASE) AND THE !C 'SATURATED LIQUID' SOLUTION (SUBROUTINE LIQCASE). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCMDRH2p1 (RHI, RHDRY, RHLIQ, DRYCASE2p1, LIQCASE2p1) INCLUDE 'module_isrpia_inc.F' EXTERNAL DRYCASE2p1, LIQCASE2p1 !C !C *** FIND WEIGHT FACTOR ********************************************** !C IF (WFTYP.EQ.0) THEN WF = ONE ELSEIF (WFTYP.EQ.1) THEN WF = 0.5D0 ELSE WF = (RHLIQ-RHI)/(RHLIQ-RHDRY) ENDIF ONEMWF = ONE - WF !C !C *** FIND FIRST SECTION ; DRY ONE ************************************ !C CALL DRYCASE2p1 IF (ABS(ONEMWF).LE.1D-5) GOTO 200 ! DRY AEROSOL !C CNH42SO = CNH42S4 ! FIRST (DRY) SOLUTION CNH4HSO = CNH4HS4 CLCO = CLC CNH4N3O = CNH4NO3 CNH4CLO = CNH4CL CNA2SO = CNA2SO4 CNAHSO = CNAHSO4 CNANO = CNANO3 CNACLO = CNACL GNH3O = GNH3 GHNO3O = GHNO3 GHCLO = GHCL !C !C *** FIND SECOND SECTION ; DRY & LIQUID ****************************** !C CNH42S4 = ZERO CNH4HS4 = ZERO CLC = ZERO CNH4NO3 = ZERO CNH4CL = ZERO CNA2SO4 = ZERO CNAHSO4 = ZERO CNANO3 = ZERO CNACL = ZERO GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO CALL LIQCASE2p1 ! SECOND (LIQUID) SOLUTION !C !C *** ADJUST THINGS FOR THE CASE THAT THE LIQUID SUB PREDICTS DRY AEROSOL !C IF (WATER.LE.TINY) THEN DO 100 I=1,NIONS MOLAL(I)= ZERO ! Aqueous phase 100 CONTINUE WATER = ZERO !C CNH42S4 = CNH42SO ! Solid phase CNA2SO4 = CNA2SO CNAHSO4 = CNAHSO CNH4HS4 = CNH4HSO CLC = CLCO CNH4NO3 = CNH4N3O CNANO3 = CNANO CNACL = CNACLO CNH4CL = CNH4CLO !C GNH3 = GNH3O ! Gas phase GHNO3 = GHNO3O GHCL = GHCLO !C GOTO 200 ENDIF !C !C *** FIND SALT DISSOLUTIONS BETWEEN DRY & LIQUID SOLUTIONS. !C DAMSUL = CNH42SO - CNH42S4 DSOSUL = CNA2SO - CNA2SO4 DAMBIS = CNH4HSO - CNH4HS4 DSOBIS = CNAHSO - CNAHSO4 DLC = CLCO - CLC DAMNIT = CNH4N3O - CNH4NO3 DAMCHL = CNH4CLO - CNH4CL DSONIT = CNANO - CNANO3 DSOCHL = CNACLO - CNACL !C !C *** FIND GAS DISSOLUTIONS BETWEEN DRY & LIQUID SOLUTIONS. !C DAMG = GNH3O - GNH3 DHAG = GHCLO - GHCL DNAG = GHNO3O - GHNO3 !C !C *** FIND SOLUTION AT MDRH BY WEIGHTING DRY & LIQUID SOLUTIONS. !C !C LIQUID !C MOLAL(1)= ONEMWF*MOLAL(1) ! H+ MOLAL(2)= ONEMWF*(2.D0*DSOSUL + DSOBIS + DSONIT + DSOCHL) ! NA+ MOLAL(3)= ONEMWF*(2.D0*DAMSUL + DAMG + DAMBIS + DAMCHL + & 3.D0*DLC + DAMNIT ) ! NH4+ MOLAL(4)= ONEMWF*( DAMCHL + DSOCHL + DHAG) ! CL- MOLAL(5)= ONEMWF*( DAMSUL + DSOSUL + DLC - MOLAL(6)) ! SO4-- !VB 17 Sept 2001 MOLAL(6)= ONEMWF*( MOLAL(6) + DSOBIS + DAMBIS + DLC) ! HSO4- MOLAL(7)= ONEMWF*( DAMNIT + DSONIT + DNAG) ! NO3- WATER = ONEMWF*WATER !C !C SOLID !C CNH42S4 = WF*CNH42SO + ONEMWF*CNH42S4 CNA2SO4 = WF*CNA2SO + ONEMWF*CNA2SO4 CNAHSO4 = WF*CNAHSO + ONEMWF*CNAHSO4 CNH4HS4 = WF*CNH4HSO + ONEMWF*CNH4HS4 CLC = WF*CLCO + ONEMWF*CLC CNH4NO3 = WF*CNH4N3O + ONEMWF*CNH4NO3 CNANO3 = WF*CNANO + ONEMWF*CNANO3 CNACL = WF*CNACLO + ONEMWF*CNACL CNH4CL = WF*CNH4CLO + ONEMWF*CNH4CL !C !C GAS !C GNH3 = WF*GNH3O + ONEMWF*GNH3 GHNO3 = WF*GHNO3O + ONEMWF*GHNO3 GHCL = WF*GHCLO + ONEMWF*GHCL !C !C *** RETURN POINT !C 200 RETURN !C !C *** END OF SUBROUTINE CALCMDRH **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE II !C *** SUBROUTINE CALCMDRH2 !C !C THIS IS THE CASE WHERE THE RELATIVE HUMIDITY IS IN THE MUTUAL !C DRH REGION. THE SOLUTION IS ASSUMED TO BE THE SUM OF TWO WEIGHTED !C SOLUTIONS ; THE 'DRY' SOLUTION (SUBROUTINE DRYCASE) AND THE !C 'SATURATED LIQUID' SOLUTION (SUBROUTINE LIQCASE). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCMDRH22p1 (RHI, RHDRY, RHLIQ, DRYCASE2p1, LIQCASE2p1) INCLUDE 'module_isrpia_inc.F' EXTERNAL DRYCASE2p1, LIQCASE2p1 !C !C *** FIND WEIGHT FACTOR ********************************************** !C IF (WFTYP.EQ.0) THEN WF = ONE ELSEIF (WFTYP.EQ.1) THEN WF = 0.5D0 ELSE WF = (RHLIQ-RHI)/(RHLIQ-RHDRY) ENDIF ONEMWF = ONE - WF !C !C *** FIND FIRST SECTION ; DRY ONE ************************************ !C CALL DRYCASE2p1 IF (ABS(ONEMWF).LE.1D-5) GOTO 200 ! DRY AEROSOL !C CNH42SO = CNH42S4 ! FIRST (DRY) SOLUTION CNH4HSO = CNH4HS4 CLCO = CLC CNH4N3O = CNH4NO3 CNH4CLO = CNH4CL CNA2SO = CNA2SO4 CNAHSO = CNAHSO4 CNANO = CNANO3 CNACLO = CNACL GNH3O = GNH3 GHNO3O = GHNO3 GHCLO = GHCL !C CCASO = CCASO4 CK2SO = CK2SO4 CMGSO = CMGSO4 CKHSO = CKHSO4 CCAN32O = CCANO32 CCAC2L = CCACL2 CKN3O = CKNO3 CKCLO = CKCL CMGN32O = CMGNO32 CMGC2L = CMGCL2 !C !C *** FIND SECOND SECTION ; DRY & LIQUID ****************************** !C CNH42S4 = ZERO CNH4HS4 = ZERO CLC = ZERO CNH4NO3 = ZERO CNH4CL = ZERO CNA2SO4 = ZERO CNAHSO4 = ZERO CNANO3 = ZERO CNACL = ZERO GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO !C CCASO4 = ZERO CK2SO4 = ZERO CMGSO4 = ZERO CKHSO4 = ZERO CCANO32 = ZERO CCACL2 = ZERO CKNO3 = ZERO CKCL = ZERO CMGNO32 = ZERO CMGCL2 = ZERO !C CALL LIQCASE2p1 ! SECOND (LIQUID) SOLUTION !C !C *** ADJUST THINGS FOR THE CASE THAT THE LIQUID SUB PREDICTS DRY AEROSOL !C IF (WATER.LE.TINY) THEN DO 100 I=1,NIONS MOLAL(I)= ZERO ! Aqueous phase 100 CONTINUE WATER = ZERO !C CNH42S4 = CNH42SO ! Solid phase CNA2SO4 = CNA2SO CNAHSO4 = CNAHSO CNH4HS4 = CNH4HSO CLC = CLCO CNH4NO3 = CNH4N3O CNANO3 = CNANO CNACL = CNACLO CNH4CL = CNH4CLO !C GNH3 = GNH3O ! Gas phase GHNO3 = GHNO3O GHCL = GHCLO !C CCASO4 = CCASO CK2SO4 = CK2SO CMGSO4 = CMGSO CKHSO4 = CKHSO CCANO32 = CCAN32O CCACL2 = CCAC2L CKNO3 = CKN3O CKCL = CKCLO CMGNO32 = CMGN32O CMGCL2 = CMGC2L !C GOTO 200 ENDIF !C !C *** FIND SALT DISSOLUTIONS BETWEEN DRY & LIQUID SOLUTIONS. !C DAMSUL = CNH42SO - CNH42S4 DSOSUL = CNA2SO - CNA2SO4 DAMBIS = CNH4HSO - CNH4HS4 DSOBIS = CNAHSO - CNAHSO4 DLC = CLCO - CLC DAMNIT = CNH4N3O - CNH4NO3 DAMCHL = CNH4CLO - CNH4CL DSONIT = CNANO - CNANO3 DSOCHL = CNACLO - CNACL !C DCASUL = CCASO - CCASO4 DPOSUL = CK2SO - CK2SO4 DMGSUL = CMGSO - CMGSO4 DPOBIS = CKHSO - CKHSO4 DCANIT = CCAN32O - CCANO32 DCACHL = CCAC2L - CCACL2 DPONIT = CKN3O - CKNO3 DPOCHL = CKCLO - CKCL DMGNIT = CMGN32O - CMGNO32 DMGCHL = CMGC2L - CMGCL2 !C !C *** FIND GAS DISSOLUTIONS BETWEEN DRY & LIQUID SOLUTIONS. !C DAMG = GNH3O - GNH3 DHAG = GHCLO - GHCL DNAG = GHNO3O - GHNO3 !C !C *** FIND SOLUTION AT MDRH BY WEIGHTING DRY & LIQUID SOLUTIONS. !C !C LIQUID !C MOLAL(1) = ONEMWF*MOLAL(1) ! H+ MOLAL(2) = ONEMWF*(2.D0*DSOSUL + DSOBIS + DSONIT + DSOCHL) ! NA+ MOLAL(3) = ONEMWF*(2.D0*DAMSUL + DAMG + DAMBIS + DAMCHL + & 3.D0*DLC + DAMNIT ) ! NH4+ MOLAL(4) = ONEMWF*(DAMCHL + DSOCHL + DHAG + 2.D0*DCACHL + & 2.D0*DMGCHL + DPOCHL) ! CL- MOLAL(5) = ONEMWF*(DAMSUL + DSOSUL + DLC - MOLAL(6) & +DCASUL + DPOSUL + DMGSUL) ! SO4-- !VB 17 Sept 2001 MOLAL(6) = ONEMWF*(MOLAL(6) + DSOBIS + DAMBIS + DLC + DPOBIS) ! HSO4- MOLAL(7) = ONEMWF*(DAMNIT + DSONIT + DNAG + 2.D0*DCANIT & + 2.D0*DMGNIT + DPONIT) ! NO3- MOLAL(8) = ONEMWF*(DCASUL + DCANIT + DCACHL) ! CA2+ MOLAL(9) = ONEMWF*(2.D0*DPOSUL + DPONIT + DPOCHL + DPOBIS) ! K+ MOLAL(10)= ONEMWF*(DMGSUL + DMGNIT + DMGCHL) ! MG2+ WATER = ONEMWF*WATER !C !C SOLID !C CNH42S4 = WF*CNH42SO + ONEMWF*CNH42S4 CNA2SO4 = WF*CNA2SO + ONEMWF*CNA2SO4 CNAHSO4 = WF*CNAHSO + ONEMWF*CNAHSO4 CNH4HS4 = WF*CNH4HSO + ONEMWF*CNH4HS4 CLC = WF*CLCO + ONEMWF*CLC CNH4NO3 = WF*CNH4N3O + ONEMWF*CNH4NO3 CNANO3 = WF*CNANO + ONEMWF*CNANO3 CNACL = WF*CNACLO + ONEMWF*CNACL CNH4CL = WF*CNH4CLO + ONEMWF*CNH4CL !C CCASO4 = WF*CCASO + ONEMWF*CCASO4 CK2SO4 = WF*CK2SO + ONEMWF*CK2SO4 CMGSO4 = WF*CMGSO + ONEMWF*CMGSO4 CKHSO4 = WF*CKHSO + ONEMWF*CKHSO4 CCANO32 = WF*CCAN32O + ONEMWF*CCANO32 CCACL2 = WF*CCAC2L + ONEMWF*CCACL2 CMGNO32 = WF*CMGN32O + ONEMWF*CMGNO32 CMGCL2 = WF*CMGC2L + ONEMWF*CMGCL2 CKCL = WF*CKCLO + ONEMWF*CKCL !C !C GAS !C GNH3 = WF*GNH3O + ONEMWF*GNH3 GHNO3 = WF*GHNO3O + ONEMWF*GHNO3 GHCL = WF*GHCLO + ONEMWF*GHCL !C !C *** RETURN POINT !C 200 RETURN !C !C *** END OF SUBROUTINE CALCMDRH2 **************************************** !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCMDRP !C !C THIS IS THE CASE WHERE THE RELATIVE HUMIDITY IS IN THE MUTUAL !C DRH REGION. THE SOLUTION IS ASSUMED TO BE THE SUM OF TWO WEIGHTED !C SOLUTIONS ; THE 'DRY' SOLUTION (SUBROUTINE DRYCASE) AND THE !C 'SATURATED LIQUID' SOLUTION (SUBROUTINE LIQCASE). (REVERSE PROBLEM) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCMDRP2p1 (RHI, RHDRY, RHLIQ, DRYCASE2p1, LIQCASE2p1) INCLUDE 'module_isrpia_inc.F' EXTERNAL DRYCASE2p1, LIQCASE2p1 !C !C *** FIND WEIGHT FACTOR ********************************************** !C IF (WFTYP.EQ.0) THEN WF = ONE ELSEIF (WFTYP.EQ.1) THEN WF = 0.5D0 ELSE WF = (RHLIQ-RHI)/(RHLIQ-RHDRY) ENDIF ONEMWF = ONE - WF !C !C *** FIND FIRST SECTION ; DRY ONE ************************************ !C CALL DRYCASE2p1 IF (ABS(ONEMWF).LE.1D-5) GOTO 200 ! DRY AEROSOL !C CNH42SO = CNH42S4 ! FIRST (DRY) SOLUTION CNH4HSO = CNH4HS4 CLCO = CLC CNH4N3O = CNH4NO3 CNH4CLO = CNH4CL CNA2SO = CNA2SO4 CNAHSO = CNAHSO4 CNANO = CNANO3 CNACLO = CNACL !C !C *** FIND SECOND SECTION ; DRY & LIQUID ****************************** !C CNH42S4 = ZERO CNH4HS4 = ZERO CLC = ZERO CNH4NO3 = ZERO CNH4CL = ZERO CNA2SO4 = ZERO CNAHSO4 = ZERO CNANO3 = ZERO CNACL = ZERO GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO CALL LIQCASE2p1 ! SECOND (LIQUID) SOLUTION !C !C *** ADJUST THINGS FOR THE CASE THAT THE LIQUID SUB PREDICTS DRY AEROSOL !C IF (WATER.LE.TINY) THEN WATER = ZERO DO 100 I=1,NIONS MOLAL(I)= ZERO 100 CONTINUE CALL DRYCASE2p1 GOTO 200 ENDIF !C !C *** FIND SALT DISSOLUTIONS BETWEEN DRY & LIQUID SOLUTIONS. !C DAMBIS = CNH4HSO - CNH4HS4 DSOBIS = CNAHSO - CNAHSO4 DLC = CLCO - CLC !C !C *** FIND SOLUTION AT MDRH BY WEIGHTING DRY & LIQUID SOLUTIONS. !C !C *** SOLID !C CNH42S4 = WF*CNH42SO + ONEMWF*CNH42S4 CNA2SO4 = WF*CNA2SO + ONEMWF*CNA2SO4 CNAHSO4 = WF*CNAHSO + ONEMWF*CNAHSO4 CNH4HS4 = WF*CNH4HSO + ONEMWF*CNH4HS4 CLC = WF*CLCO + ONEMWF*CLC CNH4NO3 = WF*CNH4N3O + ONEMWF*CNH4NO3 CNANO3 = WF*CNANO + ONEMWF*CNANO3 CNACL = WF*CNACLO + ONEMWF*CNACL CNH4CL = WF*CNH4CLO + ONEMWF*CNH4CL !C !C *** LIQUID !C WATER = ONEMWF*WATER !C MOLAL(2)= WAER(1) - 2.D0*CNA2SO4 - CNAHSO4 - CNANO3 - & CNACL ! NA+ MOLAL(3)= WAER(3) - 2.D0*CNH42S4 - CNH4HS4 - CNH4CL - & 3.D0*CLC - CNH4NO3 ! NH4+ MOLAL(4)= WAER(5) - CNACL - CNH4CL ! CL- MOLAL(7)= WAER(4) - CNANO3 - CNH4NO3 ! NO3- MOLAL(6)= ONEMWF*(MOLAL(6) + DSOBIS + DAMBIS + DLC) ! HSO4- MOLAL(5)= WAER(2) - MOLAL(6) - CLC - CNH42S4 - CNA2SO4 ! SO4-- !C A8 = XK1*WATER/GAMA(7)*(GAMA(8)/GAMA(7))**2. IF (MOLAL(5).LE.TINY) THEN HIEQ = SQRT(XKW *RH*WATER*WATER) ! Neutral solution ELSE HIEQ = A8*MOLAL(6)/MOLAL(5) ENDIF HIEN = MOLAL(4) + MOLAL(7) + MOLAL(6) + 2.D0*MOLAL(5) - & MOLAL(2) - MOLAL(3) MOLAL(1)= MAX (HIEQ, HIEN) ! H+ !C !C *** GAS (ACTIVITY COEFS FROM LIQUID SOLUTION) !C A2 = (XK2/XKW)*R*TEMP*(GAMA(10)/GAMA(5))**2. ! NH3 <==> NH4+ A3 = XK4 *R*TEMP*(WATER/GAMA(10))**2. ! HNO3 <==> NO3- A4 = XK3 *R*TEMP*(WATER/GAMA(11))**2. ! HCL <==> CL- !C GNH3 = MOLAL(3)/MAX(MOLAL(1),TINY)/A2 GHNO3 = MOLAL(1)*MOLAL(7)/A3 GHCL = MOLAL(1)*MOLAL(4)/A4 !C 200 RETURN !C !C *** END OF SUBROUTINE CALCMDRP **************************************** !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCMDRPII !C !C THIS IS THE CASE WHERE THE RELATIVE HUMIDITY IS IN THE MUTUAL !C DRH REGION. THE SOLUTION IS ASSUMED TO BE THE SUM OF TWO WEIGHTED !C SOLUTIONS ; THE 'DRY' SOLUTION (SUBROUTINE DRYCASE) AND THE !C 'SATURATED LIQUID' SOLUTION (SUBROUTINE LIQCASE). (REVERSE PROBLEM) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCMDRPII2p1 (RHI, RHDRY, RHLIQ, DRYCASE2p1, LIQCASE2p1) INCLUDE 'module_isrpia_inc.F' EXTERNAL DRYCASE2p1, LIQCASE2p1 !C !C *** FIND WEIGHT FACTOR ********************************************** !C IF (WFTYP.EQ.0) THEN WF = ONE ELSEIF (WFTYP.EQ.1) THEN WF = 0.5D0 ELSE WF = (RHLIQ-RHI)/(RHLIQ-RHDRY) ENDIF ONEMWF = ONE - WF !C !C *** FIND FIRST SECTION ; DRY ONE ************************************ !C CALL DRYCASE2p1 IF (ABS(ONEMWF).LE.1D-5) GOTO 200 ! DRY AEROSOL !C CNH42SO = CNH42S4 ! FIRST (DRY) SOLUTION CNH4HSO = CNH4HS4 CLCO = CLC CNH4N3O = CNH4NO3 CNH4CLO = CNH4CL CNA2SO = CNA2SO4 CNAHSO = CNAHSO4 CNANO = CNANO3 CNACLO = CNACL !C CCASO = CCASO4 CK2SO = CK2SO4 CMGSO = CMGSO4 CKHSO = CKHSO4 CCAN32O = CCANO32 CCAC2L = CCACL2 CKN3O = CKNO3 CKCLO = CKCL CMGN32O = CMGNO32 CMGC2L = CMGCL2 !C !C *** FIND SECOND SECTION ; DRY & LIQUID ****************************** !C CNH42S4 = ZERO CNH4HS4 = ZERO CLC = ZERO CNH4NO3 = ZERO CNH4CL = ZERO CNA2SO4 = ZERO CNAHSO4 = ZERO CNANO3 = ZERO CNACL = ZERO GNH3 = ZERO GHNO3 = ZERO GHCL = ZERO !C CCASO4 = ZERO CK2SO4 = ZERO CMGSO4 = ZERO CKHSO4 = ZERO CCANO32 = ZERO CCACL2 = ZERO CKNO3 = ZERO CKCL = ZERO CMGNO32 = ZERO CMGCL2 = ZERO !C CALL LIQCASE2p1 ! SECOND (LIQUID) SOLUTION !C !C *** ADJUST THINGS FOR THE CASE THAT THE LIQUID SUB PREDICTS DRY AEROSOL !C IF (WATER.LE.TINY) THEN WATER = ZERO DO 100 I=1,NIONS MOLAL(I)= ZERO 100 CONTINUE CALL DRYCASE2p1 GOTO 200 ENDIF !C !C *** FIND SALT DISSOLUTIONS BETWEEN DRY & LIQUID SOLUTIONS. !C DAMBIS = CNH4HSO - CNH4HS4 DSOBIS = CNAHSO - CNAHSO4 DLC = CLCO - CLC DPOBIS = CKHSO - CKHSO4 !C !C *** FIND SOLUTION AT MDRH BY WEIGHTING DRY & LIQUID SOLUTIONS. !C !C *** SOLID !C CNH42S4 = WF*CNH42SO + ONEMWF*CNH42S4 CNA2SO4 = WF*CNA2SO + ONEMWF*CNA2SO4 CNAHSO4 = WF*CNAHSO + ONEMWF*CNAHSO4 CNH4HS4 = WF*CNH4HSO + ONEMWF*CNH4HS4 CLC = WF*CLCO + ONEMWF*CLC CNH4NO3 = WF*CNH4N3O + ONEMWF*CNH4NO3 CNANO3 = WF*CNANO + ONEMWF*CNANO3 CNACL = WF*CNACLO + ONEMWF*CNACL CNH4CL = WF*CNH4CLO + ONEMWF*CNH4CL !C CCASO4 = WF*CCASO + ONEMWF*CCASO4 CK2SO4 = WF*CK2SO + ONEMWF*CK2SO4 CMGSO4 = WF*CMGSO + ONEMWF*CMGSO4 CKHSO4 = WF*CKHSO + ONEMWF*CKHSO4 CCANO32 = WF*CCAN32O + ONEMWF*CCANO32 CCACL2 = WF*CCAC2L + ONEMWF*CCACL2 CMGNO32 = WF*CMGN32O + ONEMWF*CMGNO32 CMGCL2 = WF*CMGC2L + ONEMWF*CMGCL2 CKCL = WF*CKCLO + ONEMWF*CKCL !C !C *** LIQUID !C WATER = ONEMWF*WATER !C MOLAL(2)= WAER(1) - 2.D0*CNA2SO4 - CNAHSO4 - CNANO3 - & CNACL ! NA+ MOLAL(3)= WAER(3) - 2.D0*CNH42S4 - CNH4HS4 - CNH4CL - & 3.D0*CLC - CNH4NO3 ! NH4+ MOLAL(4)= WAER(5) - CNACL - CNH4CL - 2.D0*CCACL2 - & 2.D0*CMGCL2 - CKCL ! CL- MOLAL(7)= WAER(4) - CNANO3 - CNH4NO3 - CKNO3 & - 2.D0*CCANO32 - 2.D0*CMGNO32 ! NO3- MOLAL(6)= ONEMWF*(MOLAL(6) + DSOBIS + DAMBIS + DLC + DPOBIS) ! HSO4- MOLAL(5)= WAER(2) - MOLAL(6) - CLC - CNH42S4 - CNA2SO4 & - CCASO4 - CK2SO4 - CMGSO4 ! SO4-- MOLAL(8)= WAER(6) - CCASO4 - CCANO32 - CCACL2 ! CA++ MOLAL(9)= WAER(7) - 2.D0*CK2SO4 - CKNO3 - CKCL - CKHSO4 ! K+ MOLAL(10)=WAER(8) - CMGSO4 - CMGNO32 - CMGCL2 ! MG++ !C A8 = XK1*WATER/GAMA(7)*(GAMA(8)/GAMA(7))**2. IF (MOLAL(5).LE.TINY) THEN HIEQ = SQRT(XKW *RH*WATER*WATER) ! Neutral solution ELSE HIEQ = A8*MOLAL(6)/MOLAL(5) ENDIF HIEN = MOLAL(4) + MOLAL(7) + MOLAL(6) + 2.D0*MOLAL(5) - & MOLAL(2) - MOLAL(3) MOLAL(1)= MAX (HIEQ, HIEN) ! H+ !C !C *** GAS (ACTIVITY COEFS FROM LIQUID SOLUTION) !C A2 = (XK2/XKW)*R*TEMP*(GAMA(10)/GAMA(5))**2. ! NH3 <==> NH4+ A3 = XK4 *R*TEMP*(WATER/GAMA(10))**2. ! HNO3 <==> NO3- A4 = XK3 *R*TEMP*(WATER/GAMA(11))**2. ! HCL <==> CL- !C GNH3 = MOLAL(3)/MAX(MOLAL(1),TINY)/A2 GHNO3 = MOLAL(1)*MOLAL(7)/A3 GHCL = MOLAL(1)*MOLAL(4)/A4 !C 200 RETURN !C !C *** END OF SUBROUTINE CALCMDRPII ************************************** !C END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCHS4 !C *** THIS SUBROUTINE CALCULATES THE HSO4 GENERATED FROM (H,SO4). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCHS42p1 (HI, SO4I, HSO4I, DELTA) INCLUDE 'module_isrpia_inc.F' !CC CHARACTER ERRINF*40 !C !C *** IF TOO LITTLE WATER, DONT SOLVE !C IF (WATER.LE.1d1*TINY) THEN DELTA = ZERO RETURN ENDIF !C !C *** CALCULATE HSO4 SPECIATION ***************************************** !C A8 = XK1*WATER/GAMA(7)*(GAMA(8)/GAMA(7))**2. !C BB =-(HI + SO4I + A8) CC = HI*SO4I - HSO4I*A8 DD = BB*BB - 4.D0*CC !C IF (DD.GE.ZERO) THEN SQDD = SQRT(DD) DELTA1 = 0.5*(-BB + SQDD) DELTA2 = 0.5*(-BB - SQDD) IF (HSO4I.LE.TINY) THEN DELTA = DELTA2 ELSEIF( HI*SO4I .GE. A8*HSO4I ) THEN DELTA = DELTA2 ELSEIF( HI*SO4I .LT. A8*HSO4I ) THEN DELTA = DELTA1 ELSE DELTA = ZERO ENDIF ELSE DELTA = ZERO ENDIF !CCC !CCC *** COMPARE DELTA TO TOTAL H+ ; ESTIMATE EFFECT OF HSO4 *************** !CCC !CC HYD = MAX(HI, MOLAL(1)) !CC IF (HYD.GT.TINY) THEN !CC IF (DELTA/HYD.GT.0.1d0) THEN !CC WRITE (ERRINF,'(1PE10.3)') DELTA/HYD*100.0 !CC CALL PUSHERR (0020, ERRINF) !CC ENDIF !CC ENDIF !C RETURN !C !C *** END OF SUBROUTINE CALCHS4 ***************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCPH !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE CALCPH2p1 (GG, HI, OHI) INCLUDE 'module_isrpia_inc.F' !C AKW = XKW *RH*WATER*WATER CN = SQRT(AKW) !C !C *** GG = (negative charge) - (positive charge) !C IF (GG.GT.TINY) THEN ! H+ in excess BB =-GG CC =-AKW DD = BB*BB - 4.D0*CC HI = MAX(0.5D0*(-BB + SQRT(DD)),CN) OHI= AKW/HI ELSE ! OH- in excess BB = GG CC =-AKW DD = BB*BB - 4.D0*CC OHI= MAX(0.5D0*(-BB + SQRT(DD)),CN) HI = AKW/OHI ENDIF !C RETURN !C !C *** END OF SUBROUTINE CALCPH ****************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE II !C *** SUBROUTINE CALCACT !C *** CALCULATES MULTI-COMPONENT ACTIVITY COEFFICIENTS FROM BROMLEYS !C METHOD. THE BINARY ACTIVITY COEFFICIENTS ARE CALCULATED BY !C KUSIK-MEISNER RELATION (SUBROUTINE KMTAB or SUBROUTINE KMFUL). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCACT2p1 INCLUDE 'module_isrpia_inc.F' !C COMMON /DRVINP2p1/ WI(8), RHI, TEMPI, IPROBI, METSTBLI, IACALCI, & NADJI !C IF (W(1)+W(4)+W(5)+W(6)+W(7)+W(8) .LE. TINY) THEN !Ca,K,Mg,Na,Cl,NO3=0 CALL CALCACT12p1 ELSE IF (W(1)+W(5)+W(6)+W(7)+W(8) .LE. TINY) THEN !Ca,K,Mg,Na,Cl=0 CALL CALCACT22p1 ELSE IF (W(6)+W(7)+W(8) .LE. TINY) THEN !Ca,K,Mg=0 CALL CALCACT32p1 ELSE CALL CALCACT42p1 ENDIF !C !C *** Return point ; End of subroutine !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE II !C *** SUBROUTINE CALCACT4 !C *** CALCULATES MULTI-COMPONENT ACTIVITY COEFFICIENTS FROM BROMLEYS !C METHOD FOR AN AMMONIUM-SULFATE-NITRATE-CHLORIDE-SODIUM-CALCIUM-POTASSIUM-MAGNESIUM !C AEROSOL SYSTEM. THE BINARY ACTIVITY COEFFICIENTS ARE CALCULATED BY !C KUSIK-MEISNER RELATION (SUBROUTINE KMTAB or SUBROUTINE KMFUL4). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCACT42p1 INCLUDE 'module_isrpia_inc.F' !C REAL EX102p1 REAL G0(6,4),ZPL,ZMI,AGAMA,SION,H,CH,F1(6),F2A(4),F2B(4) DOUBLE PRECISION MPL, XIJ, YJI DATA G0/24*0D0/ !C GA(I,J)= (F1(I)/Z(I) + F2A(J)/Z(J+3)) / (Z(I)+Z(J+3)) - H GB(I,J)= (F1(I)/Z(I+4) + F2B(J)/Z(J+3)) / (Z(I+4)+Z(J+3)) - H !C !C *** SAVE ACTIVITIES IN OLD ARRAY ************************************* !C IF (FRST) THEN ! Outer loop DO 10 I=1,NPAIR GAMOU(I) = GAMA(I) 10 CONTINUE ENDIF !C DO 20 I=1,NPAIR ! Inner loop GAMIN(I) = GAMA(I) 20 CONTINUE !C !C *** CALCULATE IONIC ACTIVITY OF SOLUTION ***************************** !C IONIC=0.0 DO 30 I=1,NIONS IONIC=IONIC + MOLAL(I)*Z(I)*Z(I) 30 CONTINUE IONIC = MAX(MIN(0.5*IONIC/WATER,100.d0), TINY) !C !C *** CALCULATE BINARY ACTIVITY COEFFICIENTS *************************** !C !C G0(1,1)=G11;G0(1,2)=G07;G0(1,3)=G08;G0(1,4)=G10;G0(2,1)=G01;G0(2,2)=G02 !C G0(2,3)=G12;G0(2,4)=G03;G0(3,1)=G06;G0(3,2)=G04;G0(3,3)=G09;G0(3,4)=G05 !C IF (IACALC.EQ.0) THEN ! K.M.; FULL CALL KMFUL42p1 (IONIC, SNGL(TEMP),G0(2,1),G0(2,2),G0(2,4),& G0(3,2),G0(3,4),G0(3,1),G0(1,2),G0(1,3),G0(3,3),& G0(1,4),G0(1,1),G0(2,3),G0(4,4),G0(4,1),G0(5,2),& G0(5,3),G0(5,4),G0(5,1),G0(6,2),G0(6,4),G0(6,1)) ELSE ! K.M.; TABULATED CALL KMTAB2p1 (IONIC, SNGL(TEMP),G0(2,1),G0(2,2),G0(2,4), & G0(3,2),G0(3,4),G0(3,1),G0(1,2),G0(1,3),G0(3,3),& G0(1,4),G0(1,1),G0(2,3),G0(4,4),G0(4,1),G0(5,2),& G0(5,3),G0(5,4),G0(5,1),G0(6,2),G0(6,4),G0(6,1)) ENDIF !C !C *** CALCULATE MULTICOMPONENT ACTIVITY COEFFICIENTS ******************* !C AGAMA = 0.511*(298.0/TEMP)**1.5 ! Debye Huckel const. at T SION = SQRT(IONIC) H = AGAMA*SION/(1+SION) !C DO 100 I=1,4 F1(I)=0.0 F2A(I)=0.0 F2B(I)=0.0 100 CONTINUE F1(5)=0.0 F1(6)=0.0 !C DO 110 I=1,3 ZPL = Z(I) MPL = MOLAL(I)/WATER DO 110 J=1,4 ZMI = Z(J+3) CH = 0.25*(ZPL+ZMI)*(ZPL+ZMI)/IONIC XIJ = CH*MPL YJI = CH*MOLAL(J+3)/WATER F1(I) = F1(I) + SNGL(YJI*(G0(I,J) + ZPL*ZMI*H)) F2A(J) = F2A(J) + SNGL(XIJ*(G0(I,J) + ZPL*ZMI*H)) 110 CONTINUE !C DO 330 I=4,6 ZPL = Z(I+4) MPL = MOLAL(I+4)/WATER DO 330 J=1,4 ZMI = Z(J+3) IF (J.EQ.3) THEN IF (I.EQ.4 .OR. I.EQ.6) THEN GO TO 330 ENDIF ENDIF CH = 0.25*(ZPL+ZMI)*(ZPL+ZMI)/IONIC XIJ = CH*MPL YJI = CH*MOLAL(J+3)/WATER F1(I) = F1(I) + SNGL(YJI*(G0(I,J) + ZPL*ZMI*H)) F2B(J) = F2B(J) + SNGL(XIJ*(G0(I,J) + ZPL*ZMI*H)) 330 CONTINUE !C !C *** LOG10 OF ACTIVITY COEFFICIENTS *********************************** !C GAMA(01) = GA(2,1)*ZZ(01) ! NACL GAMA(02) = GA(2,2)*ZZ(02) ! NA2SO4 GAMA(03) = GA(2,4)*ZZ(03) ! NANO3 GAMA(04) = GA(3,2)*ZZ(04) ! (NH4)2SO4 GAMA(05) = GA(3,4)*ZZ(05) ! NH4NO3 GAMA(06) = GA(3,1)*ZZ(06) ! NH4CL GAMA(07) = GA(1,2)*ZZ(07) ! 2H-SO4 GAMA(08) = GA(1,3)*ZZ(08) ! H-HSO4 GAMA(09) = GA(3,3)*ZZ(09) ! NH4HSO4 GAMA(10) = GA(1,4)*ZZ(10) ! HNO3 GAMA(11) = GA(1,1)*ZZ(11) ! HCL GAMA(12) = GA(2,3)*ZZ(12) ! NAHSO4 GAMA(13) = 0.20*(3.0*GAMA(04)+2.0*GAMA(09)) ! LC ; SCAPE !CC GAMA(13) = 0.50*(GAMA(04)+GAMA(09)) ! LC ; SEQUILIB !CC GAMA(13) = 0.25*(3.0*GAMA(04)+GAMA(07)) ! LC ; AIM GAMA(14) = 0.0d0 ! CASO4 GAMA(15) = GB(4,4)*ZZ(15) ! CA(NO3)2 GAMA(16) = GB(4,1)*ZZ(16) ! CACL2 GAMA(17) = GB(5,2)*ZZ(17) ! K2SO4 GAMA(18) = GB(5,3)*ZZ(18) ! KHSO4 GAMA(19) = GB(5,4)*ZZ(19) ! KNO3 GAMA(20) = GB(5,1)*ZZ(20) ! KCL GAMA(21) = GB(6,2)*ZZ(21) ! MGSO4 GAMA(22) = GB(6,4)*ZZ(22) ! MG(NO3)2 GAMA(23) = GB(6,1)*ZZ(23) ! MGCL2 !C !C *** CONVERT LOG (GAMA) COEFFICIENTS TO GAMA ************************** !C DO 200 I=1,NPAIR GAMA(I)=MAX(-5.0d0, MIN(GAMA(I),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(I)=10.0**GAMA(I) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] 200 CONTINUE !C !C *** SETUP ACTIVITY CALCULATION FLAGS ******************************** !C !C OUTER CALCULATION LOOP ; ONLY IF FRST=.TRUE. !C IF (FRST) THEN ERROU = ZERO ! CONVERGENCE CRITERION DO 210 I=1,NPAIR ERROU=MAX(ERROU, ABS((GAMOU(I)-GAMA(I))/GAMOU(I))) 210 CONTINUE CALAOU = ERROU .GE. EPSACT ! SETUP FLAGS FRST =.FALSE. ENDIF !C !C INNER CALCULATION LOOP ; ALWAYS !C ERRIN = ZERO ! CONVERGENCE CRITERION DO 220 I=1,NPAIR ERRIN = MAX (ERRIN, ABS((GAMIN(I)-GAMA(I))/GAMIN(I))) 220 CONTINUE CALAIN = ERRIN .GE. EPSACT !C ICLACT = ICLACT + 1 ! Increment ACTIVITY call counter !C !C *** END OF SUBROUTINE ACTIVITY **************************************** !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCACT3 !C *** CALCULATES MULTI-COMPONENT ACTIVITY COEFFICIENTS FROM BROMLEYS !C METHOD FOR AN AMMONIUM-SULFATE-NITRATE-CHLORIDE-SODIUM AEROSOL SYSTEM. !C THE BINARY ACTIVITY COEFFICIENTS ARE CALCULATED BY !C KUSIK-MEISNER RELATION (SUBROUTINE KMTAB or SUBROUTINE KMFUL3). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCACT32p1 INCLUDE 'module_isrpia_inc.F' !C REAL EX102p1, URF REAL G0(6,4),ZPL,ZMI,AGAMA,SION,H,CH,F1(3),F2(4) DOUBLE PRECISION MPL, XIJ, YJI PARAMETER (URF=0.5) !C PARAMETER (LN10=2.30258509299404568402D0) !C G(I,J)= (F1(I)/Z(I) + F2(J)/Z(J+3)) / (Z(I)+Z(J+3)) - H !C !C *** SAVE ACTIVITIES IN OLD ARRAY ************************************* !C IF (FRST) THEN ! Outer loop DO 10 I=1,13 GAMOU(I) = GAMA(I) 10 CONTINUE ENDIF !C DO 20 I=1,13 ! Inner loop GAMIN(I) = GAMA(I) 20 CONTINUE !C !C *** CALCULATE IONIC ACTIVITY OF SOLUTION ***************************** !C IONIC=0.0 DO 30 I=1,7 IONIC=IONIC + MOLAL(I)*Z(I)*Z(I) 30 CONTINUE IONIC = MAX(MIN(0.5*IONIC/WATER,100.d0), TINY) !C !C *** CALCULATE BINARY ACTIVITY COEFFICIENTS *************************** !C !C G0(1,1)=G11;G0(1,2)=G07;G0(1,3)=G08;G0(1,4)=G10;G0(2,1)=G01;G0(2,2)=G02 !C G0(2,3)=G12;G0(2,4)=G03;G0(3,1)=G06;G0(3,2)=G04;G0(3,3)=G09;G0(3,4)=G05 !C IF (IACALC.EQ.0) THEN ! K.M.; FULL CALL KMFUL32p1 (IONIC, SNGL(TEMP),G0(2,1),G0(2,2),G0(2,4), & G0(3,2),G0(3,4),G0(3,1),G0(1,2),G0(1,3),G0(3,3),& G0(1,4),G0(1,1),G0(2,3)) ELSE ! K.M.; TABULATED CALL KMTAB2p1 (IONIC, SNGL(TEMP),G0(2,1),G0(2,2),G0(2,4),& G0(3,2),G0(3,4),G0(3,1),G0(1,2),G0(1,3),G0(3,3),& G0(1,4),G0(1,1),G0(2,3),G0(4,4),G0(4,1),G0(5,2),& G0(5,3),G0(5,4),G0(5,1),G0(6,2),G0(6,4),G0(6,1)) ENDIF !C !C *** CALCULATE MULTICOMPONENT ACTIVITY COEFFICIENTS ******************* !C AGAMA = 0.511*(298.0/TEMP)**1.5 ! Debye Huckel const. at T SION = SQRT(IONIC) H = AGAMA*SION/(1+SION) !C DO 100 I=1,3 F1(I)=0.0 F2(I)=0.0 100 CONTINUE F2(4)=0.0 !C DO 110 I=1,3 ZPL = Z(I) MPL = MOLAL(I)/WATER DO 110 J=1,4 ZMI = Z(J+3) CH = 0.25*(ZPL+ZMI)*(ZPL+ZMI)/IONIC XIJ = CH*MPL YJI = CH*MOLAL(J+3)/WATER F1(I) = F1(I) + SNGL(YJI*(G0(I,J) + ZPL*ZMI*H)) F2(J) = F2(J) + SNGL(XIJ*(G0(I,J) + ZPL*ZMI*H)) 110 CONTINUE !C !C *** LOG10 OF ACTIVITY COEFFICIENTS *********************************** !C GAMA(01) = G(2,1)*ZZ(01) ! NACL GAMA(02) = G(2,2)*ZZ(02) ! NA2SO4 GAMA(03) = G(2,4)*ZZ(03) ! NANO3 GAMA(04) = G(3,2)*ZZ(04) ! (NH4)2SO4 GAMA(05) = G(3,4)*ZZ(05) ! NH4NO3 GAMA(06) = G(3,1)*ZZ(06) ! NH4CL GAMA(07) = G(1,2)*ZZ(07) ! 2H-SO4 GAMA(08) = G(1,3)*ZZ(08) ! H-HSO4 GAMA(09) = G(3,3)*ZZ(09) ! NH4HSO4 GAMA(10) = G(1,4)*ZZ(10) ! HNO3 GAMA(11) = G(1,1)*ZZ(11) ! HCL GAMA(12) = G(2,3)*ZZ(12) ! NAHSO4 GAMA(13) = 0.20*(3.0*GAMA(04)+2.0*GAMA(09)) ! LC ; SCAPE !CC GAMA(13) = 0.50*(GAMA(04)+GAMA(09)) ! LC ; SEQUILIB !CC GAMA(13) = 0.25*(3.0*GAMA(04)+GAMA(07)) ! LC ; AIM !C !C *** CONVERT LOG (GAMA) COEFFICIENTS TO GAMA ************************** !C DO 200 I=1,13 GAMA(I)=MAX(-5.0d0, MIN(GAMA(I),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(I)=10.0**GAMA(I) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(I) = GAMIN(I)*(1.0-URF) + URF*GAMA(I) ! Under-relax GAMA's 200 CONTINUE !C !C *** SETUP ACTIVITY CALCULATION FLAGS ********************************* !C !C OUTER CALCULATION LOOP ; ONLY IF FRST=.TRUE. !C IF (FRST) THEN ERROU = ZERO ! CONVERGENCE CRITERION DO 210 I=1,13 ERROU=MAX(ERROU, ABS((GAMOU(I)-GAMA(I))/GAMOU(I))) 210 CONTINUE CALAOU = ERROU .GE. EPSACT ! SETUP FLAGS FRST =.FALSE. ENDIF !C !C INNER CALCULATION LOOP ; ALWAYS !C ERRIN = ZERO ! CONVERGENCE CRITERION DO 220 I=1,13 ERRIN = MAX (ERRIN, ABS((GAMIN(I)-GAMA(I))/GAMIN(I))) 220 CONTINUE CALAIN = ERRIN .GE. EPSACT !C ICLACT = ICLACT + 1 ! Increment ACTIVITY call counter !C !C *** END OF SUBROUTINE ACTIVITY **************************************** !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCACT2 !C *** CALCULATES MULTI-COMPONENT ACTIVITY COEFFICIENTS FROM BROMLEYS !C METHOD FOR AN AMMONIUM-SULFATE-NITRATE AEROSOL SYSTEM. !C THE BINARY ACTIVITY COEFFICIENTS ARE CALCULATED BY !C KUSIK-MEISNER RELATION (SUBROUTINE KMTAB or SUBROUTINE KMFUL2). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCACT22p1 INCLUDE 'module_isrpia_inc.F' !C REAL EX102p1, URF REAL G0(6,4),ZPL,ZMI,AGAMA,SION,H,CH,F1(3),F2(4) DOUBLE PRECISION MPL, XIJ, YJI PARAMETER (URF=0.5) !C PARAMETER (LN10=2.30258509299404568402D0) !C G(I,J)= (F1(I)/Z(I) + F2(J)/Z(J+3)) / (Z(I)+Z(J+3)) - H !C !C *** SAVE ACTIVITIES IN OLD ARRAY ************************************* !C IF (FRST) THEN ! Outer loop DO 10 I=7,10 GAMOU(I) = GAMA(I) 10 CONTINUE GAMOU(4) = GAMA(4) GAMOU(5) = GAMA(5) GAMOU(13) = GAMA(13) ENDIF !C DO 20 I=7,10 ! Inner loop GAMIN(I) = GAMA(I) 20 CONTINUE GAMIN(4) = GAMA(4) GAMIN(5) = GAMA(5) GAMIN(13) = GAMA(13) !C !C *** CALCULATE IONIC ACTIVITY OF SOLUTION ***************************** !C IONIC=0.0 MOLAL(2) = ZERO MOLAL(4) = ZERO DO 30 I=1,7 IONIC=IONIC + MOLAL(I)*Z(I)*Z(I) 30 CONTINUE IONIC = MAX(MIN(0.5*IONIC/WATER,100.d0), TINY) !C !C *** CALCULATE BINARY ACTIVITY COEFFICIENTS *************************** !C !C G0(1,1)=G11;G0(1,2)=G07;G0(1,3)=G08;G0(1,4)=G10;G0(2,1)=G01;G0(2,2)=G02 !C G0(2,3)=G12;G0(2,4)=G03;G0(3,1)=G06;G0(3,2)=G04;G0(3,3)=G09;G0(3,4)=G05 !C IF (IACALC.EQ.0) THEN ! K.M.; FULL CALL KMFUL22p1 (IONIC, SNGL(TEMP),G0(3,2),G0(3,4),G0(1,2), & G0(1,3),G0(3,3),G0(1,4)) ELSE ! K.M.; TABULATED CALL KMTAB2p1 (IONIC, SNGL(TEMP),G0(2,1),G0(2,2),G0(2,4),& G0(3,2),G0(3,4),G0(3,1),G0(1,2),G0(1,3),G0(3,3),& G0(1,4),G0(1,1),G0(2,3),G0(4,4),G0(4,1),G0(5,2),& G0(5,3),G0(5,4),G0(5,1),G0(6,2),G0(6,4),G0(6,1)) ENDIF !C !C *** CALCULATE MULTICOMPONENT ACTIVITY COEFFICIENTS ******************* !C AGAMA = 0.511*(298.0/TEMP)**1.5 ! Debye Huckel const. at T SION = SQRT(IONIC) H = AGAMA*SION/(1+SION) !C DO 100 I=1,3 F1(I)=0.0 F2(I)=0.0 100 CONTINUE F2(4)=0.0 !C DO 110 I=1,3,2 ZPL = Z(I) MPL = MOLAL(I)/WATER DO 110 J=2,4 ZMI = Z(J+3) CH = 0.25*(ZPL+ZMI)*(ZPL+ZMI)/IONIC XIJ = CH*MPL YJI = CH*MOLAL(J+3)/WATER F1(I) = F1(I) + SNGL(YJI*(G0(I,J) + ZPL*ZMI*H)) F2(J) = F2(J) + SNGL(XIJ*(G0(I,J) + ZPL*ZMI*H)) 110 CONTINUE !C !C *** LOG10 OF ACTIVITY COEFFICIENTS *********************************** !C !C GAMA(01) = G(2,1)*ZZ(01) ! NACL !C GAMA(02) = G(2,2)*ZZ(02) ! NA2SO4 !C GAMA(03) = G(2,4)*ZZ(03) ! NANO3 GAMA(04) = G(3,2)*ZZ(04) ! (NH4)2SO4 GAMA(05) = G(3,4)*ZZ(05) ! NH4NO3 !C GAMA(06) = G(3,1)*ZZ(06) ! NH4CL GAMA(07) = G(1,2)*ZZ(07) ! 2H-SO4 GAMA(08) = G(1,3)*ZZ(08) ! H-HSO4 GAMA(09) = G(3,3)*ZZ(09) ! NH4HSO4 GAMA(10) = G(1,4)*ZZ(10) ! HNO3 !C GAMA(11) = G(1,1)*ZZ(11) ! HCL !C GAMA(12) = G(2,3)*ZZ(12) ! NAHSO4 GAMA(13) = 0.20*(3.0*GAMA(04)+2.0*GAMA(09)) ! LC ; SCAPE !CC GAMA(13) = 0.50*(GAMA(04)+GAMA(09)) ! LC ; SEQUILIB !CC GAMA(13) = 0.25*(3.0*GAMA(04)+GAMA(07)) ! LC ; AIM !C !C *** CONVERT LOG (GAMA) COEFFICIENTS TO GAMA ************************** !C DO 200 I=7,10 GAMA(I)=MAX(-5.0d0, MIN(GAMA(I),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(I)=10.0**GAMA(I) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(I) = GAMIN(I)*(1.0-URF) + URF*GAMA(I) ! Under-relax GAMA's 200 CONTINUE !C GAMA(4)=MAX(-5.0d0, MIN(GAMA(4),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(4)=10.0**GAMA(4) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(4) = GAMIN(4)*(1.0-URF) + URF*GAMA(4) ! Under-relax GAMA's !C GAMA(5)=MAX(-5.0d0, MIN(GAMA(5),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(5)=10.0**GAMA(5) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(5) = GAMIN(5)*(1.0-URF) + URF*GAMA(I) ! Under-relax GAMA's !C GAMA(13)=MAX(-5.0d0, MIN(GAMA(13),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(13)=10.0**GAMA(13) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(13) = GAMIN(13)*(1.0-URF) + URF*GAMA(13) ! Under-relax GAMA's !C !C *** SETUP ACTIVITY CALCULATION FLAGS ********************************* !C !C OUTER CALCULATION LOOP ; ONLY IF FRST=.TRUE. !C IF (FRST) THEN ERROU = ZERO ! CONVERGENCE CRITERION DO 210 I=7,10 ERROU=MAX(ERROU, ABS((GAMOU(I)-GAMA(I))/GAMOU(I))) 210 CONTINUE ERROU=MAX(ERROU, ABS((GAMOU(4)-GAMA(4))/GAMOU(4))) ERROU=MAX(ERROU, ABS((GAMOU(5)-GAMA(5))/GAMOU(5))) ERROU=MAX(ERROU, ABS((GAMOU(13)-GAMA(13))/GAMOU(13))) !C CALAOU = ERROU .GE. EPSACT ! SETUP FLAGS FRST =.FALSE. ENDIF !C !C INNER CALCULATION LOOP ; ALWAYS !C ERRIN = ZERO ! CONVERGENCE CRITERION DO 220 I=7,10 ERRIN = MAX (ERRIN, ABS((GAMIN(I)-GAMA(I))/GAMIN(I))) 220 CONTINUE ERRIN = MAX (ERRIN, ABS((GAMIN(4)-GAMA(4))/GAMIN(4))) ERRIN = MAX (ERRIN, ABS((GAMIN(5)-GAMA(5))/GAMIN(5))) ERRIN = MAX (ERRIN, ABS((GAMIN(13)-GAMA(13))/GAMIN(13))) CALAIN = ERRIN .GE. EPSACT !C ICLACT = ICLACT + 1 ! Increment ACTIVITY call counter !C !C *** END OF SUBROUTINE ACTIVITY **************************************** !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE CALCACT1 !C *** CALCULATES MULTI-COMPONENT ACTIVITY COEFFICIENTS FROM BROMLEYS !C METHOD FOR AN AMMONIUM-SULFATE AEROSOL SYSTEM. !C THE BINARY ACTIVITY COEFFICIENTS ARE CALCULATED BY !C KUSIK-MEISNER RELATION (SUBROUTINE KMTAB or SUBROUTINE KMFUL1). !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE CALCACT12p1 INCLUDE 'module_isrpia_inc.F' !C REAL EX102p1, URF REAL G0(6,4),ZPL,ZMI,AGAMA,SION,H,CH,F1(3),F2(4) DOUBLE PRECISION MPL, XIJ, YJI PARAMETER (URF=0.5) !C PARAMETER (LN10=2.30258509299404568402D0) !C G(I,J)= (F1(I)/Z(I) + F2(J)/Z(J+3)) / (Z(I)+Z(J+3)) - H !C !C *** SAVE ACTIVITIES IN OLD ARRAY ************************************* !C IF (FRST) THEN ! Outer loop DO 10 I=7,9 GAMOU(I) = GAMA(I) 10 CONTINUE GAMOU(4) = GAMA(4) !C GAMOU(5) = GAMA(5) GAMOU(13) = GAMA(13) ENDIF !C DO 20 I=7,9 ! Inner loop GAMIN(I) = GAMA(I) 20 CONTINUE GAMIN(4) = GAMA(4) !C GAMIN(5) = GAMA(5) GAMIN(13) = GAMA(13) !C !C *** CALCULATE IONIC ACTIVITY OF SOLUTION ***************************** !C IONIC=0.0 MOLAL(2) = ZERO MOLAL(4) = ZERO MOLAL(7) = ZERO DO 30 I=1,7 IONIC=IONIC + MOLAL(I)*Z(I)*Z(I) 30 CONTINUE IONIC = MAX(MIN(0.5*IONIC/WATER,100.d0), TINY) !C !C *** CALCULATE BINARY ACTIVITY COEFFICIENTS *************************** !C !C G0(1,1)=G11;G0(1,2)=G07;G0(1,3)=G08;G0(1,4)=G10;G0(2,1)=G01;G0(2,2)=G02 !C G0(2,3)=G12;G0(2,4)=G03;G0(3,1)=G06;G0(3,2)=G04;G0(3,3)=G09;G0(3,4)=G05 !C IF (IACALC.EQ.0) THEN ! K.M.; FULL CALL KMFUL12p1 (IONIC, SNGL(TEMP),G0(3,2),G0(1,2),& G0(1,3),G0(3,3)) ELSE ! K.M.; TABULATED CALL KMTAB2p1 (IONIC, SNGL(TEMP),G0(2,1),G0(2,2),G0(2,4),& G0(3,2),G0(3,4),G0(3,1),G0(1,2),G0(1,3),G0(3,3),& G0(1,4),G0(1,1),G0(2,3),G0(4,4),G0(4,1),G0(5,2),& G0(5,3),G0(5,4),G0(5,1),G0(6,2),G0(6,4),G0(6,1)) ENDIF !C !C *** CALCULATE MULTICOMPONENT ACTIVITY COEFFICIENTS ******************* !C AGAMA = 0.511*(298.0/TEMP)**1.5 ! Debye Huckel const. at T SION = SQRT(IONIC) H = AGAMA*SION/(1+SION) !C DO 100 I=1,3 F1(I)=0.0 F2(I)=0.0 100 CONTINUE F2(4)=0.0 !C DO 110 I=1,3,2 ZPL = Z(I) MPL = MOLAL(I)/WATER DO 110 J=2,3 ZMI = Z(J+3) CH = 0.25*(ZPL+ZMI)*(ZPL+ZMI)/IONIC XIJ = CH*MPL YJI = CH*MOLAL(J+3)/WATER F1(I) = F1(I) + SNGL(YJI*(G0(I,J) + ZPL*ZMI*H)) F2(J) = F2(J) + SNGL(XIJ*(G0(I,J) + ZPL*ZMI*H)) 110 CONTINUE !C !C *** LOG10 OF ACTIVITY COEFFICIENTS *********************************** !C !C GAMA(01) = G(2,1)*ZZ(01) ! NACL !C GAMA(02) = G(2,2)*ZZ(02) ! NA2SO4 !C GAMA(03) = G(2,4)*ZZ(03) ! NANO3 GAMA(04) = G(3,2)*ZZ(04) ! (NH4)2SO4 !C GAMA(05) = G(3,4)*ZZ(05) ! NH4NO3 !C GAMA(06) = G(3,1)*ZZ(06) ! NH4CL GAMA(07) = G(1,2)*ZZ(07) ! 2H-SO4 GAMA(08) = G(1,3)*ZZ(08) ! H-HSO4 GAMA(09) = 0.5*(GAMA(04)+GAMA(07)) ! NH4HSO4 ; AIM (Wexler & Seinfeld, 1991) !C GAMA(10) = G(1,4)*ZZ(10) ! HNO3 !C GAMA(11) = G(1,1)*ZZ(11) ! HCL !C GAMA(12) = G(2,3)*ZZ(12) ! NAHSO4 GAMA(13) = 0.20*(3.0*GAMA(04)+2.0*GAMA(09)) ! LC ; SCAPE !CC GAMA(13) = 0.50*(GAMA(04)+GAMA(09)) ! LC ; SEQUILIB !CC GAMA(13) = 0.25*(3.0*GAMA(04)+GAMA(07)) ! LC ; AIM !C !C *** CONVERT LOG (GAMA) COEFFICIENTS TO GAMA ************************** !C DO 200 I=7,9 GAMA(I)=MAX(-5.0d0, MIN(GAMA(I),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(I)=10.0**GAMA(I) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(I) = GAMIN(I)*(1.0-URF) + URF*GAMA(I) ! Under-relax GAMA's 200 CONTINUE !C GAMA(4)=MAX(-5.0d0, MIN(GAMA(4),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(4)=10.0**GAMA(4) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(4) = GAMIN(4)*(1.0-URF) + URF*GAMA(4) ! Under-relax GAMA's !C !C GAMA(5)=MAX(-5.0d0, MIN(GAMA(5),5.0d0) ) ! F77 LIBRARY ROUTINE !C GAMA(5)=10.0**GAMA(5) !CC GAMA(I)=EXP(LN10*GAMA(I)) !CCC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(5) = GAMIN(5)*(1.0-URF) + URF*GAMA(I) ! Under-relax GAMA's !C GAMA(13)=MAX(-5.0d0, MIN(GAMA(13),5.0d0) ) ! F77 LIBRARY ROUTINE GAMA(13)=10.0**GAMA(13) !C GAMA(I)=EXP(LN10*GAMA(I)) !CC GAMA(I)=EX10(SNGL(GAMA(I)), 5.0) ! CUTOFF SET TO [-5,5] !C GAMA(13) = GAMIN(13)*(1.0-URF) + URF*GAMA(13) ! Under-relax GAMA's !C !C *** SETUP ACTIVITY CALCULATION FLAGS ********************************* !C !C OUTER CALCULATION LOOP ; ONLY IF FRST=.TRUE. !C IF (FRST) THEN ERROU = ZERO ! CONVERGENCE CRITERION DO 210 I=7,9 ERROU=MAX(ERROU, ABS((GAMOU(I)-GAMA(I))/GAMOU(I))) 210 CONTINUE ERROU=MAX(ERROU, ABS((GAMOU(4)-GAMA(4))/GAMOU(4))) !C ERROU=MAX(ERROU, ABS((GAMOU(5)-GAMA(5))/GAMOU(5))) ERROU=MAX(ERROU, ABS((GAMOU(13)-GAMA(13))/GAMOU(13))) !C CALAOU = ERROU .GE. EPSACT ! SETUP FLAGS FRST =.FALSE. ENDIF !C !C INNER CALCULATION LOOP ; ALWAYS !C ERRIN = ZERO ! CONVERGENCE CRITERION DO 220 I=7,9 ERRIN = MAX (ERRIN, ABS((GAMIN(I)-GAMA(I))/GAMIN(I))) 220 CONTINUE ERRIN = MAX (ERRIN, ABS((GAMIN(4)-GAMA(4))/GAMIN(4))) !C ERRIN = MAX (ERRIN, ABS((GAMIN(5)-GAMA(5))/GAMIN(5))) ERRIN = MAX (ERRIN, ABS((GAMIN(13)-GAMA(13))/GAMIN(13))) CALAIN = ERRIN .GE. EPSACT !C ICLACT = ICLACT + 1 ! Increment ACTIVITY call counter !C !C *** END OF SUBROUTINE ACTIVITY **************************************** !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE RSTGAM !C *** RESETS ACTIVITY COEFFICIENT ARRAYS TO DEFAULT VALUE OF 0.1 !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE RSTGAM2p1 INCLUDE 'module_isrpia_inc.F' !C DO 10 I=1, NPAIR GAMA(I) = 0.1 10 CONTINUE !C !C *** END OF SUBROUTINE RSTGAM ****************************************** !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE II !C *** SUBROUTINE KMFUL4 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD !C FOR AN AMMONIUM-SULFATE-NITRATE-CHLORIDE-SODIUM-CALCIUM-POTASSIUM-MAGNESIUM !C AEROSOL SYSTEM. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE KMFUL42p1 (IONIC,TEMP,G01,G02,G03,G04,G05,G06,G07,G08,G09,& G10,G11,G12,G15,G16,G17,G18,G19,G20,& G21,G22,G23) REAL Ionic, TEMP DATA Z01,Z02,Z03,Z04,Z05,Z06,Z07,Z08,Z10,Z11,Z15,Z16,Z17,Z19,Z20,& Z21,Z22,Z23/1, 2, 1, 2, 1, 1, 2, 1, 1, 1, 2, 2, 2, 1, 1, 4,& 2, 2/ !C SION = SQRT(IONIC) !C !C *** Coefficients at 25 oC !C CALL MKBI2p1(2.230, IONIC, SION, Z01, G01) CALL MKBI2p1(-0.19, IONIC, SION, Z02, G02) CALL MKBI2p1(-0.39, IONIC, SION, Z03, G03) CALL MKBI2p1(-0.25, IONIC, SION, Z04, G04) CALL MKBI2p1(-1.15, IONIC, SION, Z05, G05) CALL MKBI2p1(0.820, IONIC, SION, Z06, G06) CALL MKBI2p1(-.100, IONIC, SION, Z07, G07) CALL MKBI2p1(8.000, IONIC, SION, Z08, G08) CALL MKBI2p1(2.600, IONIC, SION, Z10, G10) CALL MKBI2p1(6.000, IONIC, SION, Z11, G11) CALL MKBI2p1(0.930, IONIC, SION, Z15, G15) CALL MKBI2p1(2.400, IONIC, SION, Z16, G16) CALL MKBI2p1(-0.25, IONIC, SION, Z17, G17) CALL MKBI2p1(-2.33, IONIC, SION, Z19, G19) CALL MKBI2p1(0.920, IONIC, SION, Z20, G20) CALL MKBI2p1(0.150, IONIC, SION, Z21, G21) CALL MKBI2p1(2.320, IONIC, SION, Z22, G22) CALL MKBI2p1(2.900, IONIC, SION, Z23, G23) !C !C *** Correct for T other than 298 K !C TI = TEMP-273.0 TC = TI-25.0 IF (ABS(TC) .GT. 1.0) THEN CF1 = 1.125-0.005*TI CF2 = (0.125-0.005*TI)*(0.039*IONIC**0.92-0.41*SION/(1.+SION)) G01 = CF1*G01 - CF2*Z01 G02 = CF1*G02 - CF2*Z02 G03 = CF1*G03 - CF2*Z03 G04 = CF1*G04 - CF2*Z04 G05 = CF1*G05 - CF2*Z05 G06 = CF1*G06 - CF2*Z06 G07 = CF1*G07 - CF2*Z07 G08 = CF1*G08 - CF2*Z08 G10 = CF1*G10 - CF2*Z10 G11 = CF1*G11 - CF2*Z11 G15 = CF1*G15 - CF2*Z15 G16 = CF1*G16 - CF2*Z16 G17 = CF1*G17 - CF2*Z17 G19 = CF1*G19 - CF2*Z19 G20 = CF1*G20 - CF2*Z20 G21 = CF1*G21 - CF2*Z21 G22 = CF1*G22 - CF2*Z22 G23 = CF1*G23 - CF2*Z23 ENDIF !C G09 = G06 + G08 - G11 G12 = G01 + G08 - G11 G18 = G08 + G20 - G11 !C !C *** Return point ; End of subroutine !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KMFUL3 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD !C FOR AN AMMONIUM-SULFATE-NITRATE-CHLORIDE-SODIUM AEROSOL SYSTEM. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE KMFUL32p1 (IONIC,TEMP,G01,G02,G03,G04,G05,G06,G07,G08,G09,& G10,G11,G12) REAL Ionic, TEMP DATA Z01,Z02,Z03,Z04,Z05,Z06,Z07,Z08,Z10,Z11 & /1, 2, 1, 2, 1, 1, 2, 1, 1, 1/ !C SION = SQRT(IONIC) !C !C *** Coefficients at 25 oC !C CALL MKBI2p1(2.230, IONIC, SION, Z01, G01) CALL MKBI2p1(-0.19, IONIC, SION, Z02, G02) CALL MKBI2p1(-0.39, IONIC, SION, Z03, G03) CALL MKBI2p1(-0.25, IONIC, SION, Z04, G04) CALL MKBI2p1(-1.15, IONIC, SION, Z05, G05) CALL MKBI2p1(0.820, IONIC, SION, Z06, G06) CALL MKBI2p1(-.100, IONIC, SION, Z07, G07) CALL MKBI2p1(8.000, IONIC, SION, Z08, G08) CALL MKBI2p1(2.600, IONIC, SION, Z10, G10) CALL MKBI2p1(6.000, IONIC, SION, Z11, G11) !C !C *** Correct for T other than 298 K !C TI = TEMP-273.0 TC = TI-25.0 IF (ABS(TC) .GT. 1.0) THEN CF1 = 1.125-0.005*TI CF2 = (0.125-0.005*TI)*(0.039*IONIC**0.92-0.41*SION/(1.+SION)) G01 = CF1*G01 - CF2*Z01 G02 = CF1*G02 - CF2*Z02 G03 = CF1*G03 - CF2*Z03 G04 = CF1*G04 - CF2*Z04 G05 = CF1*G05 - CF2*Z05 G06 = CF1*G06 - CF2*Z06 G07 = CF1*G07 - CF2*Z07 G08 = CF1*G08 - CF2*Z08 G10 = CF1*G10 - CF2*Z10 G11 = CF1*G11 - CF2*Z11 ENDIF !C G09 = G06 + G08 - G11 G12 = G01 + G08 - G11 !C !C *** Return point ; End of subroutine !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KMFUL2 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD !C FOR AN AMMONIUM-SULFATE-NITRATE AEROSOL SYSTEM. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE KMFUL22p1 (IONIC,TEMP,G04,G05,G07,G08,G09,G10) REAL Ionic, TEMP DATA Z01,Z02,Z03,Z04,Z05,Z06,Z07,Z08,Z10,Z11 & /1, 2, 1, 2, 1, 1, 2, 1, 1, 1/ !C SION = SQRT(IONIC) !C !C *** Coefficients at 25 oC !C !C CALL MKBI(2.230, IONIC, SION, Z01, G01) !C CALL MKBI(-0.19, IONIC, SION, Z02, G02) !C CALL MKBI(-0.39, IONIC, SION, Z03, G03) CALL MKBI2p1(-0.25, IONIC, SION, Z04, G04) CALL MKBI2p1(-1.15, IONIC, SION, Z05, G05) !C CALL MKBI(0.820, IONIC, SION, Z06, G06) CALL MKBI2p1(-.100, IONIC, SION, Z07, G07) CALL MKBI2p1(8.000, IONIC, SION, Z08, G08) CALL MKBI2p1(2.600, IONIC, SION, Z10, G10) !C CALL MKBI(6.000, IONIC, SION, Z11, G11) !C !C *** Correct for T other than 298 K !C TI = TEMP-273.0 TC = TI-25.0 IF (ABS(TC) .GT. 1.0) THEN CF1 = 1.125-0.005*TI CF2 = (0.125-0.005*TI)*(0.039*IONIC**0.92-0.41*SION/(1.+SION)) !C G01 = CF1*G01 - CF2*Z01 !C G02 = CF1*G02 - CF2*Z02 !C G03 = CF1*G03 - CF2*Z03 G04 = CF1*G04 - CF2*Z04 G05 = CF1*G05 - CF2*Z05 !C G06 = CF1*G06 - CF2*Z06 G07 = CF1*G07 - CF2*Z07 G08 = CF1*G08 - CF2*Z08 G10 = CF1*G10 - CF2*Z10 !C G11 = CF1*G11 - CF2*Z11 ENDIF !C G09 = G05 + G08 - G10 !C G12 = G01 + G08 - G11 !C !C *** Return point ; End of subroutine !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KMFUL1 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD !C FOR AN AMMONIUM-SULFATE AEROSOL SYSTEM. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C !C *** WRITTEN BY CHRISTOS FOUNTOUKIS & ATHANASIOS NENES !C !C======================================================================= !C SUBROUTINE KMFUL12p1 (IONIC,TEMP,G04,G07,G08,G09) REAL Ionic, TEMP DATA Z01,Z02,Z03,Z04,Z05,Z06,Z07,Z08,Z10,Z11 & /1, 2, 1, 2, 1, 1, 2, 1, 1, 1/ !C SION = SQRT(IONIC) !C !C *** Coefficients at 25 oC !C !C CALL MKBI(2.230, IONIC, SION, Z01, G01) !C CALL MKBI(-0.19, IONIC, SION, Z02, G02) !C CALL MKBI(-0.39, IONIC, SION, Z03, G03) CALL MKBI2p1(-0.25, IONIC, SION, Z04, G04) !C CALL MKBI(-1.15, IONIC, SION, Z05, G05) !C CALL MKBI(0.820, IONIC, SION, Z06, G06) CALL MKBI2p1(-.100, IONIC, SION, Z07, G07) CALL MKBI2p1(8.000, IONIC, SION, Z08, G08) !C CALL MKBI(2.600, IONIC, SION, Z10, G10) !C CALL MKBI(6.000, IONIC, SION, Z11, G11) !C !C *** Correct for T other than 298 K !C TI = TEMP-273.0 TC = TI-25.0 IF (ABS(TC) .GT. 1.0) THEN CF1 = 1.125-0.005*TI CF2 = (0.125-0.005*TI)*(0.039*IONIC**0.92-0.41*SION/(1.+SION)) !C G01 = CF1*G01 - CF2*Z01 !C G02 = CF1*G02 - CF2*Z02 !C G03 = CF1*G03 - CF2*Z03 G04 = CF1*G04 - CF2*Z04 !C G05 = CF1*G05 - CF2*Z05 !C G06 = CF1*G06 - CF2*Z06 G07 = CF1*G07 - CF2*Z07 G08 = CF1*G08 - CF2*Z08 !C G10 = CF1*G10 - CF2*Z10 !C G11 = CF1*G11 - CF2*Z11 ENDIF !C !C G09 = G05 + G08 - G10 ! CALCULATED IN CALCACT1 !C G12 = G01 + G08 - G11 !C !C *** Return point ; End of subroutine !C RETURN END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE MKBI !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE MKBI2p1(Q,IONIC,SION,ZIP,BI) !C REAL IONIC !C B=.75-.065*Q C= 1.0 IF (IONIC.LT.6.0) C=1.+.055*Q*EXP(-.023*IONIC*IONIC*IONIC) XX=-0.5107*SION/(1.+C*SION) BI=(1.+B*(1.+.1*IONIC)**Q-B) BI=ZIP*ALOG10(BI) + ZIP*XX !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KMTAB !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IONIC' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KMTAB2p1 (IN,TEMP,G01,G02,G03,G04,G05,G06,G07,G08,G09,G10, & G11,G12,G15,G16,G17,G18,G19,G20,G21,G22,G23) REAL IN, Temp, binarray (23) !C !C *** Find temperature range !C IND = NINT((TEMP-198.0)/25.0) + 1 IND = MIN(MAX(IND,1),6) !C !C *** Call appropriate routine !C IF (IND.EQ.1) THEN CALL KM1982p1 (IN,binarray) ELSEIF (IND.EQ.2) THEN CALL KM2232p1 (IN,binarray) ELSEIF (IND.EQ.3) THEN CALL KM2482p1 (IN,binarray) ELSEIF (IND.EQ.4) THEN CALL KM2732p1 (IN,binarray) ELSEIF (IND.EQ.5) THEN CALL KM2982p1 (IN,binarray) ELSE CALL KM3232p1 (IN,binarray) ENDIF !C G01 = binarray(01) G02 = binarray(02) G03 = binarray(03) G04 = binarray(04) G05 = binarray(05) G06 = binarray(06) G07 = binarray(07) G08 = binarray(08) G09 = binarray(09) G10 = binarray(10) G11 = binarray(11) G12 = binarray(12) G13 = binarray(13) G14 = binarray(14) G15 = binarray(15) G16 = binarray(16) G17 = binarray(17) G18 = binarray(18) G19 = binarray(19) G20 = binarray(20) G21 = binarray(21) G22 = binarray(22) G23 = binarray(23) !C !C *** Return point; End of subroutine !C RETURN END !C INTEGER FUNCTION IBACPOS(IN) !CC !CC Compute the index in the binary activity coefficient array !CC based on the input ionic strength. !CC !CC Chris Nolte, 6/16/05 !CC !C implicit none !C real IN !C IF (IN .LE. 0.300000E+02) THEN !C ibacpos = MIN(NINT( 0.200000E+02*IN) + 1, 600) !C ELSE !C ibacpos = 600+NINT( 0.200000E+01*IN- 0.600000E+02) !C ENDIF !C ibacpos = min(ibacpos, 741) !C return !C end !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KM198 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IN' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C TEMPERATURE IS 198K !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KM1982p1 (IONIC, BINARR) !C !C *** Common block definition !C COMMON /KMC1982p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) REAL Binarr (23), Ionic !C !C *** Find position in arrays for bincoef !C IF (Ionic.LE. 0.200000E+02) THEN ipos = MIN(NINT( 0.200000E+02*Ionic) + 1, 400) ELSE ipos = 400+NINT( 0.200000E+01*Ionic- 0.400000E+02) ENDIF ipos = min(ipos, 561) !C !C *** Assign values to return array !C Binarr(01) = BNC01M(ipos) Binarr(02) = BNC02M(ipos) Binarr(03) = BNC03M(ipos) Binarr(04) = BNC04M(ipos) Binarr(05) = BNC05M(ipos) Binarr(06) = BNC06M(ipos) Binarr(07) = BNC07M(ipos) Binarr(08) = BNC08M(ipos) Binarr(09) = BNC09M(ipos) Binarr(10) = BNC10M(ipos) Binarr(11) = BNC11M(ipos) Binarr(12) = BNC12M(ipos) Binarr(13) = BNC13M(ipos) Binarr(14) = BNC14M(ipos) Binarr(15) = BNC15M(ipos) Binarr(16) = BNC16M(ipos) Binarr(17) = BNC17M(ipos) Binarr(18) = BNC18M(ipos) Binarr(19) = BNC19M(ipos) Binarr(20) = BNC20M(ipos) Binarr(21) = BNC21M(ipos) Binarr(22) = BNC22M(ipos) Binarr(23) = BNC23M(ipos) !C !C *** Return point ; End of subroutine !C RETURN END BLOCK DATA KMCF1982p1 !C !C *** Common block definition !C COMMON /KMC1982p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) !C !C *** NaCl !C DATA BNC01M/& -0.050,-0.103,-0.127,-0.142,-0.154,-0.162,-0.169,-0.174,-0.178,& -0.181,-0.184,-0.186,-0.188,-0.189,-0.190,-0.191,-0.191,-0.192,& -0.192,-0.191,-0.191,-0.191,-0.190,-0.189,-0.188,-0.188,-0.187,& -0.185,-0.184,-0.183,-0.182,-0.181,-0.179,-0.178,-0.176,-0.175,& -0.173,-0.172,-0.170,-0.169,-0.167,-0.166,-0.164,-0.162,-0.161,& -0.159,-0.157,-0.156,-0.154,-0.152,-0.151,-0.149,-0.147,-0.146,& -0.144,-0.142,-0.140,-0.139,-0.137,-0.135,-0.134,-0.132,-0.130,& -0.128,-0.127,-0.125,-0.123,-0.121,-0.120,-0.118,-0.116,-0.114,& -0.112,-0.111,-0.109,-0.107,-0.105,-0.103,-0.101,-0.099,-0.098,& -0.096,-0.094,-0.092,-0.090,-0.088,-0.086,-0.084,-0.082,-0.080,& -0.078,-0.075,-0.073,-0.071,-0.069,-0.067,-0.065,-0.063,-0.060,& -0.058,-0.056,-0.054,-0.051,-0.049,-0.047,-0.045,-0.042,-0.040,& -0.038,-0.035,-0.033,-0.031,-0.028,-0.026,-0.024,-0.021,-0.019,& -0.016,-0.014,-0.012,-0.009,-0.007,-0.004,-0.002, 0.000, 0.003,& 0.005, 0.008, 0.010, 0.012, 0.015, 0.017, 0.020, 0.022, 0.024,& 0.027, 0.029, 0.032, 0.034, 0.036, 0.039, 0.041, 0.044, 0.046,& 0.048, 0.051, 0.053, 0.055, 0.058, 0.060, 0.063, 0.065, 0.067,& 0.070, 0.072, 0.074, 0.077, 0.079, 0.081, 0.084, 0.086, 0.088,& 0.091, 0.093, 0.095, 0.098, 0.100, 0.102, 0.105, 0.107, 0.109,& 0.112, 0.114, 0.116, 0.118, 0.121, 0.123, 0.125, 0.127, 0.130,& 0.132, 0.134, 0.137, 0.139, 0.141, 0.143, 0.146, 0.148, 0.150,& 0.152, 0.154, 0.157, 0.159, 0.161, 0.163, 0.166, 0.168, 0.170,& 0.172, 0.174, 0.176, 0.179, 0.181, 0.183, 0.185, 0.187, 0.190,& 0.192, 0.194, 0.196, 0.198, 0.200, 0.202, 0.205, 0.207, 0.209,& 0.211, 0.213, 0.215, 0.217, 0.219, 0.222, 0.224, 0.226, 0.228,& 0.230, 0.232, 0.234, 0.236, 0.238, 0.240, 0.242, 0.244, 0.246,& 0.249, 0.251, 0.253, 0.255, 0.257, 0.259, 0.261, 0.263, 0.265,& 0.267, 0.269, 0.271, 0.273, 0.275, 0.277, 0.279, 0.281, 0.283,& 0.285, 0.287, 0.289, 0.291, 0.293, 0.295, 0.297, 0.299, 0.301,& 0.303, 0.304, 0.306, 0.308, 0.310, 0.312, 0.314, 0.316, 0.318,& 0.320, 0.322, 0.324, 0.326, 0.328, 0.329, 0.331, 0.333, 0.335,& 0.337, 0.339, 0.341, 0.343, 0.344, 0.346, 0.348, 0.350, 0.352,& 0.354, 0.356, 0.357, 0.359, 0.361, 0.363, 0.365, 0.367, 0.368,& 0.370, 0.372, 0.374, 0.376, 0.377, 0.379, 0.381, 0.383, 0.385,& 0.386, 0.388, 0.390, 0.392, 0.393, 0.395, 0.397, 0.399, 0.401,& 0.402, 0.404, 0.406, 0.408, 0.409, 0.411, 0.413, 0.414, 0.416,& 0.418, 0.420, 0.421, 0.423, 0.425, 0.426, 0.428, 0.430, 0.432,& 0.433, 0.435, 0.437, 0.438, 0.440, 0.442, 0.443, 0.445, 0.447,& 0.448, 0.450, 0.452, 0.453, 0.455, 0.457, 0.458, 0.460, 0.461,& 0.463, 0.465, 0.466, 0.468, 0.470, 0.471, 0.473, 0.474, 0.476,& 0.478, 0.479, 0.481, 0.482, 0.484, 0.486, 0.487, 0.489, 0.490,& 0.492, 0.493, 0.495, 0.497, 0.498, 0.500, 0.501, 0.503, 0.504,& 0.506, 0.508, 0.509, 0.511, 0.512, 0.514, 0.515, 0.517, 0.518,& 0.520, 0.521, 0.523, 0.524, 0.526, 0.527, 0.529, 0.530, 0.532,& 0.533, 0.535, 0.536, 0.538, 0.554, 0.568, 0.582, 0.596, 0.610,& 0.623, 0.636, 0.649, 0.661, 0.674, 0.686, 0.698, 0.709, 0.721,& 0.732, 0.743, 0.754, 0.765, 0.775, 0.786, 0.796, 0.806, 0.815,& 0.825, 0.834, 0.844, 0.853, 0.862, 0.870, 0.879, 0.887, 0.896,& 0.904, 0.912, 0.920, 0.928, 0.935, 0.943, 0.950, 0.957, 0.964,& 0.971, 0.978, 0.985, 0.992, 0.998, 1.005, 1.011, 1.017, 1.023,& 1.029, 1.035, 1.041, 1.047, 1.052, 1.058, 1.063, 1.068, 1.074,& 1.079, 1.084, 1.089, 1.094, 1.099, 1.103, 1.108, 1.112, 1.117,& 1.121, 1.126, 1.130, 1.134, 1.138, 1.142, 1.146, 1.150, 1.154,& 1.158, 1.161, 1.165, 1.169, 1.172, 1.175, 1.179, 1.182, 1.185,& 1.189, 1.192, 1.195, 1.198, 1.201, 1.204, 1.206, 1.209, 1.212,& 1.215, 1.217, 1.220, 1.222, 1.225, 1.227, 1.230, 1.232, 1.234,& 1.236, 1.239, 1.241, 1.243, 1.245, 1.247, 1.249, 1.251, 1.253,& 1.254, 1.256, 1.258, 1.260, 1.261, 1.263, 1.264, 1.266, 1.267,& 1.269, 1.270, 1.272, 1.273, 1.274, 1.276, 1.277, 1.278, 1.279,& 1.280, 1.281, 1.283, 1.284, 1.285, 1.286, 1.286, 1.287, 1.288,& 1.289, 1.290, 1.291, 1.291, 1.292, 1.293, 1.293, 1.294, 1.295,& 1.295, 1.296, 1.296, 1.297, 1.297, 1.297, 1.298, 1.298, 1.298,& 1.299, 1.299, 1.299& / !C !C *** Na2SO4 !C DATA BNC02M/& -0.103,-0.225,-0.288,-0.332,-0.367,-0.397,-0.422,-0.445,-0.465,& -0.484,-0.501,-0.516,-0.531,-0.545,-0.558,-0.570,-0.582,-0.593,& -0.604,-0.614,-0.624,-0.633,-0.643,-0.651,-0.660,-0.668,-0.676,& -0.684,-0.692,-0.699,-0.707,-0.714,-0.721,-0.727,-0.734,-0.741,& -0.747,-0.753,-0.759,-0.765,-0.771,-0.777,-0.783,-0.788,-0.794,& -0.799,-0.804,-0.810,-0.815,-0.820,-0.825,-0.830,-0.835,-0.840,& -0.845,-0.849,-0.854,-0.859,-0.863,-0.868,-0.872,-0.877,-0.881,& -0.885,-0.889,-0.894,-0.898,-0.902,-0.906,-0.910,-0.914,-0.918,& -0.922,-0.926,-0.930,-0.934,-0.938,-0.942,-0.946,-0.949,-0.953,& -0.957,-0.961,-0.964,-0.968,-0.971,-0.975,-0.979,-0.982,-0.986,& -0.989,-0.993,-0.996,-1.000,-1.003,-1.007,-1.010,-1.014,-1.017,& -1.020,-1.024,-1.027,-1.030,-1.034,-1.037,-1.040,-1.044,-1.047,& -1.050,-1.053,-1.057,-1.060,-1.063,-1.066,-1.069,-1.072,-1.076,& -1.079,-1.082,-1.085,-1.088,-1.091,-1.094,-1.097,-1.100,-1.103,& -1.106,-1.109,-1.112,-1.115,-1.118,-1.121,-1.124,-1.127,-1.130,& -1.133,-1.136,-1.139,-1.142,-1.145,-1.147,-1.150,-1.153,-1.156,& -1.159,-1.162,-1.165,-1.167,-1.170,-1.173,-1.176,-1.179,-1.181,& -1.184,-1.187,-1.190,-1.192,-1.195,-1.198,-1.200,-1.203,-1.206,& -1.209,-1.211,-1.214,-1.217,-1.219,-1.222,-1.225,-1.227,-1.230,& -1.232,-1.235,-1.238,-1.240,-1.243,-1.246,-1.248,-1.251,-1.253,& -1.256,-1.258,-1.261,-1.264,-1.266,-1.269,-1.271,-1.274,-1.276,& -1.279,-1.281,-1.284,-1.286,-1.289,-1.291,-1.294,-1.296,-1.299,& -1.301,-1.304,-1.306,-1.309,-1.311,-1.313,-1.316,-1.318,-1.321,& -1.323,-1.326,-1.328,-1.330,-1.333,-1.335,-1.338,-1.340,-1.342,& -1.345,-1.347,-1.350,-1.352,-1.354,-1.357,-1.359,-1.361,-1.364,& -1.366,-1.368,-1.371,-1.373,-1.375,-1.378,-1.380,-1.382,-1.385,& -1.387,-1.389,-1.392,-1.394,-1.396,-1.399,-1.401,-1.403,-1.405,& -1.408,-1.410,-1.412,-1.415,-1.417,-1.419,-1.421,-1.424,-1.426,& -1.428,-1.430,-1.433,-1.435,-1.437,-1.439,-1.442,-1.444,-1.446,& -1.448,-1.450,-1.453,-1.455,-1.457,-1.459,-1.461,-1.464,-1.466,& -1.468,-1.470,-1.472,-1.475,-1.477,-1.479,-1.481,-1.483,-1.485,& -1.488,-1.490,-1.492,-1.494,-1.496,-1.498,-1.501,-1.503,-1.505,& -1.507,-1.509,-1.511,-1.513,-1.516,-1.518,-1.520,-1.522,-1.524,& -1.526,-1.528,-1.530,-1.533,-1.535,-1.537,-1.539,-1.541,-1.543,& -1.545,-1.547,-1.549,-1.551,-1.554,-1.556,-1.558,-1.560,-1.562,& -1.564,-1.566,-1.568,-1.570,-1.572,-1.574,-1.576,-1.578,-1.580,& -1.583,-1.585,-1.587,-1.589,-1.591,-1.593,-1.595,-1.597,-1.599,& -1.601,-1.603,-1.605,-1.607,-1.609,-1.611,-1.613,-1.615,-1.617,& -1.619,-1.621,-1.623,-1.625,-1.627,-1.629,-1.631,-1.633,-1.635,& -1.637,-1.639,-1.641,-1.643,-1.645,-1.647,-1.649,-1.651,-1.653,& -1.655,-1.657,-1.659,-1.661,-1.663,-1.665,-1.667,-1.669,-1.671,& -1.673,-1.675,-1.677,-1.679,-1.681,-1.683,-1.685,-1.687,-1.689,& -1.691,-1.693,-1.695,-1.696,-1.698,-1.700,-1.702,-1.704,-1.706,& -1.708,-1.710,-1.712,-1.714,-1.716,-1.718,-1.720,-1.722,-1.724,& -1.726,-1.727,-1.729,-1.731,-1.752,-1.771,-1.790,-1.808,-1.827,& -1.845,-1.864,-1.882,-1.900,-1.918,-1.936,-1.954,-1.972,-1.989,& -2.007,-2.024,-2.042,-2.059,-2.076,-2.093,-2.110,-2.127,-2.144,& -2.161,-2.178,-2.194,-2.211,-2.228,-2.244,-2.261,-2.277,-2.293,& -2.310,-2.326,-2.342,-2.358,-2.374,-2.390,-2.406,-2.422,-2.438,& -2.454,-2.470,-2.486,-2.501,-2.517,-2.533,-2.548,-2.564,-2.579,& -2.595,-2.610,-2.626,-2.641,-2.657,-2.672,-2.687,-2.702,-2.718,& -2.733,-2.748,-2.763,-2.778,-2.793,-2.808,-2.823,-2.838,-2.853,& -2.868,-2.883,-2.898,-2.913,-2.927,-2.942,-2.957,-2.972,-2.986,& -3.001,-3.016,-3.030,-3.045,-3.059,-3.074,-3.089,-3.103,-3.118,& -3.132,-3.147,-3.161,-3.175,-3.190,-3.204,-3.219,-3.233,-3.247,& -3.261,-3.276,-3.290,-3.304,-3.318,-3.333,-3.347,-3.361,-3.375,& 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8.354, 8.381, 8.407, 8.433, 8.458, 8.484, 8.509,& 8.534, 8.559, 8.584, 8.609, 8.633, 8.657, 8.681, 8.705, 8.729,& 8.752, 8.776, 8.799, 8.822, 8.845, 8.868, 8.890, 8.913, 8.935,& 8.957, 8.979, 9.001, 9.022, 9.044, 9.065, 9.086, 9.107, 9.128,& 9.149, 9.170, 9.190, 9.211, 9.231, 9.251, 9.271, 9.291, 9.311,& 9.330, 9.350, 9.369, 9.388, 9.407, 9.426, 9.445, 9.464, 9.483,& 9.501, 9.520, 9.538, 9.556, 9.574, 9.592, 9.610, 9.628, 9.645,& 9.663, 9.680, 9.698 & / !C !C *** NH4HSO4 !C DATA BNC09M/ & -0.050,-0.107,-0.134,-0.153,-0.167,-0.179,-0.189,-0.197,-0.204,& -0.211,-0.216,-0.221,-0.226,-0.230,-0.234,-0.237,-0.240,-0.243,& -0.245,-0.247,-0.249,-0.251,-0.252,-0.254,-0.255,-0.256,-0.256,& -0.257,-0.257,-0.258,-0.258,-0.258,-0.258,-0.258,-0.257,-0.257,& -0.256,-0.255,-0.255,-0.254,-0.253,-0.252,-0.250,-0.249,-0.248,& -0.246,-0.245,-0.243,-0.242,-0.240,-0.238,-0.236,-0.234,-0.232,& -0.230,-0.228,-0.226,-0.224,-0.221,-0.219,-0.217,-0.214,-0.212,& -0.209,-0.207,-0.204,-0.201,-0.199,-0.196,-0.193,-0.190,-0.188,& -0.185,-0.182,-0.179,-0.176,-0.173,-0.170,-0.167,-0.163,-0.160,& -0.157,-0.154,-0.150,-0.147,-0.144,-0.140,-0.137,-0.133,-0.130,& -0.126,-0.123,-0.119,-0.116,-0.112,-0.108,-0.104,-0.101,-0.097,& -0.093,-0.089,-0.086,-0.082,-0.078,-0.074,-0.070,-0.066,-0.062,& -0.058,-0.054,-0.050,-0.046,-0.042,-0.038,-0.034,-0.030,-0.026,& -0.022,-0.018,-0.014,-0.010,-0.006,-0.002, 0.002, 0.006, 0.010,& 0.014, 0.018, 0.022, 0.026, 0.030, 0.034, 0.038, 0.042, 0.046,& 0.050, 0.054, 0.058, 0.062, 0.066, 0.070, 0.074, 0.078, 0.082,& 0.086, 0.090, 0.094, 0.098, 0.102, 0.106, 0.110, 0.114, 0.117,& 0.121, 0.125, 0.129, 0.133, 0.137, 0.140, 0.144, 0.148, 0.152,& 0.156, 0.159, 0.163, 0.167, 0.171, 0.174, 0.178, 0.182, 0.186,& 0.189, 0.193, 0.197, 0.200, 0.204, 0.208, 0.211, 0.215, 0.219,& 0.222, 0.226, 0.229, 0.233, 0.237, 0.240, 0.244, 0.247, 0.251,& 0.254, 0.258, 0.261, 0.265, 0.268, 0.272, 0.275, 0.279, 0.282,& 0.286, 0.289, 0.293, 0.296, 0.299, 0.303, 0.306, 0.309, 0.313,& 0.316, 0.320, 0.323, 0.326, 0.330, 0.333, 0.336, 0.339, 0.343,& 0.346, 0.349, 0.353, 0.356, 0.359, 0.362, 0.366, 0.369, 0.372,& 0.375, 0.378, 0.382, 0.385, 0.388, 0.391, 0.394, 0.397, 0.401,& 0.404, 0.407, 0.410, 0.413, 0.416, 0.419, 0.422, 0.425, 0.428,& 0.431, 0.434, 0.438, 0.441, 0.444, 0.447, 0.450, 0.453, 0.456,& 0.459, 0.462, 0.465, 0.467, 0.470, 0.473, 0.476, 0.479, 0.482,& 0.485, 0.488, 0.491, 0.494, 0.497, 0.500, 0.502, 0.505, 0.508,& 0.511, 0.514, 0.517, 0.520, 0.522, 0.525, 0.528, 0.531, 0.534,& 0.536, 0.539, 0.542, 0.545, 0.547, 0.550, 0.553, 0.556, 0.558,& 0.561, 0.564, 0.567, 0.569, 0.572, 0.575, 0.577, 0.580, 0.583,& 0.585, 0.588, 0.591, 0.593, 0.596, 0.599, 0.601, 0.604, 0.607,& 0.609, 0.612, 0.614, 0.617, 0.620, 0.622, 0.625, 0.627, 0.630,& 0.633, 0.635, 0.638, 0.640, 0.643, 0.645, 0.648, 0.650, 0.653,& 0.655, 0.658, 0.660, 0.663, 0.665, 0.668, 0.670, 0.673, 0.675,& 0.678, 0.680, 0.683, 0.685, 0.687, 0.690, 0.692, 0.695, 0.697,& 0.700, 0.702, 0.704, 0.707, 0.709, 0.711, 0.714, 0.716, 0.719,& 0.721, 0.723, 0.726, 0.728, 0.730, 0.733, 0.735, 0.737, 0.740,& 0.742, 0.744, 0.747, 0.749, 0.751, 0.754, 0.756, 0.758, 0.760,& 0.763, 0.765, 0.767, 0.769, 0.772, 0.774, 0.776, 0.778, 0.781,& 0.783, 0.785, 0.787, 0.790, 0.792, 0.794, 0.796, 0.798, 0.801,& 0.803, 0.805, 0.807, 0.809, 0.811, 0.814, 0.816, 0.818, 0.820,& 0.822, 0.824, 0.827, 0.829, 0.851, 0.872, 0.892, 0.912, 0.932,& 0.951, 0.969, 0.988, 1.006, 1.024, 1.041, 1.058, 1.075, 1.091,& 1.107, 1.123, 1.139, 1.154, 1.169, 1.184, 1.199, 1.213, 1.227,& 1.241, 1.255, 1.268, 1.282, 1.295, 1.307, 1.320, 1.332, 1.345,& 1.357, 1.368, 1.380, 1.392, 1.403, 1.414, 1.425, 1.436, 1.446,& 1.457, 1.467, 1.478, 1.488, 1.497, 1.507, 1.517, 1.526, 1.536,& 1.545, 1.554, 1.563, 1.572, 1.580, 1.589, 1.597, 1.606, 1.614,& 1.622, 1.630, 1.638, 1.646, 1.653, 1.661, 1.668, 1.676, 1.683,& 1.690, 1.697, 1.704, 1.711, 1.718, 1.724, 1.731, 1.737, 1.744,& 1.750, 1.756, 1.762, 1.769, 1.775, 1.780, 1.786, 1.792, 1.798,& 1.803, 1.809, 1.814, 1.820, 1.825, 1.830, 1.835, 1.840, 1.845,& 1.850, 1.855, 1.860, 1.865, 1.870, 1.874, 1.879, 1.883, 1.888,& 1.892, 1.896, 1.901, 1.905, 1.909, 1.913, 1.917, 1.921, 1.925,& 1.929, 1.933, 1.936, 1.940, 1.944, 1.947, 1.951, 1.955, 1.958,& 1.961, 1.965, 1.968, 1.971, 1.975, 1.978, 1.981, 1.984, 1.987,& 1.990, 1.993, 1.996, 1.999, 2.001, 2.004, 2.007, 2.010, 2.012,& 2.015, 2.017, 2.020, 2.022, 2.025, 2.027, 2.030, 2.032, 2.034,& 2.037, 2.039, 2.041, 2.043, 2.045, 2.047, 2.049, 2.051, 2.053,& 2.055, 2.057, 2.059 & / !C !C *** (H,NO3) !C DATA BNC10M/& -0.049,-0.102,-0.125,-0.140,-0.150,-0.158,-0.163,-0.168,-0.171,& -0.174,-0.176,-0.178,-0.179,-0.179,-0.179,-0.179,-0.179,-0.179,& -0.178,-0.177,-0.176,-0.175,-0.174,-0.172,-0.171,-0.169,-0.168,& -0.166,-0.164,-0.162,-0.160,-0.158,-0.156,-0.154,-0.152,-0.150,& -0.148,-0.146,-0.144,-0.141,-0.139,-0.137,-0.135,-0.132,-0.130,& -0.128,-0.126,-0.123,-0.121,-0.119,-0.116,-0.114,-0.112,-0.109,& -0.107,-0.105,-0.102,-0.100,-0.098,-0.095,-0.093,-0.091,-0.088,& -0.086,-0.084,-0.081,-0.079,-0.077,-0.074,-0.072,-0.070,-0.067,& -0.065,-0.062,-0.060,-0.057,-0.055,-0.052,-0.050,-0.048,-0.045,& -0.042,-0.040,-0.037,-0.035,-0.032,-0.030,-0.027,-0.024,-0.022,& -0.019,-0.016,-0.013,-0.011,-0.008,-0.005,-0.002, 0.001, 0.003,& 0.006, 0.009, 0.012, 0.015, 0.018, 0.021, 0.024, 0.027, 0.030,& 0.033, 0.036, 0.039, 0.042, 0.045, 0.048, 0.051, 0.054, 0.057,& 0.060, 0.063, 0.066, 0.069, 0.072, 0.075, 0.078, 0.081, 0.084,& 0.087, 0.091, 0.094, 0.097, 0.100, 0.103, 0.106, 0.109, 0.112,& 0.115, 0.118, 0.121, 0.124, 0.127, 0.130, 0.133, 0.136, 0.139,& 0.142, 0.146, 0.149, 0.152, 0.155, 0.158, 0.161, 0.164, 0.167,& 0.170, 0.173, 0.176, 0.179, 0.182, 0.185, 0.188, 0.191, 0.193,& 0.196, 0.199, 0.202, 0.205, 0.208, 0.211, 0.214, 0.217, 0.220,& 0.223, 0.226, 0.229, 0.232, 0.235, 0.237, 0.240, 0.243, 0.246,& 0.249, 0.252, 0.255, 0.258, 0.260, 0.263, 0.266, 0.269, 0.272,& 0.275, 0.278, 0.280, 0.283, 0.286, 0.289, 0.292, 0.294, 0.297,& 0.300, 0.303, 0.306, 0.308, 0.311, 0.314, 0.317, 0.319, 0.322,& 0.325, 0.328, 0.330, 0.333, 0.336, 0.339, 0.341, 0.344, 0.347,& 0.349, 0.352, 0.355, 0.358, 0.360, 0.363, 0.366, 0.368, 0.371,& 0.374, 0.376, 0.379, 0.382, 0.384, 0.387, 0.389, 0.392, 0.395,& 0.397, 0.400, 0.403, 0.405, 0.408, 0.410, 0.413, 0.415, 0.418,& 0.421, 0.423, 0.426, 0.428, 0.431, 0.433, 0.436, 0.438, 0.441,& 0.444, 0.446, 0.449, 0.451, 0.454, 0.456, 0.459, 0.461, 0.464,& 0.466, 0.469, 0.471, 0.473, 0.476, 0.478, 0.481, 0.483, 0.486,& 0.488, 0.491, 0.493, 0.495, 0.498, 0.500, 0.503, 0.505, 0.508,& 0.510, 0.512, 0.515, 0.517, 0.519, 0.522, 0.524, 0.527, 0.529,& 0.531, 0.534, 0.536, 0.538, 0.541, 0.543, 0.545, 0.548, 0.550,& 0.552, 0.555, 0.557, 0.559, 0.562, 0.564, 0.566, 0.568, 0.571,& 0.573, 0.575, 0.578, 0.580, 0.582, 0.584, 0.587, 0.589, 0.591,& 0.593, 0.595, 0.598, 0.600, 0.602, 0.604, 0.607, 0.609, 0.611,& 0.613, 0.615, 0.618, 0.620, 0.622, 0.624, 0.626, 0.628, 0.631,& 0.633, 0.635, 0.637, 0.639, 0.641, 0.644, 0.646, 0.648, 0.650,& 0.652, 0.654, 0.656, 0.658, 0.660, 0.663, 0.665, 0.667, 0.669,& 0.671, 0.673, 0.675, 0.677, 0.679, 0.681, 0.683, 0.685, 0.688,& 0.690, 0.692, 0.694, 0.696, 0.698, 0.700, 0.702, 0.704, 0.706,& 0.708, 0.710, 0.712, 0.714, 0.716, 0.718, 0.720, 0.722, 0.724,& 0.726, 0.728, 0.730, 0.732, 0.734, 0.736, 0.738, 0.740, 0.742,& 0.743, 0.745, 0.747, 0.749, 0.751, 0.753, 0.755, 0.757, 0.759,& 0.761, 0.763, 0.765, 0.767, 0.787, 0.805, 0.824, 0.841, 0.859,& 0.876, 0.893, 0.909, 0.926, 0.942, 0.957, 0.973, 0.988, 1.003,& 1.017, 1.032, 1.046, 1.060, 1.073, 1.087, 1.100, 1.113, 1.126,& 1.138, 1.151, 1.163, 1.175, 1.187, 1.198, 1.210, 1.221, 1.232,& 1.243, 1.253, 1.264, 1.274, 1.285, 1.295, 1.305, 1.314, 1.324,& 1.333, 1.343, 1.352, 1.361, 1.370, 1.378, 1.387, 1.395, 1.404,& 1.412, 1.420, 1.428, 1.436, 1.444, 1.451, 1.459, 1.466, 1.474,& 1.481, 1.488, 1.495, 1.502, 1.509, 1.515, 1.522, 1.529, 1.535,& 1.541, 1.548, 1.554, 1.560, 1.566, 1.572, 1.577, 1.583, 1.589,& 1.594, 1.600, 1.605, 1.610, 1.616, 1.621, 1.626, 1.631, 1.636,& 1.641, 1.645, 1.650, 1.655, 1.659, 1.664, 1.668, 1.673, 1.677,& 1.681, 1.685, 1.690, 1.694, 1.698, 1.702, 1.705, 1.709, 1.713,& 1.717, 1.720, 1.724, 1.728, 1.731, 1.734, 1.738, 1.741, 1.744,& 1.748, 1.751, 1.754, 1.757, 1.760, 1.763, 1.766, 1.769, 1.772,& 1.775, 1.777, 1.780, 1.783, 1.785, 1.788, 1.790, 1.793, 1.795,& 1.798, 1.800, 1.802, 1.805, 1.807, 1.809, 1.811, 1.813, 1.815,& 1.817, 1.819, 1.821, 1.823, 1.825, 1.827, 1.829, 1.831, 1.832,& 1.834, 1.836, 1.838, 1.839, 1.841, 1.842, 1.844, 1.845, 1.847,& 1.848, 1.849, 1.851 & / !C !C *** (H,Cl) !C DATA BNC11M/ & -0.048,-0.094,-0.112,-0.122,-0.128,-0.131,-0.133,-0.133,-0.133,& -0.131,-0.129,-0.126,-0.123,-0.119,-0.116,-0.111,-0.107,-0.102,& -0.097,-0.092,-0.086,-0.080,-0.075,-0.069,-0.062,-0.056,-0.050,& -0.043,-0.037,-0.030,-0.023,-0.016,-0.009,-0.002, 0.005, 0.012,& 0.020, 0.027, 0.035, 0.042, 0.050, 0.057, 0.065, 0.072, 0.080,& 0.088, 0.095, 0.103, 0.111, 0.119, 0.126, 0.134, 0.142, 0.150,& 0.158, 0.166, 0.174, 0.182, 0.190, 0.198, 0.206, 0.214, 0.222,& 0.230, 0.238, 0.246, 0.254, 0.262, 0.270, 0.278, 0.287, 0.295,& 0.303, 0.311, 0.320, 0.328, 0.336, 0.345, 0.353, 0.362, 0.370,& 0.379, 0.387, 0.396, 0.405, 0.413, 0.422, 0.431, 0.440, 0.449,& 0.457, 0.466, 0.475, 0.484, 0.494, 0.503, 0.512, 0.521, 0.530,& 0.540, 0.549, 0.558, 0.568, 0.577, 0.587, 0.596, 0.606, 0.615,& 0.625, 0.634, 0.644, 0.653, 0.663, 0.673, 0.682, 0.692, 0.702,& 0.711, 0.721, 0.731, 0.740, 0.750, 0.760, 0.769, 0.779, 0.789,& 0.798, 0.808, 0.818, 0.827, 0.837, 0.847, 0.856, 0.866, 0.875,& 0.885, 0.895, 0.904, 0.914, 0.923, 0.933, 0.942, 0.952, 0.961,& 0.971, 0.980, 0.990, 0.999, 1.009, 1.018, 1.027, 1.037, 1.046,& 1.055, 1.065, 1.074, 1.083, 1.093, 1.102, 1.111, 1.120, 1.130,& 1.139, 1.148, 1.157, 1.166, 1.175, 1.184, 1.194, 1.203, 1.212,& 1.221, 1.230, 1.239, 1.248, 1.257, 1.266, 1.275, 1.283, 1.292,& 1.301, 1.310, 1.319, 1.328, 1.336, 1.345, 1.354, 1.363, 1.372,& 1.380, 1.389, 1.398, 1.406, 1.415, 1.423, 1.432, 1.441, 1.449,& 1.458, 1.466, 1.475, 1.483, 1.492, 1.500, 1.509, 1.517, 1.526,& 1.534, 1.542, 1.551, 1.559, 1.567, 1.576, 1.584, 1.592, 1.600,& 1.609, 1.617, 1.625, 1.633, 1.641, 1.649, 1.658, 1.666, 1.674,& 1.682, 1.690, 1.698, 1.706, 1.714, 1.722, 1.730, 1.738, 1.746,& 1.754, 1.762, 1.769, 1.777, 1.785, 1.793, 1.801, 1.809, 1.816,& 1.824, 1.832, 1.840, 1.847, 1.855, 1.863, 1.870, 1.878, 1.886,& 1.893, 1.901, 1.908, 1.916, 1.924, 1.931, 1.939, 1.946, 1.954,& 1.961, 1.969, 1.976, 1.983, 1.991, 1.998, 2.006, 2.013, 2.020,& 2.028, 2.035, 2.042, 2.049, 2.057, 2.064, 2.071, 2.078, 2.086,& 2.093, 2.100, 2.107, 2.114, 2.122, 2.129, 2.136, 2.143, 2.150,& 2.157, 2.164, 2.171, 2.178, 2.185, 2.192, 2.199, 2.206, 2.213,& 2.220, 2.227, 2.234, 2.241, 2.247, 2.254, 2.261, 2.268, 2.275,& 2.282, 2.288, 2.295, 2.302, 2.309, 2.315, 2.322, 2.329, 2.336,& 2.342, 2.349, 2.356, 2.362, 2.369, 2.376, 2.382, 2.389, 2.395,& 2.402, 2.408, 2.415, 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5.331,& 5.355, 5.378, 5.401, 5.424, 5.447, 5.469, 5.492, 5.514, 5.536,& 5.557, 5.579, 5.600, 5.621, 5.642, 5.663, 5.684, 5.704, 5.724,& 5.744, 5.764, 5.784, 5.803, 5.823, 5.842, 5.861, 5.880, 5.898,& 5.917, 5.935, 5.953, 5.972, 5.989, 6.007, 6.025, 6.042, 6.060,& 6.077, 6.094, 6.111, 6.128, 6.144, 6.161, 6.177, 6.194, 6.210,& 6.226, 6.242, 6.257, 6.273, 6.289, 6.304, 6.319, 6.334, 6.350,& 6.365, 6.379, 6.394, 6.409, 6.423, 6.438, 6.452, 6.466, 6.480,& 6.494, 6.508, 6.522, 6.536, 6.549, 6.563, 6.576, 6.589, 6.602,& 6.616, 6.629, 6.641, 6.654, 6.667, 6.680, 6.692, 6.705, 6.717,& 6.729, 6.742, 6.754, 6.766, 6.778, 6.790, 6.801, 6.813, 6.825,& 6.836, 6.848, 6.859 & / !C !C *** NaHSO4 !C DATA BNC12M/ & -0.049,-0.101,-0.125,-0.140,-0.151,-0.159,-0.166,-0.171,-0.175,& -0.178,-0.181,-0.183,-0.184,-0.185,-0.186,-0.186,-0.186,-0.186,& -0.186,-0.185,-0.184,-0.183,-0.181,-0.180,-0.178,-0.176,-0.174,& -0.172,-0.170,-0.167,-0.165,-0.162,-0.159,-0.156,-0.153,-0.150,& 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1.883, 1.888,& 1.892, 1.897, 1.902, 1.906, 1.954, 1.998, 2.040, 2.082, 2.124,& 2.164, 2.204, 2.243, 2.282, 2.319, 2.356, 2.393, 2.429, 2.464,& 2.499, 2.533, 2.567, 2.600, 2.632, 2.664, 2.695, 2.726, 2.757,& 2.787, 2.816, 2.845, 2.874, 2.902, 2.930, 2.957, 2.984, 3.010,& 3.036, 3.062, 3.087, 3.112, 3.137, 3.161, 3.185, 3.208, 3.232,& 3.254, 3.277, 3.299, 3.321, 3.342, 3.364, 3.385, 3.405, 3.426,& 3.446, 3.466, 3.485, 3.504, 3.523, 3.542, 3.561, 3.579, 3.597,& 3.615, 3.632, 3.649, 3.666, 3.683, 3.700, 3.716, 3.732, 3.748,& 3.764, 3.779, 3.795, 3.810, 3.825, 3.839, 3.854, 3.868, 3.882,& 3.896, 3.910, 3.924, 3.937, 3.950, 3.964, 3.976, 3.989, 4.002,& 4.014, 4.026, 4.039, 4.050, 4.062, 4.074, 4.085, 4.097, 4.108,& 4.119, 4.130, 4.141, 4.151, 4.162, 4.172, 4.182, 4.192, 4.202,& 4.212, 4.222, 4.231, 4.241, 4.250, 4.259, 4.268, 4.277, 4.286,& 4.295, 4.304, 4.312, 4.321, 4.329, 4.337, 4.345, 4.353, 4.361,& 4.369, 4.376, 4.384, 4.391, 4.399, 4.406, 4.413, 4.420, 4.427,& 4.434, 4.441, 4.447, 4.454, 4.460, 4.467, 4.473, 4.479, 4.485,& 4.491, 4.497, 4.503, 4.509, 4.515, 4.520, 4.526, 4.531, 4.537,& 4.542, 4.547, 4.552, 4.557, 4.562, 4.567, 4.572, 4.577, 4.582,& 4.586, 4.591, 4.595 & / END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KM223 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IN' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C TEMPERATURE IS 223K !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KM2232p1 (IONIC, BINARR) !C !C *** Common block definition !C COMMON /KMC2232p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) REAL Binarr (23), Ionic !C !C *** Find position in arrays for bincoef !C IF (Ionic.LE. 0.200000E+02) THEN ipos = MIN(NINT( 0.200000E+02*Ionic) + 1, 400) ELSE ipos = 400+NINT( 0.200000E+01*Ionic- 0.400000E+02) ENDIF ipos = min(ipos, 561) !C !C *** Assign values to return array !C Binarr(01) = BNC01M(ipos) Binarr(02) = BNC02M(ipos) Binarr(03) = BNC03M(ipos) Binarr(04) = BNC04M(ipos) Binarr(05) = BNC05M(ipos) Binarr(06) = BNC06M(ipos) Binarr(07) = BNC07M(ipos) Binarr(08) = BNC08M(ipos) Binarr(09) = BNC09M(ipos) Binarr(10) = BNC10M(ipos) Binarr(11) = BNC11M(ipos) Binarr(12) = BNC12M(ipos) Binarr(13) = BNC13M(ipos) Binarr(14) = BNC14M(ipos) Binarr(15) = BNC15M(ipos) Binarr(16) = BNC16M(ipos) Binarr(17) = BNC17M(ipos) Binarr(18) = BNC18M(ipos) Binarr(19) = BNC19M(ipos) Binarr(20) = BNC20M(ipos) Binarr(21) = BNC21M(ipos) Binarr(22) = BNC22M(ipos) Binarr(23) = BNC23M(ipos) !C !C *** Return point ; End of subroutine !C RETURN END BLOCK DATA KMCF2232p1 !C !C *** Common block definition !C COMMON /KMC2232p1/& BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) !C !C *** NaCl !C DATA BNC01M/ & -0.049,-0.101,-0.124,-0.140,-0.151,-0.159,-0.166,-0.171,-0.175,& -0.178,-0.181,-0.183,-0.185,-0.187,-0.188,-0.188,-0.189,-0.189,& -0.189,-0.189,-0.189,-0.189,-0.188,-0.187,-0.187,-0.186,-0.185,& -0.184,-0.183,-0.182,-0.181,-0.180,-0.178,-0.177,-0.176,-0.174,& -0.173,-0.172,-0.170,-0.169,-0.167,-0.166,-0.164,-0.163,-0.161,& -0.159,-0.158,-0.156,-0.155,-0.153,-0.151,-0.150,-0.148,-0.147,& -0.145,-0.143,-0.142,-0.140,-0.138,-0.137,-0.135,-0.134,-0.132,& -0.130,-0.128,-0.127,-0.125,-0.123,-0.122,-0.120,-0.118,-0.117,& -0.115,-0.113,-0.111,-0.110,-0.108,-0.106,-0.104,-0.102,-0.101,& -0.099,-0.097,-0.095,-0.093,-0.091,-0.089,-0.087,-0.085,-0.083,& -0.081,-0.079,-0.077,-0.075,-0.073,-0.071,-0.069,-0.067,-0.065,& -0.063,-0.061,-0.058,-0.056,-0.054,-0.052,-0.050,-0.048,-0.045,& -0.043,-0.041,-0.039,-0.036,-0.034,-0.032,-0.030,-0.027,-0.025,& -0.023,-0.020,-0.018,-0.016,-0.014,-0.011,-0.009,-0.007,-0.004,& -0.002, 0.000, 0.003, 0.005, 0.007, 0.010, 0.012, 0.014, 0.016,& 0.019, 0.021, 0.023, 0.026, 0.028, 0.030, 0.033, 0.035, 0.037,& 0.039, 0.042, 0.044, 0.046, 0.049, 0.051, 0.053, 0.055, 0.058,& 0.060, 0.062, 0.064, 0.067, 0.069, 0.071, 0.073, 0.076, 0.078,& 0.080, 0.082, 0.085, 0.087, 0.089, 0.091, 0.094, 0.096, 0.098,& 0.100, 0.102, 0.105, 0.107, 0.109, 0.111, 0.113, 0.116, 0.118,& 0.120, 0.122, 0.124, 0.126, 0.129, 0.131, 0.133, 0.135, 0.137,& 0.139, 0.142, 0.144, 0.146, 0.148, 0.150, 0.152, 0.154, 0.157,& 0.159, 0.161, 0.163, 0.165, 0.167, 0.169, 0.171, 0.173, 0.175,& 0.178, 0.180, 0.182, 0.184, 0.186, 0.188, 0.190, 0.192, 0.194,& 0.196, 0.198, 0.200, 0.202, 0.204, 0.206, 0.208, 0.211, 0.213,& 0.215, 0.217, 0.219, 0.221, 0.223, 0.225, 0.227, 0.229, 0.231,& 0.233, 0.235, 0.237, 0.239, 0.241, 0.243, 0.245, 0.246, 0.248,& 0.250, 0.252, 0.254, 0.256, 0.258, 0.260, 0.262, 0.264, 0.266,& 0.268, 0.270, 0.272, 0.274, 0.276, 0.277, 0.279, 0.281, 0.283,& 0.285, 0.287, 0.289, 0.291, 0.293, 0.295, 0.296, 0.298, 0.300,& 0.302, 0.304, 0.306, 0.308, 0.309, 0.311, 0.313, 0.315, 0.317,& 0.319, 0.320, 0.322, 0.324, 0.326, 0.328, 0.330, 0.331, 0.333,& 0.335, 0.337, 0.339, 0.340, 0.342, 0.344, 0.346, 0.348, 0.349,& 0.351, 0.353, 0.355, 0.356, 0.358, 0.360, 0.362, 0.363, 0.365,& 0.367, 0.369, 0.370, 0.372, 0.374, 0.376, 0.377, 0.379, 0.381,& 0.383, 0.384, 0.386, 0.388, 0.389, 0.391, 0.393, 0.394, 0.396,& 0.398, 0.400, 0.401, 0.403, 0.405, 0.406, 0.408, 0.410, 0.411,& 0.413, 0.415, 0.416, 0.418, 0.420, 0.421, 0.423, 0.424, 0.426,& 0.428, 0.429, 0.431, 0.433, 0.434, 0.436, 0.437, 0.439, 0.441,& 0.442, 0.444, 0.446, 0.447, 0.449, 0.450, 0.452, 0.453, 0.455,& 0.457, 0.458, 0.460, 0.461, 0.463, 0.464, 0.466, 0.468, 0.469,& 0.471, 0.472, 0.474, 0.475, 0.477, 0.478, 0.480, 0.482, 0.483,& 0.485, 0.486, 0.488, 0.489, 0.491, 0.492, 0.494, 0.495, 0.497,& 0.498, 0.500, 0.501, 0.503, 0.504, 0.506, 0.507, 0.509, 0.510,& 0.512, 0.513, 0.515, 0.516, 0.532, 0.546, 0.560, 0.574, 0.588,& 0.601, 0.614, 0.627, 0.639, 0.652, 0.664, 0.676, 0.688, 0.700,& 0.711, 0.722, 0.733, 0.744, 0.755, 0.765, 0.776, 0.786, 0.796,& 0.806, 0.816, 0.825, 0.835, 0.844, 0.853, 0.862, 0.871, 0.880,& 0.888, 0.897, 0.905, 0.913, 0.921, 0.929, 0.937, 0.945, 0.952,& 0.960, 0.967, 0.975, 0.982, 0.989, 0.996, 1.003, 1.009, 1.016,& 1.023, 1.029, 1.036, 1.042, 1.048, 1.054, 1.060, 1.066, 1.072,& 1.078, 1.084, 1.089, 1.095, 1.100, 1.106, 1.111, 1.116, 1.121,& 1.126, 1.131, 1.136, 1.141, 1.146, 1.151, 1.156, 1.160, 1.165,& 1.169, 1.174, 1.178, 1.182, 1.187, 1.191, 1.195, 1.199, 1.203,& 1.207, 1.211, 1.215, 1.219, 1.223, 1.226, 1.230, 1.234, 1.237,& 1.241, 1.244, 1.247, 1.251, 1.254, 1.257, 1.261, 1.264, 1.267,& 1.270, 1.273, 1.276, 1.279, 1.282, 1.285, 1.288, 1.291, 1.293,& 1.296, 1.299, 1.301, 1.304, 1.306, 1.309, 1.311, 1.314, 1.316,& 1.319, 1.321, 1.323, 1.326, 1.328, 1.330, 1.332, 1.334, 1.336,& 1.339, 1.341, 1.343, 1.345, 1.347, 1.348, 1.350, 1.352, 1.354,& 1.356, 1.358, 1.359, 1.361, 1.363, 1.364, 1.366, 1.368, 1.369,& 1.371, 1.372, 1.374, 1.375, 1.377, 1.378, 1.379, 1.381, 1.382,& 1.383, 1.385, 1.386 & / !C !C *** Na2SO4 !C DATA BNC02M/ & -0.100,-0.220,-0.280,-0.323,-0.357,-0.385,-0.409,-0.431,-0.450,& -0.468,-0.484,-0.499,-0.513,-0.526,-0.538,-0.549,-0.560,-0.571,& -0.581,-0.590,-0.600,-0.608,-0.617,-0.625,-0.633,-0.641,-0.648,& -0.655,-0.662,-0.669,-0.676,-0.682,-0.689,-0.695,-0.701,-0.707,& -0.713,-0.718,-0.724,-0.729,-0.735,-0.740,-0.745,-0.750,-0.755,& -0.760,-0.765,-0.769,-0.774,-0.779,-0.783,-0.788,-0.792,-0.796,& -0.800,-0.805,-0.809,-0.813,-0.817,-0.821,-0.825,-0.829,-0.833,& -0.836,-0.840,-0.844,-0.848,-0.851,-0.855,-0.858,-0.862,-0.866,& -0.869,-0.873,-0.876,-0.879,-0.883,-0.886,-0.889,-0.893,-0.896,& -0.899,-0.902,-0.906,-0.909,-0.912,-0.915,-0.918,-0.921,-0.924,& -0.927,-0.930,-0.933,-0.936,-0.939,-0.942,-0.945,-0.948,-0.951,& -0.954,-0.957,-0.960,-0.963,-0.966,-0.968,-0.971,-0.974,-0.977,& -0.980,-0.982,-0.985,-0.988,-0.991,-0.993,-0.996,-0.999,-1.001,& -1.004,-1.007,-1.009,-1.012,-1.015,-1.017,-1.020,-1.022,-1.025,& -1.028,-1.030,-1.033,-1.035,-1.038,-1.040,-1.043,-1.045,-1.048,& -1.050,-1.053,-1.055,-1.058,-1.060,-1.062,-1.065,-1.067,-1.070,& -1.072,-1.074,-1.077,-1.079,-1.082,-1.084,-1.086,-1.089,-1.091,& -1.093,-1.096,-1.098,-1.100,-1.102,-1.105,-1.107,-1.109,-1.112,& -1.114,-1.116,-1.118,-1.121,-1.123,-1.125,-1.127,-1.129,-1.132,& -1.134,-1.136,-1.138,-1.140,-1.143,-1.145,-1.147,-1.149,-1.151,& -1.153,-1.155,-1.158,-1.160,-1.162,-1.164,-1.166,-1.168,-1.170,& -1.172,-1.174,-1.177,-1.179,-1.181,-1.183,-1.185,-1.187,-1.189,& -1.191,-1.193,-1.195,-1.197,-1.199,-1.201,-1.203,-1.205,-1.207,& -1.209,-1.211,-1.213,-1.215,-1.217,-1.219,-1.221,-1.223,-1.225,& -1.227,-1.229,-1.231,-1.233,-1.235,-1.237,-1.239,-1.241,-1.243,& -1.245,-1.247,-1.248,-1.250,-1.252,-1.254,-1.256,-1.258,-1.260,& -1.262,-1.264,-1.266,-1.268,-1.269,-1.271,-1.273,-1.275,-1.277,& -1.279,-1.281,-1.283,-1.284,-1.286,-1.288,-1.290,-1.292,-1.294,& -1.296,-1.297,-1.299,-1.301,-1.303,-1.305,-1.306,-1.308,-1.310,& -1.312,-1.314,-1.316,-1.317,-1.319,-1.321,-1.323,-1.325,-1.326,& -1.328,-1.330,-1.332,-1.333,-1.335,-1.337,-1.339,-1.341,-1.342,& -1.344,-1.346,-1.348,-1.349,-1.351,-1.353,-1.355,-1.356,-1.358,& -1.360,-1.362,-1.363,-1.365,-1.367,-1.369,-1.370,-1.372,-1.374,& -1.375,-1.377,-1.379,-1.381,-1.382,-1.384,-1.386,-1.387,-1.389,& -1.391,-1.393,-1.394,-1.396,-1.398,-1.399,-1.401,-1.403,-1.404,& -1.406,-1.408,-1.409,-1.411,-1.413,-1.414,-1.416,-1.418,-1.419,& -1.421,-1.423,-1.424,-1.426,-1.428,-1.429,-1.431,-1.433,-1.434,& -1.436,-1.438,-1.439,-1.441,-1.442,-1.444,-1.446,-1.447,-1.449,& -1.451,-1.452,-1.454,-1.456,-1.457,-1.459,-1.460,-1.462,-1.464,& -1.465,-1.467,-1.468,-1.470,-1.472,-1.473,-1.475,-1.476,-1.478,& -1.480,-1.481,-1.483,-1.484,-1.486,-1.488,-1.489,-1.491,-1.492,& 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7.762, 7.788, 7.813, 7.838, 7.862, 7.887, 7.912, 7.936,& 7.960, 7.984, 8.008, 8.031, 8.055, 8.078, 8.101, 8.124, 8.147,& 8.169, 8.192, 8.214, 8.236, 8.258, 8.280, 8.302, 8.323, 8.345,& 8.366, 8.387, 8.408, 8.429, 8.450, 8.470, 8.491, 8.511, 8.531,& 8.552, 8.572, 8.591, 8.611, 8.631, 8.650, 8.670, 8.689, 8.708,& 8.727, 8.746, 8.765, 8.783, 8.802, 8.820, 8.839, 8.857, 8.875,& 8.893, 8.911, 8.929, 8.946, 8.964, 8.981, 8.999, 9.016, 9.033,& 9.050, 9.067, 9.084 & / !C !C *** NH4HSO4 !C DATA BNC09M/ & -0.049,-0.104,-0.131,-0.149,-0.163,-0.174,-0.184,-0.192,-0.199,& -0.205,-0.211,-0.216,-0.220,-0.224,-0.228,-0.231,-0.234,-0.236,& -0.238,-0.240,-0.242,-0.244,-0.245,-0.247,-0.248,-0.248,-0.249,& -0.250,-0.250,-0.250,-0.251,-0.251,-0.250,-0.250,-0.250,-0.249,& -0.249,-0.248,-0.247,-0.247,-0.246,-0.245,-0.243,-0.242,-0.241,& -0.240,-0.238,-0.237,-0.235,-0.233,-0.232,-0.230,-0.228,-0.226,& -0.224,-0.222,-0.220,-0.218,-0.216,-0.214,-0.211,-0.209,-0.207,& -0.204,-0.202,-0.199,-0.197,-0.194,-0.192,-0.189,-0.187,-0.184,& -0.181,-0.178,-0.176,-0.173,-0.170,-0.167,-0.164,-0.161,-0.158,& -0.155,-0.152,-0.149,-0.146,-0.142,-0.139,-0.136,-0.133,-0.129,& -0.126,-0.123,-0.119,-0.116,-0.112,-0.109,-0.105,-0.102,-0.098,& -0.095,-0.091,-0.088,-0.084,-0.080,-0.077,-0.073,-0.069,-0.066,& -0.062,-0.058,-0.055,-0.051,-0.047,-0.043,-0.039,-0.036,-0.032,& -0.028,-0.024,-0.020,-0.017,-0.013,-0.009,-0.005,-0.001, 0.002,& 0.006, 0.010, 0.014, 0.018, 0.021, 0.025, 0.029, 0.033, 0.037,& 0.040, 0.044, 0.048, 0.052, 0.055, 0.059, 0.063, 0.067, 0.070,& 0.074, 0.078, 0.081, 0.085, 0.089, 0.093, 0.096, 0.100, 0.104,& 0.107, 0.111, 0.114, 0.118, 0.122, 0.125, 0.129, 0.133, 0.136,& 0.140, 0.143, 0.147, 0.150, 0.154, 0.157, 0.161, 0.165, 0.168,& 0.172, 0.175, 0.178, 0.182, 0.185, 0.189, 0.192, 0.196, 0.199,& 0.203, 0.206, 0.209, 0.213, 0.216, 0.220, 0.223, 0.226, 0.230,& 0.233, 0.236, 0.240, 0.243, 0.246, 0.250, 0.253, 0.256, 0.259,& 0.263, 0.266, 0.269, 0.272, 0.276, 0.279, 0.282, 0.285, 0.289,& 0.292, 0.295, 0.298, 0.301, 0.304, 0.308, 0.311, 0.314, 0.317,& 0.320, 0.323, 0.326, 0.329, 0.332, 0.336, 0.339, 0.342, 0.345,& 0.348, 0.351, 0.354, 0.357, 0.360, 0.363, 0.366, 0.369, 0.372,& 0.375, 0.378, 0.381, 0.384, 0.387, 0.390, 0.393, 0.395, 0.398,& 0.401, 0.404, 0.407, 0.410, 0.413, 0.416, 0.419, 0.421, 0.424,& 0.427, 0.430, 0.433, 0.436, 0.438, 0.441, 0.444, 0.447, 0.450,& 0.452, 0.455, 0.458, 0.461, 0.464, 0.466, 0.469, 0.472, 0.475,& 0.477, 0.480, 0.483, 0.485, 0.488, 0.491, 0.493, 0.496, 0.499,& 0.501, 0.504, 0.507, 0.509, 0.512, 0.515, 0.517, 0.520, 0.523,& 0.525, 0.528, 0.530, 0.533, 0.536, 0.538, 0.541, 0.543, 0.546,& 0.548, 0.551, 0.554, 0.556, 0.559, 0.561, 0.564, 0.566, 0.569,& 0.571, 0.574, 0.576, 0.579, 0.581, 0.584, 0.586, 0.589, 0.591,& 0.594, 0.596, 0.598, 0.601, 0.603, 0.606, 0.608, 0.611, 0.613,& 0.615, 0.618, 0.620, 0.623, 0.625, 0.627, 0.630, 0.632, 0.635,& 0.637, 0.639, 0.642, 0.644, 0.646, 0.649, 0.651, 0.653, 0.656,& 0.658, 0.660, 0.663, 0.665, 0.667, 0.670, 0.672, 0.674, 0.676,& 0.679, 0.681, 0.683, 0.685, 0.688, 0.690, 0.692, 0.694, 0.697,& 0.699, 0.701, 0.703, 0.706, 0.708, 0.710, 0.712, 0.714, 0.717,& 0.719, 0.721, 0.723, 0.725, 0.728, 0.730, 0.732, 0.734, 0.736,& 0.738, 0.741, 0.743, 0.745, 0.747, 0.749, 0.751, 0.753, 0.756,& 0.758, 0.760, 0.762, 0.764, 0.766, 0.768, 0.770, 0.772, 0.774,& 0.777, 0.779, 0.781, 0.783, 0.805, 0.825, 0.845, 0.864, 0.883,& 0.901, 0.920, 0.938, 0.955, 0.973, 0.990, 1.006, 1.023, 1.039,& 1.055, 1.071, 1.086, 1.101, 1.116, 1.131, 1.145, 1.160, 1.174,& 1.188, 1.201, 1.215, 1.228, 1.241, 1.254, 1.266, 1.279, 1.291,& 1.303, 1.315, 1.327, 1.339, 1.350, 1.361, 1.372, 1.383, 1.394,& 1.405, 1.416, 1.426, 1.436, 1.446, 1.456, 1.466, 1.476, 1.486,& 1.495, 1.505, 1.514, 1.523, 1.532, 1.541, 1.550, 1.559, 1.567,& 1.576, 1.584, 1.592, 1.601, 1.609, 1.617, 1.625, 1.632, 1.640,& 1.648, 1.655, 1.663, 1.670, 1.677, 1.684, 1.692, 1.699, 1.706,& 1.712, 1.719, 1.726, 1.732, 1.739, 1.746, 1.752, 1.758, 1.765,& 1.771, 1.777, 1.783, 1.789, 1.795, 1.801, 1.806, 1.812, 1.818,& 1.823, 1.829, 1.834, 1.840, 1.845, 1.850, 1.856, 1.861, 1.866,& 1.871, 1.876, 1.881, 1.886, 1.891, 1.896, 1.900, 1.905, 1.910,& 1.914, 1.919, 1.923, 1.928, 1.932, 1.937, 1.941, 1.945, 1.949,& 1.953, 1.958, 1.962, 1.966, 1.970, 1.974, 1.978, 1.981, 1.985,& 1.989, 1.993, 1.996, 2.000, 2.004, 2.007, 2.011, 2.014, 2.018,& 2.021, 2.025, 2.028, 2.031, 2.035, 2.038, 2.041, 2.044, 2.047,& 2.050, 2.053, 2.056, 2.059, 2.062, 2.065, 2.068, 2.071, 2.074,& 2.077, 2.080, 2.082 & / !C !C *** (H,NO3) !C DATA BNC10M/ & -0.048,-0.100,-0.123,-0.137,-0.147,-0.155,-0.161,-0.165,-0.169,& -0.172,-0.174,-0.175,-0.177,-0.177,-0.178,-0.178,-0.178,-0.177,& -0.177,-0.176,-0.175,-0.174,-0.173,-0.172,-0.171,-0.169,-0.168,& -0.166,-0.165,-0.163,-0.161,-0.159,-0.157,-0.156,-0.154,-0.152,& -0.150,-0.148,-0.146,-0.144,-0.141,-0.139,-0.137,-0.135,-0.133,& -0.131,-0.129,-0.127,-0.124,-0.122,-0.120,-0.118,-0.116,-0.113,& -0.111,-0.109,-0.107,-0.105,-0.102,-0.100,-0.098,-0.096,-0.094,& -0.091,-0.089,-0.087,-0.085,-0.082,-0.080,-0.078,-0.076,-0.073,& -0.071,-0.069,-0.067,-0.064,-0.062,-0.060,-0.057,-0.055,-0.052,& -0.050,-0.048,-0.045,-0.043,-0.040,-0.038,-0.035,-0.033,-0.030,& -0.027,-0.025,-0.022,-0.020,-0.017,-0.014,-0.012,-0.009,-0.006,& -0.004,-0.001, 0.002, 0.005, 0.007, 0.010, 0.013, 0.016, 0.019,& 0.021, 0.024, 0.027, 0.030, 0.033, 0.036, 0.039, 0.041, 0.044,& 0.047, 0.050, 0.053, 0.056, 0.059, 0.062, 0.065, 0.068, 0.071,& 0.073, 0.076, 0.079, 0.082, 0.085, 0.088, 0.091, 0.094, 0.097,& 0.100, 0.103, 0.105, 0.108, 0.111, 0.114, 0.117, 0.120, 0.123,& 0.126, 0.129, 0.131, 0.134, 0.137, 0.140, 0.143, 0.146, 0.149,& 0.152, 0.154, 0.157, 0.160, 0.163, 0.166, 0.169, 0.171, 0.174,& 0.177, 0.180, 0.183, 0.186, 0.188, 0.191, 0.194, 0.197, 0.200,& 0.202, 0.205, 0.208, 0.211, 0.213, 0.216, 0.219, 0.222, 0.224,& 0.227, 0.230, 0.233, 0.235, 0.238, 0.241, 0.244, 0.246, 0.249,& 0.252, 0.254, 0.257, 0.260, 0.263, 0.265, 0.268, 0.271, 0.273,& 0.276, 0.279, 0.281, 0.284, 0.287, 0.289, 0.292, 0.294, 0.297,& 0.300, 0.302, 0.305, 0.308, 0.310, 0.313, 0.315, 0.318, 0.321,& 0.323, 0.326, 0.328, 0.331, 0.333, 0.336, 0.339, 0.341, 0.344,& 0.346, 0.349, 0.351, 0.354, 0.356, 0.359, 0.361, 0.364, 0.366,& 0.369, 0.372, 0.374, 0.376, 0.379, 0.381, 0.384, 0.386, 0.389,& 0.391, 0.394, 0.396, 0.399, 0.401, 0.404, 0.406, 0.409, 0.411,& 0.413, 0.416, 0.418, 0.421, 0.423, 0.425, 0.428, 0.430, 0.433,& 0.435, 0.437, 0.440, 0.442, 0.445, 0.447, 0.449, 0.452, 0.454,& 0.456, 0.459, 0.461, 0.463, 0.466, 0.468, 0.470, 0.473, 0.475,& 0.477, 0.480, 0.482, 0.484, 0.486, 0.489, 0.491, 0.493, 0.496,& 0.498, 0.500, 0.502, 0.505, 0.507, 0.509, 0.511, 0.514, 0.516,& 0.518, 0.520, 0.523, 0.525, 0.527, 0.529, 0.531, 0.534, 0.536,& 0.538, 0.540, 0.542, 0.545, 0.547, 0.549, 0.551, 0.553, 0.555,& 0.558, 0.560, 0.562, 0.564, 0.566, 0.568, 0.570, 0.573, 0.575,& 0.577, 0.579, 0.581, 0.583, 0.585, 0.587, 0.590, 0.592, 0.594,& 0.596, 0.598, 0.600, 0.602, 0.604, 0.606, 0.608, 0.610, 0.612,& 0.614, 0.617, 0.619, 0.621, 0.623, 0.625, 0.627, 0.629, 0.631,& 0.633, 0.635, 0.637, 0.639, 0.641, 0.643, 0.645, 0.647, 0.649,& 0.651, 0.653, 0.655, 0.657, 0.659, 0.661, 0.663, 0.665, 0.667,& 0.669, 0.671, 0.673, 0.674, 0.676, 0.678, 0.680, 0.682, 0.684,& 0.686, 0.688, 0.690, 0.692, 0.694, 0.696, 0.698, 0.700, 0.701,& 0.703, 0.705, 0.707, 0.709, 0.711, 0.713, 0.715, 0.716, 0.718,& 0.720, 0.722, 0.724, 0.726, 0.746, 0.764, 0.781, 0.799, 0.816,& 0.833, 0.849, 0.866, 0.882, 0.897, 0.913, 0.928, 0.943, 0.958,& 0.972, 0.987, 1.001, 1.015, 1.028, 1.042, 1.055, 1.068, 1.081,& 1.093, 1.106, 1.118, 1.130, 1.142, 1.154, 1.165, 1.177, 1.188,& 1.199, 1.210, 1.221, 1.231, 1.242, 1.252, 1.262, 1.272, 1.282,& 1.292, 1.301, 1.311, 1.320, 1.329, 1.338, 1.347, 1.356, 1.365,& 1.374, 1.382, 1.391, 1.399, 1.407, 1.415, 1.423, 1.431, 1.439,& 1.446, 1.454, 1.462, 1.469, 1.476, 1.483, 1.491, 1.498, 1.505,& 1.511, 1.518, 1.525, 1.531, 1.538, 1.544, 1.551, 1.557, 1.563,& 1.569, 1.576, 1.582, 1.587, 1.593, 1.599, 1.605, 1.610, 1.616,& 1.622, 1.627, 1.632, 1.638, 1.643, 1.648, 1.653, 1.658, 1.663,& 1.668, 1.673, 1.678, 1.683, 1.688, 1.692, 1.697, 1.701, 1.706,& 1.710, 1.715, 1.719, 1.723, 1.728, 1.732, 1.736, 1.740, 1.744,& 1.748, 1.752, 1.756, 1.760, 1.764, 1.768, 1.771, 1.775, 1.779,& 1.782, 1.786, 1.789, 1.793, 1.796, 1.800, 1.803, 1.806, 1.810,& 1.813, 1.816, 1.819, 1.822, 1.825, 1.828, 1.831, 1.834, 1.837,& 1.840, 1.843, 1.846, 1.849, 1.852, 1.854, 1.857, 1.860, 1.862,& 1.865, 1.867, 1.870, 1.872, 1.875, 1.877, 1.880, 1.882, 1.885,& 1.887, 1.889, 1.891 & / !C !C *** (H,Cl) !C DATA BNC11M/ & -0.047,-0.093,-0.111,-0.121,-0.127,-0.131,-0.133,-0.134,-0.133,& -0.132,-0.131,-0.128,-0.126,-0.123,-0.119,-0.115,-0.111,-0.107,& -0.102,-0.098,-0.093,-0.088,-0.082,-0.077,-0.071,-0.065,-0.060,& -0.054,-0.048,-0.041,-0.035,-0.029,-0.022,-0.016,-0.009,-0.003,& 0.004, 0.011, 0.018, 0.025, 0.032, 0.038, 0.045, 0.053, 0.060,& 0.067, 0.074, 0.081, 0.088, 0.095, 0.103, 0.110, 0.117, 0.124,& 0.132, 0.139, 0.146, 0.154, 0.161, 0.168, 0.176, 0.183, 0.191,& 0.198, 0.206, 0.213, 0.221, 0.228, 0.236, 0.243, 0.251, 0.258,& 0.266, 0.274, 0.281, 0.289, 0.297, 0.305, 0.312, 0.320, 0.328,& 0.336, 0.344, 0.352, 0.360, 0.368, 0.376, 0.384, 0.393, 0.401,& 0.409, 0.417, 0.426, 0.434, 0.443, 0.451, 0.460, 0.468, 0.477,& 0.485, 0.494, 0.503, 0.511, 0.520, 0.529, 0.538, 0.546, 0.555,& 0.564, 0.573, 0.582, 0.591, 0.600, 0.608, 0.617, 0.626, 0.635,& 0.644, 0.653, 0.662, 0.671, 0.680, 0.689, 0.698, 0.707, 0.716,& 0.725, 0.734, 0.743, 0.752, 0.761, 0.770, 0.779, 0.788, 0.796,& 0.805, 0.814, 0.823, 0.832, 0.841, 0.850, 0.859, 0.867, 0.876,& 0.885, 0.894, 0.903, 0.911, 0.920, 0.929, 0.937, 0.946, 0.955,& 0.964, 0.972, 0.981, 0.989, 0.998, 1.007, 1.015, 1.024, 1.032,& 1.041, 1.049, 1.058, 1.066, 1.075, 1.083, 1.092, 1.100, 1.109,& 1.117, 1.125, 1.134, 1.142, 1.150, 1.159, 1.167, 1.175, 1.183,& 1.192, 1.200, 1.208, 1.216, 1.224, 1.233, 1.241, 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1.075, 1.081, 1.086, 1.092, 1.098, 1.103, 1.109,& 1.114, 1.120, 1.125, 1.131, 1.136, 1.142, 1.148, 1.153, 1.159,& 1.164, 1.169, 1.175, 1.180, 1.186, 1.191, 1.197, 1.202, 1.208,& 1.213, 1.218, 1.224, 1.229, 1.234, 1.240, 1.245, 1.250, 1.256,& 1.261, 1.266, 1.272, 1.277, 1.282, 1.287, 1.293, 1.298, 1.303,& 1.308, 1.314, 1.319, 1.324, 1.329, 1.334, 1.339, 1.345, 1.350,& 1.355, 1.360, 1.365, 1.370, 1.375, 1.380, 1.385, 1.390, 1.396,& 1.401, 1.406, 1.411, 1.416, 1.421, 1.426, 1.431, 1.436, 1.441,& 1.446, 1.451, 1.456, 1.460, 1.465, 1.470, 1.475, 1.480, 1.485,& 1.490, 1.495, 1.500, 1.504, 1.509, 1.514, 1.519, 1.524, 1.529,& 1.533, 1.538, 1.543, 1.548, 1.553, 1.557, 1.562, 1.567, 1.572,& 1.576, 1.581, 1.586, 1.590, 1.595, 1.600, 1.604, 1.609, 1.614,& 1.618, 1.623, 1.628, 1.632, 1.637, 1.642, 1.646, 1.651, 1.655,& 1.660, 1.664, 1.669, 1.674, 1.678, 1.683, 1.687, 1.692, 1.696,& 1.701, 1.705, 1.710, 1.714, 1.719, 1.723, 1.728, 1.732, 1.736,& 1.741, 1.745, 1.750, 1.754, 1.759, 1.763, 1.767, 1.772, 1.776,& 1.780, 1.785, 1.789, 1.793, 1.840, 1.882, 1.923, 1.964, 2.004,& 2.044, 2.082, 2.120, 2.158, 2.195, 2.231, 2.267, 2.302, 2.336,& 2.370, 2.404, 2.437, 2.469, 2.501, 2.533, 2.564, 2.594, 2.624,& 2.654, 2.683, 2.712, 2.741, 2.768, 2.796, 2.823, 2.850, 2.877,& 2.903, 2.928, 2.954, 2.979, 3.003, 3.028, 3.052, 3.076, 3.099,& 3.122, 3.145, 3.167, 3.190, 3.211, 3.233, 3.254, 3.276, 3.296,& 3.317, 3.337, 3.357, 3.377, 3.397, 3.416, 3.435, 3.454, 3.473,& 3.491, 3.509, 3.527, 3.545, 3.563, 3.580, 3.597, 3.614, 3.631,& 3.647, 3.664, 3.680, 3.696, 3.712, 3.727, 3.743, 3.758, 3.773,& 3.788, 3.803, 3.817, 3.832, 3.846, 3.860, 3.874, 3.888, 3.902,& 3.915, 3.928, 3.942, 3.955, 3.968, 3.980, 3.993, 4.006, 4.018,& 4.030, 4.042, 4.054, 4.066, 4.078, 4.089, 4.101, 4.112, 4.123,& 4.134, 4.145, 4.156, 4.167, 4.178, 4.188, 4.199, 4.209, 4.219,& 4.229, 4.239, 4.249, 4.259, 4.269, 4.278, 4.288, 4.297, 4.306,& 4.316, 4.325, 4.334, 4.343, 4.351, 4.360, 4.369, 4.377, 4.386,& 4.394, 4.402, 4.411, 4.419, 4.427, 4.435, 4.442, 4.450, 4.458,& 4.466, 4.473, 4.480, 4.488, 4.495, 4.502, 4.510, 4.517, 4.524,& 4.531, 4.537, 4.544, 4.551, 4.558, 4.564, 4.571, 4.577, 4.583,& 4.590, 4.596, 4.602 & / END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KM248 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IN' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C TEMPERATURE IS 248K !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KM2482p1 (IONIC, BINARR) !C !C *** Common block definition !C COMMON /KMC2482p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) REAL Binarr (23), Ionic !C !C *** Find position in arrays for bincoef !C IF (Ionic.LE. 0.200000E+02) THEN ipos = MIN(NINT( 0.200000E+02*Ionic) + 1, 400) ELSE ipos = 400+NINT( 0.200000E+01*Ionic- 0.400000E+02) ENDIF ipos = min(ipos, 561) !C !C *** Assign values to return array !C Binarr(01) = BNC01M(ipos) Binarr(02) = BNC02M(ipos) Binarr(03) = BNC03M(ipos) Binarr(04) = BNC04M(ipos) Binarr(05) = BNC05M(ipos) Binarr(06) = BNC06M(ipos) Binarr(07) = BNC07M(ipos) Binarr(08) = BNC08M(ipos) Binarr(09) = BNC09M(ipos) Binarr(10) = BNC10M(ipos) Binarr(11) = BNC11M(ipos) Binarr(12) = BNC12M(ipos) Binarr(13) = BNC13M(ipos) Binarr(14) = BNC14M(ipos) Binarr(15) = BNC15M(ipos) Binarr(16) = BNC16M(ipos) Binarr(17) = BNC17M(ipos) Binarr(18) = BNC18M(ipos) Binarr(19) = BNC19M(ipos) Binarr(20) = BNC20M(ipos) Binarr(21) = BNC21M(ipos) Binarr(22) = BNC22M(ipos) Binarr(23) = BNC23M(ipos) !C !C *** Return point ; End of subroutine !C RETURN END BLOCK DATA KMCF2482p1 !C !C *** Common block definition !C COMMON /KMC2482p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) !C !C *** NaCl !C DATA BNC01M/ & -0.047,-0.099,-0.122,-0.137,-0.148,-0.156,-0.163,-0.168,-0.172,& -0.176,-0.178,-0.181,-0.182,-0.184,-0.185,-0.186,-0.186,-0.187,& -0.187,-0.187,-0.187,-0.187,-0.186,-0.186,-0.185,-0.184,-0.184,& -0.183,-0.182,-0.181,-0.180,-0.179,-0.178,-0.176,-0.175,-0.174,& -0.173,-0.171,-0.170,-0.168,-0.167,-0.166,-0.164,-0.163,-0.161,& -0.160,-0.158,-0.157,-0.155,-0.154,-0.152,-0.151,-0.149,-0.148,& -0.146,-0.145,-0.143,-0.141,-0.140,-0.138,-0.137,-0.135,-0.134,& -0.132,-0.130,-0.129,-0.127,-0.126,-0.124,-0.122,-0.121,-0.119,& -0.117,-0.116,-0.114,-0.112,-0.111,-0.109,-0.107,-0.105,-0.104,& -0.102,-0.100,-0.098,-0.096,-0.095,-0.093,-0.091,-0.089,-0.087,& -0.085,-0.083,-0.081,-0.079,-0.077,-0.075,-0.073,-0.071,-0.069,& -0.067,-0.065,-0.063,-0.061,-0.059,-0.057,-0.055,-0.053,-0.051,& -0.048,-0.046,-0.044,-0.042,-0.040,-0.038,-0.036,-0.033,-0.031,& -0.029,-0.027,-0.025,-0.022,-0.020,-0.018,-0.016,-0.014,-0.011,& -0.009,-0.007,-0.005,-0.003, 0.000, 0.002, 0.004, 0.006, 0.008,& 0.011, 0.013, 0.015, 0.017, 0.020, 0.022, 0.024, 0.026, 0.028,& 0.030, 0.033, 0.035, 0.037, 0.039, 0.041, 0.044, 0.046, 0.048,& 0.050, 0.052, 0.054, 0.057, 0.059, 0.061, 0.063, 0.065, 0.067,& 0.070, 0.072, 0.074, 0.076, 0.078, 0.080, 0.082, 0.085, 0.087,& 0.089, 0.091, 0.093, 0.095, 0.097, 0.099, 0.102, 0.104, 0.106,& 0.108, 0.110, 0.112, 0.114, 0.116, 0.118, 0.120, 0.122, 0.125,& 0.127, 0.129, 0.131, 0.133, 0.135, 0.137, 0.139, 0.141, 0.143,& 0.145, 0.147, 0.149, 0.151, 0.153, 0.155, 0.157, 0.159, 0.161,& 0.163, 0.165, 0.167, 0.169, 0.171, 0.173, 0.175, 0.177, 0.179,& 0.181, 0.183, 0.185, 0.187, 0.189, 0.191, 0.193, 0.195, 0.197,& 0.199, 0.201, 0.203, 0.205, 0.207, 0.209, 0.211, 0.213, 0.215,& 0.217, 0.219, 0.221, 0.223, 0.224, 0.226, 0.228, 0.230, 0.232,& 0.234, 0.236, 0.238, 0.240, 0.242, 0.243, 0.245, 0.247, 0.249,& 0.251, 0.253, 0.255, 0.257, 0.258, 0.260, 0.262, 0.264, 0.266,& 0.268, 0.270, 0.271, 0.273, 0.275, 0.277, 0.279, 0.281, 0.282,& 0.284, 0.286, 0.288, 0.290, 0.291, 0.293, 0.295, 0.297, 0.299,& 0.300, 0.302, 0.304, 0.306, 0.308, 0.309, 0.311, 0.313, 0.315,& 0.316, 0.318, 0.320, 0.322, 0.323, 0.325, 0.327, 0.329, 0.330,& 0.332, 0.334, 0.336, 0.337, 0.339, 0.341, 0.342, 0.344, 0.346,& 0.348, 0.349, 0.351, 0.353, 0.354, 0.356, 0.358, 0.359, 0.361,& 0.363, 0.364, 0.366, 0.368, 0.370, 0.371, 0.373, 0.374, 0.376,& 0.378, 0.379, 0.381, 0.383, 0.384, 0.386, 0.388, 0.389, 0.391,& 0.393, 0.394, 0.396, 0.397, 0.399, 0.401, 0.402, 0.404, 0.406,& 0.407, 0.409, 0.410, 0.412, 0.414, 0.415, 0.417, 0.418, 0.420,& 0.421, 0.423, 0.425, 0.426, 0.428, 0.429, 0.431, 0.433, 0.434,& 0.436, 0.437, 0.439, 0.440, 0.442, 0.443, 0.445, 0.446, 0.448,& 0.450, 0.451, 0.453, 0.454, 0.456, 0.457, 0.459, 0.460, 0.462,& 0.463, 0.465, 0.466, 0.468, 0.469, 0.471, 0.472, 0.474, 0.475,& 0.477, 0.478, 0.480, 0.481, 0.483, 0.484, 0.486, 0.487, 0.489,& 0.490, 0.491, 0.493, 0.494, 0.510, 0.524, 0.538, 0.552, 0.566,& 0.579, 0.592, 0.605, 0.618, 0.630, 0.642, 0.655, 0.667, 0.678,& 0.690, 0.701, 0.713, 0.724, 0.735, 0.745, 0.756, 0.766, 0.777,& 0.787, 0.797, 0.807, 0.817, 0.826, 0.836, 0.845, 0.854, 0.864,& 0.873, 0.881, 0.890, 0.899, 0.907, 0.916, 0.924, 0.932, 0.940,& 0.948, 0.956, 0.964, 0.972, 0.979, 0.987, 0.994, 1.002, 1.009,& 1.016, 1.023, 1.030, 1.037, 1.044, 1.051, 1.057, 1.064, 1.070,& 1.077, 1.083, 1.089, 1.096, 1.102, 1.108, 1.114, 1.120, 1.126,& 1.132, 1.137, 1.143, 1.149, 1.154, 1.160, 1.165, 1.170, 1.176,& 1.181, 1.186, 1.191, 1.196, 1.201, 1.206, 1.211, 1.216, 1.221,& 1.226, 1.231, 1.235, 1.240, 1.244, 1.249, 1.253, 1.258, 1.262,& 1.267, 1.271, 1.275, 1.279, 1.284, 1.288, 1.292, 1.296, 1.300,& 1.304, 1.308, 1.312, 1.315, 1.319, 1.323, 1.327, 1.330, 1.334,& 1.338, 1.341, 1.345, 1.348, 1.352, 1.355, 1.358, 1.362, 1.365,& 1.368, 1.372, 1.375, 1.378, 1.381, 1.384, 1.388, 1.391, 1.394,& 1.397, 1.400, 1.403, 1.406, 1.409, 1.411, 1.414, 1.417, 1.420,& 1.423, 1.425, 1.428, 1.431, 1.433, 1.436, 1.439, 1.441, 1.444,& 1.446, 1.449, 1.451, 1.454, 1.456, 1.458, 1.461, 1.463, 1.466,& 1.468, 1.470, 1.472 & / !C !C *** Na2SO4 !C DATA BNC02M/ & -0.098,-0.214,-0.272,-0.313,-0.346,-0.373,-0.396,-0.417,-0.435,& -0.452,-0.467,-0.481,-0.494,-0.506,-0.518,-0.529,-0.539,-0.549,& -0.558,-0.567,-0.575,-0.583,-0.591,-0.599,-0.606,-0.613,-0.620,& -0.627,-0.633,-0.639,-0.645,-0.651,-0.657,-0.662,-0.668,-0.673,& -0.678,-0.683,-0.688,-0.693,-0.698,-0.703,-0.707,-0.712,-0.716,& -0.721,-0.725,-0.729,-0.733,-0.737,-0.741,-0.745,-0.749,-0.753,& -0.756,-0.760,-0.764,-0.767,-0.771,-0.774,-0.778,-0.781,-0.784,& -0.788,-0.791,-0.794,-0.797,-0.801,-0.804,-0.807,-0.810,-0.813,& -0.816,-0.819,-0.822,-0.825,-0.827,-0.830,-0.833,-0.836,-0.839,& -0.841,-0.844,-0.847,-0.850,-0.852,-0.855,-0.858,-0.860,-0.863,& -0.865,-0.868,-0.871,-0.873,-0.876,-0.878,-0.881,-0.883,-0.885,& -0.888,-0.890,-0.893,-0.895,-0.897,-0.900,-0.902,-0.905,-0.907,& -0.909,-0.911,-0.914,-0.916,-0.918,-0.921,-0.923,-0.925,-0.927,& -0.929,-0.932,-0.934,-0.936,-0.938,-0.940,-0.942,-0.945,-0.947,& -0.949,-0.951,-0.953,-0.955,-0.957,-0.959,-0.961,-0.963,-0.965,& -0.967,-0.969,-0.971,-0.973,-0.975,-0.977,-0.979,-0.981,-0.983,& -0.985,-0.987,-0.989,-0.991,-0.993,-0.995,-0.997,-0.999,-1.001,& -1.002,-1.004,-1.006,-1.008,-1.010,-1.012,-1.014,-1.015,-1.017,& -1.019,-1.021,-1.023,-1.025,-1.026,-1.028,-1.030,-1.032,-1.033,& -1.035,-1.037,-1.039,-1.040,-1.042,-1.044,-1.046,-1.047,-1.049,& -1.051,-1.053,-1.054,-1.056,-1.058,-1.059,-1.061,-1.063,-1.064,& -1.066,-1.068,-1.069,-1.071,-1.073,-1.074,-1.076,-1.078,-1.079,& -1.081,-1.082,-1.084,-1.086,-1.087,-1.089,-1.090,-1.092,-1.094,& -1.095,-1.097,-1.098,-1.100,-1.102,-1.103,-1.105,-1.106,-1.108,& -1.109,-1.111,-1.112,-1.114,-1.116,-1.117,-1.119,-1.120,-1.122,& -1.123,-1.125,-1.126,-1.128,-1.129,-1.131,-1.132,-1.134,-1.135,& 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3.074, 3.081, 3.088, 3.095,& 3.103, 3.110, 3.117, 3.125, 3.132, 3.139, 3.146, 3.153, 3.161,& 3.168, 3.175, 3.182, 3.189, 3.196, 3.203, 3.210, 3.217, 3.225,& 3.232, 3.239, 3.246, 3.253, 3.260, 3.267, 3.274, 3.281, 3.288,& 3.294, 3.301, 3.308, 3.315, 3.322, 3.329, 3.336, 3.343, 3.350,& 3.356, 3.363, 3.370, 3.377, 3.450, 3.516, 3.581, 3.645, 3.708,& 3.770, 3.831, 3.891, 3.950, 4.008, 4.065, 4.122, 4.178, 4.233,& 4.287, 4.340, 4.393, 4.445, 4.496, 4.547, 4.597, 4.646, 4.695,& 4.743, 4.790, 4.837, 4.884, 4.929, 4.974, 5.019, 5.063, 5.107,& 5.150, 5.193, 5.235, 5.277, 5.318, 5.359, 5.399, 5.439, 5.478,& 5.517, 5.556, 5.594, 5.632, 5.670, 5.707, 5.743, 5.780, 5.816,& 5.852, 5.887, 5.922, 5.956, 5.991, 6.025, 6.058, 6.092, 6.125,& 6.158, 6.190, 6.222, 6.254, 6.286, 6.317, 6.348, 6.379, 6.410,& 6.440, 6.470, 6.500, 6.529, 6.559, 6.588, 6.616, 6.645, 6.673,& 6.701, 6.729, 6.757, 6.784, 6.812, 6.839, 6.865, 6.892, 6.919,& 6.945, 6.971, 6.997, 7.022, 7.048, 7.073, 7.098, 7.123, 7.148,& 7.172, 7.196, 7.221, 7.245, 7.269, 7.292, 7.316, 7.339, 7.362,& 7.385, 7.408, 7.431, 7.454, 7.476, 7.498, 7.520, 7.542, 7.564,& 7.586, 7.607, 7.629, 7.650, 7.671, 7.692, 7.713, 7.734, 7.755,& 7.775, 7.795, 7.816, 7.836, 7.856, 7.876, 7.895, 7.915, 7.935,& 7.954, 7.973, 7.992, 8.012, 8.030, 8.049, 8.068, 8.087, 8.105,& 8.124, 8.142, 8.160, 8.178, 8.196, 8.214, 8.232, 8.250, 8.267,& 8.285, 8.302, 8.319, 8.337, 8.354, 8.371, 8.388, 8.404, 8.421,& 8.438, 8.454, 8.471 & / !C !C *** NH4HSO4 !C DATA BNC09M/ & -0.048,-0.102,-0.128,-0.146,-0.159,-0.170,-0.179,-0.187,-0.194,& -0.200,-0.205,-0.210,-0.214,-0.218,-0.221,-0.224,-0.227,-0.230,& -0.232,-0.234,-0.235,-0.237,-0.238,-0.239,-0.240,-0.241,-0.242,& -0.242,-0.243,-0.243,-0.243,-0.243,-0.243,-0.243,-0.242,-0.242,& -0.241,-0.241,-0.240,-0.239,-0.238,-0.237,-0.236,-0.235,-0.234,& -0.233,-0.231,-0.230,-0.228,-0.227,-0.225,-0.224,-0.222,-0.220,& -0.218,-0.216,-0.214,-0.212,-0.210,-0.208,-0.206,-0.204,-0.202,& -0.199,-0.197,-0.195,-0.192,-0.190,-0.188,-0.185,-0.183,-0.180,& -0.178,-0.175,-0.172,-0.170,-0.167,-0.164,-0.161,-0.159,-0.156,& -0.153,-0.150,-0.147,-0.144,-0.141,-0.138,-0.135,-0.132,-0.129,& -0.126,-0.123,-0.119,-0.116,-0.113,-0.110,-0.106,-0.103,-0.100,& -0.096,-0.093,-0.090,-0.086,-0.083,-0.080,-0.076,-0.073,-0.069,& -0.066,-0.062,-0.059,-0.055,-0.052,-0.048,-0.045,-0.041,-0.037,& -0.034,-0.030,-0.027,-0.023,-0.020,-0.016,-0.012,-0.009,-0.005,& -0.002, 0.002, 0.005, 0.009, 0.013, 0.016, 0.020, 0.023, 0.027,& 0.030, 0.034, 0.037, 0.041, 0.044, 0.048, 0.051, 0.055, 0.058,& 0.062, 0.065, 0.069, 0.072, 0.076, 0.079, 0.083, 0.086, 0.090,& 0.093, 0.097, 0.100, 0.103, 0.107, 0.110, 0.114, 0.117, 0.120,& 0.124, 0.127, 0.130, 0.134, 0.137, 0.140, 0.144, 0.147, 0.150,& 0.154, 0.157, 0.160, 0.164, 0.167, 0.170, 0.173, 0.177, 0.180,& 0.183, 0.186, 0.189, 0.193, 0.196, 0.199, 0.202, 0.205, 0.209,& 0.212, 0.215, 0.218, 0.221, 0.224, 0.227, 0.231, 0.234, 0.237,& 0.240, 0.243, 0.246, 0.249, 0.252, 0.255, 0.258, 0.261, 0.264,& 0.267, 0.270, 0.273, 0.276, 0.279, 0.282, 0.285, 0.288, 0.291,& 0.294, 0.297, 0.300, 0.303, 0.306, 0.309, 0.312, 0.315, 0.317,& 0.320, 0.323, 0.326, 0.329, 0.332, 0.335, 0.338, 0.340, 0.343,& 0.346, 0.349, 0.352, 0.354, 0.357, 0.360, 0.363, 0.366, 0.368,& 0.371, 0.374, 0.377, 0.379, 0.382, 0.385, 0.388, 0.390, 0.393,& 0.396, 0.398, 0.401, 0.404, 0.407, 0.409, 0.412, 0.415, 0.417,& 0.420, 0.422, 0.425, 0.428, 0.430, 0.433, 0.436, 0.438, 0.441,& 0.443, 0.446, 0.449, 0.451, 0.454, 0.456, 0.459, 0.461, 0.464,& 0.467, 0.469, 0.472, 0.474, 0.477, 0.479, 0.482, 0.484, 0.487,& 0.489, 0.492, 0.494, 0.497, 0.499, 0.502, 0.504, 0.507, 0.509,& 0.511, 0.514, 0.516, 0.519, 0.521, 0.524, 0.526, 0.528, 0.531,& 0.533, 0.536, 0.538, 0.540, 0.543, 0.545, 0.548, 0.550, 0.552,& 0.555, 0.557, 0.559, 0.562, 0.564, 0.566, 0.569, 0.571, 0.573,& 0.576, 0.578, 0.580, 0.583, 0.585, 0.587, 0.589, 0.592, 0.594,& 0.596, 0.599, 0.601, 0.603, 0.605, 0.608, 0.610, 0.612, 0.614,& 0.617, 0.619, 0.621, 0.623, 0.625, 0.628, 0.630, 0.632, 0.634,& 0.636, 0.639, 0.641, 0.643, 0.645, 0.647, 0.649, 0.652, 0.654,& 0.656, 0.658, 0.660, 0.662, 0.665, 0.667, 0.669, 0.671, 0.673,& 0.675, 0.677, 0.679, 0.681, 0.684, 0.686, 0.688, 0.690, 0.692,& 0.694, 0.696, 0.698, 0.700, 0.702, 0.704, 0.706, 0.708, 0.710,& 0.713, 0.715, 0.717, 0.719, 0.721, 0.723, 0.725, 0.727, 0.729,& 0.731, 0.733, 0.735, 0.737, 0.758, 0.778, 0.797, 0.815, 0.834,& 0.852, 0.870, 0.887, 0.905, 0.922, 0.938, 0.955, 0.971, 0.987,& 1.003, 1.018, 1.033, 1.048, 1.063, 1.078, 1.092, 1.106, 1.120,& 1.134, 1.148, 1.161, 1.174, 1.187, 1.200, 1.213, 1.225, 1.238,& 1.250, 1.262, 1.274, 1.286, 1.297, 1.309, 1.320, 1.331, 1.342,& 1.353, 1.364, 1.374, 1.385, 1.395, 1.406, 1.416, 1.426, 1.436,& 1.446, 1.455, 1.465, 1.475, 1.484, 1.493, 1.502, 1.512, 1.521,& 1.529, 1.538, 1.547, 1.556, 1.564, 1.572, 1.581, 1.589, 1.597,& 1.605, 1.613, 1.621, 1.629, 1.637, 1.645, 1.652, 1.660, 1.667,& 1.675, 1.682, 1.689, 1.696, 1.704, 1.711, 1.718, 1.725, 1.731,& 1.738, 1.745, 1.752, 1.758, 1.765, 1.771, 1.778, 1.784, 1.790,& 1.796, 1.803, 1.809, 1.815, 1.821, 1.827, 1.833, 1.839, 1.844,& 1.850, 1.856, 1.861, 1.867, 1.873, 1.878, 1.884, 1.889, 1.894,& 1.900, 1.905, 1.910, 1.915, 1.920, 1.926, 1.931, 1.936, 1.941,& 1.946, 1.950, 1.955, 1.960, 1.965, 1.970, 1.974, 1.979, 1.983,& 1.988, 1.993, 1.997, 2.001, 2.006, 2.010, 2.015, 2.019, 2.023,& 2.027, 2.032, 2.036, 2.040, 2.044, 2.048, 2.052, 2.056, 2.060,& 2.064, 2.068, 2.072, 2.076, 2.080, 2.083, 2.087, 2.091, 2.095,& 2.098, 2.102, 2.106 & / !C !C *** (H,NO3) !C DATA BNC10M/ & -0.047,-0.098,-0.120,-0.135,-0.145,-0.153,-0.158,-0.163,-0.167,& -0.169,-0.172,-0.173,-0.175,-0.176,-0.176,-0.176,-0.176,-0.176,& -0.176,-0.175,-0.175,-0.174,-0.173,-0.172,-0.170,-0.169,-0.168,& -0.166,-0.165,-0.163,-0.162,-0.160,-0.159,-0.157,-0.155,-0.153,& -0.151,-0.149,-0.148,-0.146,-0.144,-0.142,-0.140,-0.138,-0.136,& -0.134,-0.132,-0.130,-0.128,-0.126,-0.124,-0.122,-0.120,-0.118,& -0.115,-0.113,-0.111,-0.109,-0.107,-0.105,-0.103,-0.101,-0.099,& -0.097,-0.095,-0.093,-0.090,-0.088,-0.086,-0.084,-0.082,-0.080,& -0.078,-0.075,-0.073,-0.071,-0.069,-0.067,-0.064,-0.062,-0.060,& -0.057,-0.055,-0.053,-0.051,-0.048,-0.046,-0.043,-0.041,-0.039,& -0.036,-0.034,-0.031,-0.029,-0.026,-0.024,-0.021,-0.019,-0.016,& -0.014,-0.011,-0.008,-0.006,-0.003, 0.000, 0.002, 0.005, 0.007,& 0.010, 0.013, 0.016, 0.018, 0.021, 0.024, 0.026, 0.029, 0.032,& 0.035, 0.037, 0.040, 0.043, 0.046, 0.048, 0.051, 0.054, 0.057,& 0.059, 0.062, 0.065, 0.068, 0.070, 0.073, 0.076, 0.079, 0.081,& 0.084, 0.087, 0.090, 0.092, 0.095, 0.098, 0.101, 0.103, 0.106,& 0.109, 0.112, 0.114, 0.117, 0.120, 0.123, 0.125, 0.128, 0.131,& 0.133, 0.136, 0.139, 0.142, 0.144, 0.147, 0.150, 0.152, 0.155,& 0.158, 0.160, 0.163, 0.166, 0.168, 0.171, 0.174, 0.176, 0.179,& 0.182, 0.184, 0.187, 0.190, 0.192, 0.195, 0.198, 0.200, 0.203,& 0.205, 0.208, 0.211, 0.213, 0.216, 0.218, 0.221, 0.224, 0.226,& 0.229, 0.231, 0.234, 0.236, 0.239, 0.242, 0.244, 0.247, 0.249,& 0.252, 0.254, 0.257, 0.259, 0.262, 0.264, 0.267, 0.269, 0.272,& 0.275, 0.277, 0.280, 0.282, 0.285, 0.287, 0.289, 0.292, 0.294,& 0.297, 0.299, 0.302, 0.304, 0.307, 0.309, 0.312, 0.314, 0.317,& 0.319, 0.321, 0.324, 0.326, 0.329, 0.331, 0.334, 0.336, 0.338,& 0.341, 0.343, 0.346, 0.348, 0.350, 0.353, 0.355, 0.357, 0.360,& 0.362, 0.364, 0.367, 0.369, 0.372, 0.374, 0.376, 0.379, 0.381,& 0.383, 0.386, 0.388, 0.390, 0.392, 0.395, 0.397, 0.399, 0.402,& 0.404, 0.406, 0.409, 0.411, 0.413, 0.415, 0.418, 0.420, 0.422,& 0.424, 0.427, 0.429, 0.431, 0.433, 0.436, 0.438, 0.440, 0.442,& 0.445, 0.447, 0.449, 0.451, 0.453, 0.456, 0.458, 0.460, 0.462,& 0.464, 0.467, 0.469, 0.471, 0.473, 0.475, 0.477, 0.480, 0.482,& 0.484, 0.486, 0.488, 0.490, 0.492, 0.495, 0.497, 0.499, 0.501,& 0.503, 0.505, 0.507, 0.509, 0.511, 0.514, 0.516, 0.518, 0.520,& 0.522, 0.524, 0.526, 0.528, 0.530, 0.532, 0.534, 0.536, 0.539,& 0.541, 0.543, 0.545, 0.547, 0.549, 0.551, 0.553, 0.555, 0.557,& 0.559, 0.561, 0.563, 0.565, 0.567, 0.569, 0.571, 0.573, 0.575,& 0.577, 0.579, 0.581, 0.583, 0.585, 0.587, 0.589, 0.591, 0.593,& 0.595, 0.597, 0.599, 0.601, 0.603, 0.604, 0.606, 0.608, 0.610,& 0.612, 0.614, 0.616, 0.618, 0.620, 0.622, 0.624, 0.626, 0.628,& 0.629, 0.631, 0.633, 0.635, 0.637, 0.639, 0.641, 0.643, 0.645,& 0.646, 0.648, 0.650, 0.652, 0.654, 0.656, 0.658, 0.659, 0.661,& 0.663, 0.665, 0.667, 0.669, 0.671, 0.672, 0.674, 0.676, 0.678,& 0.680, 0.681, 0.683, 0.685, 0.704, 0.722, 0.739, 0.756, 0.773,& 0.790, 0.806, 0.822, 0.838, 0.853, 0.869, 0.884, 0.899, 0.913,& 0.928, 0.942, 0.956, 0.970, 0.983, 0.996, 1.010, 1.023, 1.036,& 1.048, 1.061, 1.073, 1.085, 1.097, 1.109, 1.121, 1.132, 1.144,& 1.155, 1.166, 1.177, 1.188, 1.198, 1.209, 1.219, 1.230, 1.240,& 1.250, 1.260, 1.270, 1.279, 1.289, 1.298, 1.308, 1.317, 1.326,& 1.335, 1.344, 1.353, 1.362, 1.370, 1.379, 1.387, 1.396, 1.404,& 1.412, 1.420, 1.428, 1.436, 1.444, 1.451, 1.459, 1.467, 1.474,& 1.481, 1.489, 1.496, 1.503, 1.510, 1.517, 1.524, 1.531, 1.538,& 1.545, 1.551, 1.558, 1.565, 1.571, 1.578, 1.584, 1.590, 1.596,& 1.603, 1.609, 1.615, 1.621, 1.627, 1.632, 1.638, 1.644, 1.650,& 1.655, 1.661, 1.667, 1.672, 1.678, 1.683, 1.688, 1.694, 1.699,& 1.704, 1.709, 1.714, 1.719, 1.724, 1.729, 1.734, 1.739, 1.744,& 1.749, 1.753, 1.758, 1.763, 1.767, 1.772, 1.776, 1.781, 1.785,& 1.790, 1.794, 1.799, 1.803, 1.807, 1.811, 1.815, 1.820, 1.824,& 1.828, 1.832, 1.836, 1.840, 1.844, 1.848, 1.852, 1.855, 1.859,& 1.863, 1.867, 1.870, 1.874, 1.878, 1.881, 1.885, 1.888, 1.892,& 1.895, 1.899, 1.902, 1.906, 1.909, 1.913, 1.916, 1.919, 1.922,& 1.926, 1.929, 1.932 & / !C !C *** (H,Cl) !C DATA BNC11M/ & -0.046,-0.091,-0.110,-0.120,-0.127,-0.131,-0.133,-0.134,-0.134,& -0.134,-0.132,-0.131,-0.128,-0.126,-0.123,-0.120,-0.116,-0.112,& -0.108,-0.104,-0.099,-0.095,-0.090,-0.085,-0.080,-0.075,-0.070,& -0.064,-0.059,-0.053,-0.047,-0.042,-0.036,-0.030,-0.024,-0.018,& -0.011,-0.005, 0.001, 0.007, 0.014, 0.020, 0.026, 0.033, 0.039,& 0.046, 0.052, 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0.127, 0.133, 0.140, 0.146, 0.152, 0.159, 0.165,& 0.171, 0.178, 0.184, 0.191, 0.197, 0.203, 0.210, 0.216, 0.223,& 0.229, 0.236, 0.242, 0.249, 0.255, 0.261, 0.268, 0.274, 0.281,& 0.287, 0.293, 0.300, 0.306, 0.313, 0.319, 0.325, 0.332, 0.338,& 0.345, 0.351, 0.357, 0.364, 0.370, 0.376, 0.383, 0.389, 0.395,& 0.402, 0.408, 0.414, 0.421, 0.427, 0.433, 0.439, 0.446, 0.452,& 0.458, 0.464, 0.471, 0.477, 0.483, 0.489, 0.495, 0.502, 0.508,& 0.514, 0.520, 0.526, 0.532, 0.538, 0.545, 0.551, 0.557, 0.563,& 0.569, 0.575, 0.581, 0.587, 0.593, 0.599, 0.605, 0.611, 0.617,& 0.623, 0.629, 0.635, 0.641, 0.647, 0.653, 0.659, 0.665, 0.671,& 0.677, 0.683, 0.689, 0.694, 0.700, 0.706, 0.712, 0.718, 0.724,& 0.730, 0.735, 0.741, 0.747, 0.753, 0.759, 0.764, 0.770, 0.776,& 0.782, 0.787, 0.793, 0.799, 0.804, 0.810, 0.816, 0.822, 0.827,& 0.833, 0.838, 0.844, 0.850, 0.855, 0.861, 0.867, 0.872, 0.878,& 0.883, 0.889, 0.894, 0.900, 0.905, 0.911, 0.916, 0.922, 0.927,& 0.933, 0.938, 0.944, 0.949, 0.955, 0.960, 0.966, 0.971, 0.976,& 0.982, 0.987, 0.993, 0.998, 1.003, 1.009, 1.014, 1.019, 1.025,& 1.030, 1.035, 1.041, 1.046, 1.051, 1.056, 1.062, 1.067, 1.072,& 1.077, 1.083, 1.088, 1.093, 1.098, 1.103, 1.109, 1.114, 1.119,& 1.124, 1.129, 1.134, 1.139, 1.144, 1.150, 1.155, 1.160, 1.165,& 1.170, 1.175, 1.180, 1.185, 1.190, 1.195, 1.200, 1.205, 1.210,& 1.215, 1.220, 1.225, 1.230, 1.235, 1.240, 1.245, 1.250, 1.255,& 1.260, 1.264, 1.269, 1.274, 1.279, 1.284, 1.289, 1.294, 1.299,& 1.303, 1.308, 1.313, 1.318, 1.323, 1.327, 1.332, 1.337, 1.342,& 1.346, 1.351, 1.356, 1.361, 1.365, 1.370, 1.375, 1.380, 1.384,& 1.389, 1.394, 1.398, 1.403, 1.408, 1.412, 1.417, 1.421, 1.426,& 1.431, 1.435, 1.440, 1.444, 1.449, 1.454, 1.458, 1.463, 1.467,& 1.472, 1.476, 1.481, 1.485, 1.490, 1.494, 1.499, 1.503, 1.508,& 1.512, 1.517, 1.521, 1.526, 1.530, 1.535, 1.539, 1.543, 1.548,& 1.552, 1.557, 1.561, 1.565, 1.570, 1.574, 1.578, 1.583, 1.587,& 1.591, 1.596, 1.600, 1.604, 1.609, 1.613, 1.617, 1.622, 1.626,& 1.630, 1.634, 1.639, 1.643, 1.647, 1.651, 1.656, 1.660, 1.664,& 1.668, 1.672, 1.677, 1.681, 1.726, 1.766, 1.807, 1.846, 1.885,& 1.923, 1.961, 1.998, 2.034, 2.070, 2.105, 2.140, 2.175, 2.208,& 2.242, 2.275, 2.307, 2.339, 2.370, 2.401, 2.432, 2.462, 2.492,& 2.521, 2.550, 2.579, 2.607, 2.635, 2.662, 2.690, 2.716, 2.743,& 2.769, 2.795, 2.820, 2.845, 2.870, 2.895, 2.919, 2.943, 2.966,& 2.990, 3.013, 3.036, 3.058, 3.081, 3.103, 3.124, 3.146, 3.167,& 3.188, 3.209, 3.230, 3.250, 3.270, 3.290, 3.310, 3.329, 3.349,& 3.368, 3.387, 3.405, 3.424, 3.442, 3.460, 3.478, 3.496, 3.513,& 3.531, 3.548, 3.565, 3.582, 3.599, 3.615, 3.631, 3.648, 3.664,& 3.680, 3.695, 3.711, 3.726, 3.742, 3.757, 3.772, 3.787, 3.801,& 3.816, 3.830, 3.845, 3.859, 3.873, 3.887, 3.901, 3.914, 3.928,& 3.941, 3.955, 3.968, 3.981, 3.994, 4.007, 4.019, 4.032, 4.044,& 4.057, 4.069, 4.081, 4.093, 4.105, 4.117, 4.129, 4.141, 4.152,& 4.164, 4.175, 4.186, 4.197, 4.209, 4.220, 4.230, 4.241, 4.252,& 4.263, 4.273, 4.284, 4.294, 4.304, 4.314, 4.324, 4.335, 4.344,& 4.354, 4.364, 4.374, 4.383, 4.393, 4.402, 4.412, 4.421, 4.430,& 4.440, 4.449, 4.458, 4.467, 4.476, 4.484, 4.493, 4.502, 4.510,& 4.519, 4.527, 4.536, 4.544, 4.553, 4.561, 4.569, 4.577, 4.585,& 4.593, 4.601, 4.609 & / END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KM273 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IN' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C TEMPERATURE IS 273K !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KM2732p1 (IONIC, BINARR) !C !C *** Common block definition !C COMMON /KMC2732p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561), & BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561), & BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561), & BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561), & BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561), & BNC21M( 561),BNC22M( 561),BNC23M( 561) REAL Binarr (23), Ionic !C !C *** Find position in arrays for bincoef !C IF (Ionic.LE. 0.200000E+02) THEN ipos = MIN(NINT( 0.200000E+02*Ionic) + 1, 400) ELSE ipos = 400+NINT( 0.200000E+01*Ionic- 0.400000E+02) ENDIF ipos = min(ipos, 561) !C !C *** Assign values to return array !C Binarr(01) = BNC01M(ipos) Binarr(02) = BNC02M(ipos) Binarr(03) = BNC03M(ipos) Binarr(04) = BNC04M(ipos) Binarr(05) = BNC05M(ipos) Binarr(06) = BNC06M(ipos) Binarr(07) = BNC07M(ipos) Binarr(08) = BNC08M(ipos) Binarr(09) = BNC09M(ipos) Binarr(10) = BNC10M(ipos) Binarr(11) = BNC11M(ipos) Binarr(12) = BNC12M(ipos) Binarr(13) = BNC13M(ipos) Binarr(14) = BNC14M(ipos) Binarr(15) = BNC15M(ipos) Binarr(16) = BNC16M(ipos) Binarr(17) = BNC17M(ipos) Binarr(18) = BNC18M(ipos) Binarr(19) = BNC19M(ipos) Binarr(20) = BNC20M(ipos) Binarr(21) = BNC21M(ipos) Binarr(22) = BNC22M(ipos) Binarr(23) = BNC23M(ipos) !C !C *** Return point ; End of subroutine !C RETURN END BLOCK DATA KMCF2732p1 !C !C *** Common block definition !C COMMON /KMC2732p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) !C !C *** NaCl !C DATA BNC01M/ & -0.046,-0.097,-0.119,-0.134,-0.145,-0.153,-0.160,-0.165,-0.169,& -0.173,-0.176,-0.178,-0.180,-0.181,-0.182,-0.183,-0.184,-0.184,& -0.185,-0.185,-0.185,-0.185,-0.184,-0.184,-0.183,-0.183,-0.182,& -0.181,-0.181,-0.180,-0.179,-0.178,-0.177,-0.176,-0.174,-0.173,& -0.172,-0.171,-0.170,-0.168,-0.167,-0.166,-0.164,-0.163,-0.162,& -0.160,-0.159,-0.157,-0.156,-0.155,-0.153,-0.152,-0.150,-0.149,& -0.147,-0.146,-0.144,-0.143,-0.141,-0.140,-0.138,-0.137,-0.135,& -0.134,-0.132,-0.131,-0.129,-0.128,-0.126,-0.124,-0.123,-0.121,& -0.120,-0.118,-0.116,-0.115,-0.113,-0.112,-0.110,-0.108,-0.107,& -0.105,-0.103,-0.101,-0.100,-0.098,-0.096,-0.094,-0.093,-0.091,& -0.089,-0.087,-0.085,-0.083,-0.081,-0.080,-0.078,-0.076,-0.074,& -0.072,-0.070,-0.068,-0.066,-0.064,-0.062,-0.060,-0.058,-0.056,& -0.054,-0.052,-0.050,-0.048,-0.046,-0.044,-0.042,-0.039,-0.037,& -0.035,-0.033,-0.031,-0.029,-0.027,-0.025,-0.023,-0.021,-0.018,& -0.016,-0.014,-0.012,-0.010,-0.008,-0.006,-0.004,-0.002, 0.001,& 0.003, 0.005, 0.007, 0.009, 0.011, 0.013, 0.015, 0.017, 0.019,& 0.022, 0.024, 0.026, 0.028, 0.030, 0.032, 0.034, 0.036, 0.038,& 0.040, 0.042, 0.045, 0.047, 0.049, 0.051, 0.053, 0.055, 0.057,& 0.059, 0.061, 0.063, 0.065, 0.067, 0.069, 0.071, 0.073, 0.075,& 0.078, 0.080, 0.082, 0.084, 0.086, 0.088, 0.090, 0.092, 0.094,& 0.096, 0.098, 0.100, 0.102, 0.104, 0.106, 0.108, 0.110, 0.112,& 0.114, 0.116, 0.118, 0.120, 0.122, 0.124, 0.126, 0.128, 0.130,& 0.132, 0.134, 0.136, 0.138, 0.140, 0.142, 0.143, 0.145, 0.147,& 0.149, 0.151, 0.153, 0.155, 0.157, 0.159, 0.161, 0.163, 0.165,& 0.167, 0.169, 0.171, 0.172, 0.174, 0.176, 0.178, 0.180, 0.182,& 0.184, 0.186, 0.188, 0.190, 0.191, 0.193, 0.195, 0.197, 0.199,& 0.201, 0.203, 0.205, 0.206, 0.208, 0.210, 0.212, 0.214, 0.216,& 0.218, 0.219, 0.221, 0.223, 0.225, 0.227, 0.229, 0.230, 0.232,& 0.234, 0.236, 0.238, 0.239, 0.241, 0.243, 0.245, 0.247, 0.248,& 0.250, 0.252, 0.254, 0.256, 0.257, 0.259, 0.261, 0.263, 0.265,& 0.266, 0.268, 0.270, 0.272, 0.273, 0.275, 0.277, 0.279, 0.280,& 0.282, 0.284, 0.286, 0.287, 0.289, 0.291, 0.292, 0.294, 0.296,& 0.298, 0.299, 0.301, 0.303, 0.305, 0.306, 0.308, 0.310, 0.311,& 0.313, 0.315, 0.316, 0.318, 0.320, 0.321, 0.323, 0.325, 0.326,& 0.328, 0.330, 0.331, 0.333, 0.335, 0.336, 0.338, 0.340, 0.341,& 0.343, 0.345, 0.346, 0.348, 0.350, 0.351, 0.353, 0.355, 0.356,& 0.358, 0.359, 0.361, 0.363, 0.364, 0.366, 0.367, 0.369, 0.371,& 0.372, 0.374, 0.375, 0.377, 0.379, 0.380, 0.382, 0.383, 0.385,& 0.387, 0.388, 0.390, 0.391, 0.393, 0.394, 0.396, 0.398, 0.399,& 0.401, 0.402, 0.404, 0.405, 0.407, 0.408, 0.410, 0.412, 0.413,& 0.415, 0.416, 0.418, 0.419, 0.421, 0.422, 0.424, 0.425, 0.427,& 0.428, 0.430, 0.431, 0.433, 0.434, 0.436, 0.437, 0.439, 0.440,& 0.442, 0.443, 0.445, 0.446, 0.448, 0.449, 0.451, 0.452, 0.454,& 0.455, 0.457, 0.458, 0.460, 0.461, 0.463, 0.464, 0.465, 0.467,& 0.468, 0.470, 0.471, 0.473, 0.488, 0.502, 0.516, 0.530, 0.544,& 0.557, 0.570, 0.583, 0.596, 0.608, 0.621, 0.633, 0.645, 0.657,& 0.669, 0.680, 0.692, 0.703, 0.714, 0.725, 0.736, 0.747, 0.758,& 0.768, 0.778, 0.789, 0.799, 0.809, 0.819, 0.828, 0.838, 0.847,& 0.857, 0.866, 0.875, 0.884, 0.893, 0.902, 0.911, 0.920, 0.928,& 0.937, 0.945, 0.954, 0.962, 0.970, 0.978, 0.986, 0.994, 1.002,& 1.010, 1.017, 1.025, 1.032, 1.040, 1.047, 1.054, 1.062, 1.069,& 1.076, 1.083, 1.090, 1.097, 1.103, 1.110, 1.117, 1.124, 1.130,& 1.137, 1.143, 1.149, 1.156, 1.162, 1.168, 1.174, 1.181, 1.187,& 1.193, 1.199, 1.205, 1.210, 1.216, 1.222, 1.228, 1.233, 1.239,& 1.245, 1.250, 1.255, 1.261, 1.266, 1.272, 1.277, 1.282, 1.287,& 1.293, 1.298, 1.303, 1.308, 1.313, 1.318, 1.323, 1.328, 1.333,& 1.337, 1.342, 1.347, 1.352, 1.356, 1.361, 1.366, 1.370, 1.375,& 1.379, 1.384, 1.388, 1.392, 1.397, 1.401, 1.406, 1.410, 1.414,& 1.418, 1.422, 1.427, 1.431, 1.435, 1.439, 1.443, 1.447, 1.451,& 1.455, 1.459, 1.463, 1.467, 1.470, 1.474, 1.478, 1.482, 1.486,& 1.489, 1.493, 1.497, 1.500, 1.504, 1.508, 1.511, 1.515, 1.518,& 1.522, 1.525, 1.529, 1.532, 1.536, 1.539, 1.542, 1.546, 1.549,& 1.552, 1.556, 1.559 & / !C !C *** Na2SO4 !C DATA BNC02M/ & -0.096,-0.208,-0.264,-0.304,-0.335,-0.361,-0.383,-0.403,-0.420,& -0.436,-0.450,-0.464,-0.476,-0.487,-0.498,-0.508,-0.517,-0.526,& -0.535,-0.543,-0.551,-0.558,-0.566,-0.572,-0.579,-0.586,-0.592,& -0.598,-0.603,-0.609,-0.614,-0.620,-0.625,-0.630,-0.635,-0.639,& -0.644,-0.649,-0.653,-0.657,-0.661,-0.666,-0.670,-0.674,-0.677,& -0.681,-0.685,-0.689,-0.692,-0.696,-0.699,-0.702,-0.706,-0.709,& -0.712,-0.715,-0.718,-0.721,-0.725,-0.727,-0.730,-0.733,-0.736,& -0.739,-0.742,-0.744,-0.747,-0.750,-0.752,-0.755,-0.757,-0.760,& -0.763,-0.765,-0.767,-0.770,-0.772,-0.775,-0.777,-0.779,-0.782,& -0.784,-0.786,-0.788,-0.791,-0.793,-0.795,-0.797,-0.799,-0.801,& -0.803,-0.806,-0.808,-0.810,-0.812,-0.814,-0.816,-0.818,-0.820,& 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2.788, 2.795, 2.802, 2.808,& 2.815, 2.822, 2.828, 2.835, 2.842, 2.848, 2.855, 2.862, 2.868,& 2.875, 2.881, 2.888, 2.894, 2.901, 2.907, 2.914, 2.920, 2.927,& 2.933, 2.940, 2.946, 2.953, 2.959, 2.966, 2.972, 2.978, 2.985,& 2.991, 2.998, 3.004, 3.010, 3.017, 3.023, 3.029, 3.036, 3.042,& 3.048, 3.054, 3.061, 3.067, 3.134, 3.195, 3.254, 3.313, 3.371,& 3.428, 3.485, 3.540, 3.595, 3.648, 3.701, 3.754, 3.805, 3.856,& 3.906, 3.955, 4.004, 4.052, 4.100, 4.147, 4.193, 4.239, 4.284,& 4.328, 4.372, 4.416, 4.459, 4.501, 4.543, 4.585, 4.626, 4.666,& 4.707, 4.746, 4.786, 4.824, 4.863, 4.901, 4.938, 4.976, 5.013,& 5.049, 5.085, 5.121, 5.156, 5.191, 5.226, 5.260, 5.294, 5.328,& 5.361, 5.395, 5.427, 5.460, 5.492, 5.524, 5.555, 5.587, 5.618,& 5.649, 5.679, 5.709, 5.739, 5.769, 5.799, 5.828, 5.857, 5.886,& 5.914, 5.942, 5.971, 5.998, 6.026, 6.053, 6.081, 6.108, 6.134,& 6.161, 6.187, 6.214, 6.240, 6.265, 6.291, 6.316, 6.342, 6.367,& 6.392, 6.416, 6.441, 6.465, 6.489, 6.513, 6.537, 6.561, 6.584,& 6.608, 6.631, 6.654, 6.677, 6.699, 6.722, 6.744, 6.767, 6.789,& 6.811, 6.833, 6.854, 6.876, 6.897, 6.919, 6.940, 6.961, 6.982,& 7.003, 7.023, 7.044, 7.064, 7.085, 7.105, 7.125, 7.145, 7.165,& 7.184, 7.204, 7.223, 7.243, 7.262, 7.281, 7.300, 7.319, 7.338,& 7.356, 7.375, 7.394, 7.412, 7.430, 7.448, 7.467, 7.485, 7.502,& 7.520, 7.538, 7.556, 7.573, 7.591, 7.608, 7.625, 7.642, 7.659,& 7.676, 7.693, 7.710, 7.727, 7.743, 7.760, 7.776, 7.793, 7.809,& 7.825, 7.841, 7.858 & / !C !C *** NH4HSO4 !C DATA BNC09M/ & -0.047,-0.099,-0.125,-0.142,-0.155,-0.166,-0.175,-0.182,-0.189,& -0.195,-0.200,-0.204,-0.208,-0.212,-0.215,-0.218,-0.221,-0.223,& -0.225,-0.227,-0.228,-0.230,-0.231,-0.232,-0.233,-0.234,-0.235,& -0.235,-0.235,-0.236,-0.236,-0.236,-0.236,-0.235,-0.235,-0.235,& -0.234,-0.233,-0.233,-0.232,-0.231,-0.230,-0.229,-0.228,-0.227,& -0.226,-0.224,-0.223,-0.222,-0.220,-0.219,-0.217,-0.215,-0.214,& -0.212,-0.210,-0.208,-0.207,-0.205,-0.203,-0.201,-0.199,-0.197,& 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0.228, 0.231, 0.234, 0.237, 0.240,& 0.243, 0.246, 0.248, 0.251, 0.254, 0.257, 0.260, 0.262, 0.265,& 0.268, 0.271, 0.274, 0.276, 0.279, 0.282, 0.285, 0.287, 0.290,& 0.293, 0.296, 0.298, 0.301, 0.304, 0.306, 0.309, 0.312, 0.315,& 0.317, 0.320, 0.323, 0.325, 0.328, 0.330, 0.333, 0.336, 0.338,& 0.341, 0.344, 0.346, 0.349, 0.351, 0.354, 0.357, 0.359, 0.362,& 0.364, 0.367, 0.369, 0.372, 0.375, 0.377, 0.380, 0.382, 0.385,& 0.387, 0.390, 0.392, 0.395, 0.397, 0.400, 0.402, 0.405, 0.407,& 0.410, 0.412, 0.415, 0.417, 0.419, 0.422, 0.424, 0.427, 0.429,& 0.432, 0.434, 0.437, 0.439, 0.441, 0.444, 0.446, 0.449, 0.451,& 0.453, 0.456, 0.458, 0.460, 0.463, 0.465, 0.467, 0.470, 0.472,& 0.474, 0.477, 0.479, 0.481, 0.484, 0.486, 0.488, 0.491, 0.493,& 0.495, 0.498, 0.500, 0.502, 0.504, 0.507, 0.509, 0.511, 0.513,& 0.516, 0.518, 0.520, 0.522, 0.525, 0.527, 0.529, 0.531, 0.534,& 0.536, 0.538, 0.540, 0.542, 0.545, 0.547, 0.549, 0.551, 0.553,& 0.556, 0.558, 0.560, 0.562, 0.564, 0.566, 0.569, 0.571, 0.573,& 0.575, 0.577, 0.579, 0.581, 0.584, 0.586, 0.588, 0.590, 0.592,& 0.594, 0.596, 0.598, 0.600, 0.602, 0.605, 0.607, 0.609, 0.611,& 0.613, 0.615, 0.617, 0.619, 0.621, 0.623, 0.625, 0.627, 0.629,& 0.631, 0.633, 0.635, 0.637, 0.639, 0.642, 0.644, 0.646, 0.648,& 0.650, 0.652, 0.654, 0.656, 0.658, 0.660, 0.662, 0.663, 0.665,& 0.667, 0.669, 0.671, 0.673, 0.675, 0.677, 0.679, 0.681, 0.683,& 0.685, 0.687, 0.689, 0.691, 0.712, 0.730, 0.749, 0.767, 0.785,& 0.803, 0.820, 0.837, 0.854, 0.871, 0.887, 0.903, 0.919, 0.935,& 0.950, 0.965, 0.980, 0.995, 1.010, 1.024, 1.039, 1.053, 1.067,& 1.080, 1.094, 1.107, 1.120, 1.133, 1.146, 1.159, 1.172, 1.184,& 1.196, 1.209, 1.221, 1.232, 1.244, 1.256, 1.267, 1.279, 1.290,& 1.301, 1.312, 1.323, 1.334, 1.344, 1.355, 1.365, 1.376, 1.386,& 1.396, 1.406, 1.416, 1.426, 1.436, 1.445, 1.455, 1.464, 1.474,& 1.483, 1.492, 1.501, 1.511, 1.519, 1.528, 1.537, 1.546, 1.555,& 1.563, 1.572, 1.580, 1.588, 1.597, 1.605, 1.613, 1.621, 1.629,& 1.637, 1.645, 1.653, 1.660, 1.668, 1.676, 1.683, 1.691, 1.698,& 1.706, 1.713, 1.720, 1.727, 1.734, 1.742, 1.749, 1.756, 1.763,& 1.769, 1.776, 1.783, 1.790, 1.796, 1.803, 1.810, 1.816, 1.823,& 1.829, 1.835, 1.842, 1.848, 1.854, 1.861, 1.867, 1.873, 1.879,& 1.885, 1.891, 1.897, 1.903, 1.909, 1.915, 1.920, 1.926, 1.932,& 1.938, 1.943, 1.949, 1.954, 1.960, 1.965, 1.971, 1.976, 1.982,& 1.987, 1.992, 1.998, 2.003, 2.008, 2.013, 2.018, 2.024, 2.029,& 2.034, 2.039, 2.044, 2.049, 2.054, 2.059, 2.063, 2.068, 2.073,& 2.078, 2.083, 2.087, 2.092, 2.097, 2.101, 2.106, 2.111, 2.115,& 2.120, 2.124, 2.129 & / !C !C *** (H,NO3) !C DATA BNC10M/ & -0.046,-0.096,-0.118,-0.132,-0.142,-0.150,-0.156,-0.161,-0.164,& -0.167,-0.170,-0.171,-0.173,-0.174,-0.174,-0.175,-0.175,-0.175,& -0.175,-0.174,-0.174,-0.173,-0.172,-0.171,-0.170,-0.169,-0.168,& -0.167,-0.165,-0.164,-0.163,-0.161,-0.160,-0.158,-0.156,-0.155,& -0.153,-0.151,-0.150,-0.148,-0.146,-0.144,-0.142,-0.141,-0.139,& -0.137,-0.135,-0.133,-0.131,-0.129,-0.127,-0.125,-0.124,-0.122,& -0.120,-0.118,-0.116,-0.114,-0.112,-0.110,-0.108,-0.106,-0.104,& -0.102,-0.100,-0.098,-0.096,-0.094,-0.092,-0.090,-0.088,-0.086,& -0.084,-0.082,-0.080,-0.078,-0.076,-0.074,-0.071,-0.069,-0.067,& -0.065,-0.063,-0.061,-0.058,-0.056,-0.054,-0.052,-0.049,-0.047,& -0.045,-0.043,-0.040,-0.038,-0.035,-0.033,-0.031,-0.028,-0.026,& -0.023,-0.021,-0.019,-0.016,-0.014,-0.011,-0.009,-0.006,-0.004,& -0.001, 0.001, 0.004, 0.007, 0.009, 0.012, 0.014, 0.017, 0.019,& 0.022, 0.025, 0.027, 0.030, 0.032, 0.035, 0.038, 0.040, 0.043,& 0.045, 0.048, 0.051, 0.053, 0.056, 0.058, 0.061, 0.064, 0.066,& 0.069, 0.071, 0.074, 0.077, 0.079, 0.082, 0.084, 0.087, 0.090,& 0.092, 0.095, 0.097, 0.100, 0.103, 0.105, 0.108, 0.110, 0.113,& 0.115, 0.118, 0.121, 0.123, 0.126, 0.128, 0.131, 0.133, 0.136,& 0.138, 0.141, 0.143, 0.146, 0.148, 0.151, 0.154, 0.156, 0.159,& 0.161, 0.164, 0.166, 0.169, 0.171, 0.174, 0.176, 0.179, 0.181,& 0.184, 0.186, 0.189, 0.191, 0.193, 0.196, 0.198, 0.201, 0.203,& 0.206, 0.208, 0.211, 0.213, 0.216, 0.218, 0.220, 0.223, 0.225,& 0.228, 0.230, 0.232, 0.235, 0.237, 0.240, 0.242, 0.245, 0.247,& 0.249, 0.252, 0.254, 0.256, 0.259, 0.261, 0.264, 0.266, 0.268,& 0.271, 0.273, 0.275, 0.278, 0.280, 0.282, 0.285, 0.287, 0.289,& 0.292, 0.294, 0.296, 0.299, 0.301, 0.303, 0.306, 0.308, 0.310,& 0.312, 0.315, 0.317, 0.319, 0.322, 0.324, 0.326, 0.328, 0.331,& 0.333, 0.335, 0.337, 0.340, 0.342, 0.344, 0.346, 0.349, 0.351,& 0.353, 0.355, 0.357, 0.360, 0.362, 0.364, 0.366, 0.369, 0.371,& 0.373, 0.375, 0.377, 0.379, 0.382, 0.384, 0.386, 0.388, 0.390,& 0.393, 0.395, 0.397, 0.399, 0.401, 0.403, 0.405, 0.408, 0.410,& 0.412, 0.414, 0.416, 0.418, 0.420, 0.422, 0.425, 0.427, 0.429,& 0.431, 0.433, 0.435, 0.437, 0.439, 0.441, 0.443, 0.445, 0.448,& 0.450, 0.452, 0.454, 0.456, 0.458, 0.460, 0.462, 0.464, 0.466,& 0.468, 0.470, 0.472, 0.474, 0.476, 0.478, 0.480, 0.482, 0.484,& 0.486, 0.488, 0.490, 0.492, 0.494, 0.496, 0.498, 0.500, 0.502,& 0.504, 0.506, 0.508, 0.510, 0.512, 0.514, 0.516, 0.518, 0.520,& 0.522, 0.524, 0.526, 0.528, 0.530, 0.532, 0.534, 0.536, 0.537,& 0.539, 0.541, 0.543, 0.545, 0.547, 0.549, 0.551, 0.553, 0.555,& 0.557, 0.558, 0.560, 0.562, 0.564, 0.566, 0.568, 0.570, 0.572,& 0.574, 0.575, 0.577, 0.579, 0.581, 0.583, 0.585, 0.587, 0.588,& 0.590, 0.592, 0.594, 0.596, 0.598, 0.599, 0.601, 0.603, 0.605,& 0.607, 0.609, 0.610, 0.612, 0.614, 0.616, 0.618, 0.619, 0.621,& 0.623, 0.625, 0.627, 0.628, 0.630, 0.632, 0.634, 0.635, 0.637,& 0.639, 0.641, 0.643, 0.644, 0.663, 0.680, 0.697, 0.714, 0.730,& 0.747, 0.763, 0.778, 0.794, 0.809, 0.824, 0.839, 0.854, 0.868,& 0.883, 0.897, 0.911, 0.924, 0.938, 0.951, 0.965, 0.978, 0.990,& 1.003, 1.016, 1.028, 1.040, 1.053, 1.065, 1.076, 1.088, 1.100,& 1.111, 1.122, 1.133, 1.145, 1.155, 1.166, 1.177, 1.188, 1.198,& 1.208, 1.219, 1.229, 1.239, 1.249, 1.258, 1.268, 1.278, 1.287,& 1.297, 1.306, 1.315, 1.324, 1.333, 1.342, 1.351, 1.360, 1.369,& 1.377, 1.386, 1.394, 1.403, 1.411, 1.419, 1.428, 1.436, 1.444,& 1.452, 1.459, 1.467, 1.475, 1.483, 1.490, 1.498, 1.505, 1.513,& 1.520, 1.527, 1.535, 1.542, 1.549, 1.556, 1.563, 1.570, 1.577,& 1.584, 1.590, 1.597, 1.604, 1.610, 1.617, 1.623, 1.630, 1.636,& 1.643, 1.649, 1.655, 1.661, 1.667, 1.674, 1.680, 1.686, 1.692,& 1.698, 1.703, 1.709, 1.715, 1.721, 1.727, 1.732, 1.738, 1.744,& 1.749, 1.755, 1.760, 1.766, 1.771, 1.776, 1.782, 1.787, 1.792,& 1.797, 1.803, 1.808, 1.813, 1.818, 1.823, 1.828, 1.833, 1.838,& 1.843, 1.848, 1.853, 1.857, 1.862, 1.867, 1.872, 1.876, 1.881,& 1.886, 1.890, 1.895, 1.899, 1.904, 1.908, 1.913, 1.917, 1.922,& 1.926, 1.930, 1.935, 1.939, 1.943, 1.948, 1.952, 1.956, 1.960,& 1.964, 1.968, 1.973 & / !C !C *** (H,Cl) !C DATA BNC11M/ & -0.045,-0.090,-0.108,-0.119,-0.126,-0.130,-0.133,-0.135,-0.135,& -0.135,-0.134,-0.133,-0.131,-0.129,-0.126,-0.124,-0.121,-0.117,& -0.114,-0.110,-0.106,-0.102,-0.098,-0.093,-0.089,-0.084,-0.079,& -0.075,-0.070,-0.065,-0.059,-0.054,-0.049,-0.044,-0.038,-0.033,& -0.027,-0.022,-0.016,-0.010,-0.004, 0.001, 0.007, 0.013, 0.019,& 0.025, 0.031, 0.037, 0.043, 0.049, 0.055, 0.061, 0.067, 0.073,& 0.079, 0.085, 0.091, 0.098, 0.104, 0.110, 0.116, 0.122, 0.129,& 0.135, 0.141, 0.147, 0.154, 0.160, 0.166, 0.173, 0.179, 0.185,& 0.192, 0.198, 0.205, 0.211, 0.218, 0.224, 0.231, 0.238, 0.244,& 0.251, 0.258, 0.264, 0.271, 0.278, 0.285, 0.292, 0.298, 0.305,& 0.312, 0.319, 0.326, 0.333, 0.341, 0.348, 0.355, 0.362, 0.369,& 0.377, 0.384, 0.391, 0.398, 0.406, 0.413, 0.421, 0.428, 0.435,& 0.443, 0.450, 0.458, 0.465, 0.473, 0.480, 0.488, 0.495, 0.503,& 0.510, 0.518, 0.526, 0.533, 0.541, 0.548, 0.556, 0.563, 0.571,& 0.578, 0.586, 0.594, 0.601, 0.609, 0.616, 0.624, 0.631, 0.639,& 0.646, 0.654, 0.661, 0.669, 0.676, 0.684, 0.691, 0.699, 0.706,& 0.713, 0.721, 0.728, 0.736, 0.743, 0.750, 0.758, 0.765, 0.772,& 0.780, 0.787, 0.794, 0.802, 0.809, 0.816, 0.823, 0.831, 0.838,& 0.845, 0.852, 0.859, 0.867, 0.874, 0.881, 0.888, 0.895, 0.902,& 0.909, 0.916, 0.924, 0.931, 0.938, 0.945, 0.952, 0.959, 0.966,& 0.973, 0.980, 0.987, 0.994, 1.000, 1.007, 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4.270, 4.291,& 4.312, 4.332, 4.353, 4.373, 4.394, 4.414, 4.434, 4.453, 4.473,& 4.493, 4.512, 4.531, 4.550, 4.569, 4.588, 4.606, 4.625, 4.643,& 4.661, 4.679, 4.697, 4.715, 4.733, 4.750, 4.768, 4.785, 4.802,& 4.819, 4.836, 4.853, 4.870, 4.886, 4.903, 4.919, 4.936, 4.952,& 4.968, 4.984, 5.000, 5.015, 5.031, 5.046, 5.062, 5.077, 5.093,& 5.108, 5.123, 5.138, 5.153, 5.167, 5.182, 5.197, 5.211, 5.226,& 5.240, 5.254, 5.268, 5.282, 5.296, 5.310, 5.324, 5.338, 5.352,& 5.365, 5.379, 5.392, 5.406, 5.419, 5.432, 5.445, 5.458, 5.471,& 5.484, 5.497, 5.510, 5.523, 5.535, 5.548, 5.560, 5.573, 5.585,& 5.598, 5.610, 5.622, 5.634, 5.646, 5.658, 5.670, 5.682, 5.694,& 5.706, 5.717, 5.729 & / !C !C ** NaHSO4 !C DATA BNC12M/ & -0.046,-0.096,-0.118,-0.132,-0.143,-0.151,-0.158,-0.163,-0.167,& -0.170,-0.173,-0.175,-0.177,-0.178,-0.179,-0.180,-0.180,-0.180,& -0.180,-0.180,-0.179,-0.179,-0.178,-0.177,-0.176,-0.174,-0.173,& -0.171,-0.170,-0.168,-0.166,-0.164,-0.162,-0.159,-0.157,-0.155,& 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2.562, 2.577, 2.592,& 2.608, 2.623, 2.638, 2.653, 2.667, 2.682, 2.697, 2.711, 2.725,& 2.739, 2.753, 2.767, 2.781, 2.795, 2.808, 2.822, 2.835, 2.848,& 2.861, 2.874, 2.887, 2.900, 2.913, 2.925, 2.938, 2.950, 2.963,& 2.975, 2.987, 2.999, 3.011, 3.023, 3.035, 3.046, 3.058, 3.069,& 3.081, 3.092, 3.104, 3.115, 3.126, 3.137, 3.148, 3.159, 3.170,& 3.180, 3.191, 3.202, 3.212, 3.223, 3.233, 3.244, 3.254, 3.264,& 3.274, 3.284, 3.294, 3.304, 3.314, 3.324, 3.334, 3.343, 3.353,& 3.363, 3.372, 3.382, 3.391, 3.400, 3.410, 3.419, 3.428, 3.437,& 3.446, 3.455, 3.464, 3.473, 3.482, 3.491, 3.499, 3.508, 3.517,& 3.525, 3.534, 3.542, 3.551, 3.559, 3.568, 3.576, 3.584, 3.592,& 3.601, 3.609, 3.617, 3.625, 3.633, 3.641, 3.649, 3.657, 3.664,& 3.672, 3.680, 3.688 & / !C !C ** (NH4)3H(SO4)2 !C DATA BNC13M/ & -0.076,-0.165,-0.209,-0.240,-0.264,-0.284,-0.301,-0.316,-0.329,& -0.341,-0.352,-0.362,-0.371,-0.379,-0.387,-0.394,-0.401,-0.408,& -0.414,-0.420,-0.425,-0.430,-0.435,-0.440,-0.444,-0.449,-0.453,& 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3.305, 3.312, 3.319 & / !C !C ** MGCL2 !C DATA BNC23M/ & -0.092,-0.190,-0.233,-0.261,-0.280,-0.295,-0.306,-0.314,-0.321,& -0.326,-0.330,-0.333,-0.335,-0.336,-0.336,-0.336,-0.336,-0.335,& -0.334,-0.332,-0.330,-0.328,-0.326,-0.323,-0.320,-0.317,-0.314,& -0.311,-0.308,-0.304,-0.300,-0.297,-0.293,-0.289,-0.285,-0.281,& -0.277,-0.272,-0.268,-0.264,-0.259,-0.255,-0.251,-0.246,-0.242,& -0.237,-0.233,-0.228,-0.224,-0.219,-0.215,-0.210,-0.205,-0.201,& -0.196,-0.192,-0.187,-0.182,-0.178,-0.173,-0.168,-0.164,-0.159,& -0.154,-0.150,-0.145,-0.140,-0.135,-0.131,-0.126,-0.121,-0.116,& -0.111,-0.106,-0.102,-0.097,-0.092,-0.087,-0.082,-0.077,-0.072,& -0.067,-0.062,-0.056,-0.051,-0.046,-0.041,-0.036,-0.030,-0.025,& -0.019,-0.014,-0.009,-0.003, 0.002, 0.008, 0.013, 0.019, 0.025,& 0.030, 0.036, 0.042, 0.047, 0.053, 0.059, 0.065, 0.071, 0.077,& 0.082, 0.088, 0.094, 0.100, 0.106, 0.112, 0.118, 0.124, 0.130,& 0.136, 0.142, 0.148, 0.154, 0.160, 0.166, 0.172, 0.178, 0.184,& 0.190, 0.196, 0.202, 0.208, 0.214, 0.220, 0.226, 0.232, 0.238,& 0.244, 0.250, 0.256, 0.262, 0.268, 0.274, 0.280, 0.286, 0.292,& 0.298, 0.304, 0.310, 0.316, 0.322, 0.328, 0.334, 0.340, 0.346,& 0.352, 0.358, 0.364, 0.370, 0.376, 0.382, 0.387, 0.393, 0.399,& 0.405, 0.411, 0.417, 0.423, 0.429, 0.434, 0.440, 0.446, 0.452,& 0.458, 0.463, 0.469, 0.475, 0.481, 0.487, 0.492, 0.498, 0.504,& 0.509, 0.515, 0.521, 0.527, 0.532, 0.538, 0.544, 0.549, 0.555,& 0.561, 0.566, 0.572, 0.578, 0.583, 0.589, 0.594, 0.600, 0.606,& 0.611, 0.617, 0.622, 0.628, 0.633, 0.639, 0.645, 0.650, 0.656,& 0.661, 0.667, 0.672, 0.678, 0.683, 0.688, 0.694, 0.699, 0.705,& 0.710, 0.716, 0.721, 0.726, 0.732, 0.737, 0.743, 0.748, 0.753,& 0.759, 0.764, 0.769, 0.775, 0.780, 0.785, 0.791, 0.796, 0.801,& 0.807, 0.812, 0.817, 0.822, 0.828, 0.833, 0.838, 0.843, 0.848,& 0.854, 0.859, 0.864, 0.869, 0.874, 0.879, 0.885, 0.890, 0.895,& 0.900, 0.905, 0.910, 0.915, 0.920, 0.925, 0.931, 0.936, 0.941,& 0.946, 0.951, 0.956, 0.961, 0.966, 0.971, 0.976, 0.981, 0.986,& 0.991, 0.996, 1.001, 1.006, 1.011, 1.015, 1.020, 1.025, 1.030,& 1.035, 1.040, 1.045, 1.050, 1.055, 1.059, 1.064, 1.069, 1.074,& 1.079, 1.084, 1.088, 1.093, 1.098, 1.103, 1.108, 1.112, 1.117,& 1.122, 1.127, 1.131, 1.136, 1.141, 1.146, 1.150, 1.155, 1.160,& 1.164, 1.169, 1.174, 1.178, 1.183, 1.188, 1.192, 1.197, 1.201,& 1.206, 1.211, 1.215, 1.220, 1.224, 1.229, 1.234, 1.238, 1.243,& 1.247, 1.252, 1.256, 1.261, 1.265, 1.270, 1.274, 1.279, 1.283,& 1.288, 1.292, 1.297, 1.301, 1.306, 1.310, 1.315, 1.319, 1.323,& 1.328, 1.332, 1.337, 1.341, 1.345, 1.350, 1.354, 1.359, 1.363,& 1.367, 1.372, 1.376, 1.380, 1.385, 1.389, 1.393, 1.398, 1.402,& 1.406, 1.410, 1.415, 1.419, 1.423, 1.428, 1.432, 1.436, 1.440,& 1.444, 1.449, 1.453, 1.457, 1.461, 1.466, 1.470, 1.474, 1.478,& 1.482, 1.486, 1.491, 1.495, 1.499, 1.503, 1.507, 1.511, 1.515,& 1.519, 1.524, 1.528, 1.532, 1.536, 1.540, 1.544, 1.548, 1.552,& 1.556, 1.560, 1.564, 1.568, 1.611, 1.651, 1.690, 1.728, 1.765,& 1.802, 1.839, 1.875, 1.911, 1.945, 1.980, 2.014, 2.048, 2.081,& 2.113, 2.146, 2.177, 2.209, 2.240, 2.270, 2.300, 2.330, 2.360,& 2.389, 2.417, 2.446, 2.474, 2.502, 2.529, 2.556, 2.583, 2.609,& 2.635, 2.661, 2.686, 2.712, 2.737, 2.761, 2.786, 2.810, 2.834,& 2.857, 2.881, 2.904, 2.927, 2.950, 2.972, 2.994, 3.016, 3.038,& 3.060, 3.081, 3.102, 3.123, 3.144, 3.164, 3.184, 3.205, 3.225,& 3.244, 3.264, 3.283, 3.302, 3.322, 3.340, 3.359, 3.378, 3.396,& 3.414, 3.432, 3.450, 3.468, 3.485, 3.503, 3.520, 3.537, 3.554,& 3.571, 3.588, 3.604, 3.621, 3.637, 3.653, 3.669, 3.685, 3.701,& 3.717, 3.732, 3.748, 3.763, 3.778, 3.793, 3.808, 3.823, 3.838,& 3.852, 3.867, 3.881, 3.896, 3.910, 3.924, 3.938, 3.952, 3.966,& 3.979, 3.993, 4.006, 4.020, 4.033, 4.046, 4.059, 4.072, 4.085,& 4.098, 4.111, 4.123, 4.136, 4.148, 4.161, 4.173, 4.185, 4.197,& 4.210, 4.222, 4.233, 4.245, 4.257, 4.269, 4.280, 4.292, 4.303,& 4.315, 4.326, 4.337, 4.348, 4.359, 4.370, 4.381, 4.392, 4.403,& 4.414, 4.424, 4.435, 4.446, 4.456, 4.466, 4.477, 4.487, 4.497,& 4.507, 4.518, 4.528, 4.538, 4.548, 4.557, 4.567, 4.577, 4.587,& 4.596, 4.606, 4.615 & / END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KM298 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IN' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C TEMPERATURE IS 298K !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KM2982p1 (IONIC, BINARR) !C !C *** Common block definition !C COMMON /KMC2982p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) REAL Binarr (23), Ionic !C !C *** Find position in arrays for bincoef !C IF (Ionic.LE. 0.200000E+02) THEN ipos = MIN(NINT( 0.200000E+02*Ionic) + 1, 400) ELSE ipos = 400+NINT( 0.200000E+01*Ionic- 0.400000E+02) ENDIF ipos = min(ipos, 561) !C !C *** Assign values to return array !C Binarr(01) = BNC01M(ipos) Binarr(02) = BNC02M(ipos) Binarr(03) = BNC03M(ipos) Binarr(04) = BNC04M(ipos) Binarr(05) = BNC05M(ipos) Binarr(06) = BNC06M(ipos) Binarr(07) = BNC07M(ipos) Binarr(08) = BNC08M(ipos) Binarr(09) = BNC09M(ipos) Binarr(10) = BNC10M(ipos) Binarr(11) = BNC11M(ipos) Binarr(12) = BNC12M(ipos) Binarr(13) = BNC13M(ipos) Binarr(14) = BNC14M(ipos) Binarr(15) = BNC15M(ipos) Binarr(16) = BNC16M(ipos) Binarr(17) = BNC17M(ipos) Binarr(18) = BNC18M(ipos) Binarr(19) = BNC19M(ipos) Binarr(20) = BNC20M(ipos) Binarr(21) = BNC21M(ipos) Binarr(22) = BNC22M(ipos) Binarr(23) = BNC23M(ipos) !C !C *** Return point ; End of subroutine !C RETURN END BLOCK DATA KMCF2982p1 !C !C *** Common block definition !C COMMON /KMC2982p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) !C !C *** NaCl !C DATA BNC01M/ & -0.045,-0.095,-0.117,-0.132,-0.142,-0.150,-0.157,-0.162,-0.166,& -0.170,-0.173,-0.175,-0.177,-0.179,-0.180,-0.181,-0.182,-0.182,& -0.183,-0.183,-0.183,-0.183,-0.182,-0.182,-0.182,-0.181,-0.181,& -0.180,-0.179,-0.178,-0.178,-0.177,-0.176,-0.175,-0.174,-0.173,& -0.172,-0.170,-0.169,-0.168,-0.167,-0.166,-0.164,-0.163,-0.162,& -0.161,-0.159,-0.158,-0.157,-0.155,-0.154,-0.153,-0.151,-0.150,& -0.148,-0.147,-0.146,-0.144,-0.143,-0.141,-0.140,-0.138,-0.137,& -0.136,-0.134,-0.133,-0.131,-0.130,-0.128,-0.127,-0.125,-0.124,& -0.122,-0.121,-0.119,-0.117,-0.116,-0.114,-0.113,-0.111,-0.110,& -0.108,-0.106,-0.105,-0.103,-0.101,-0.100,-0.098,-0.096,-0.094,& -0.093,-0.091,-0.089,-0.087,-0.086,-0.084,-0.082,-0.080,-0.078,& -0.076,-0.075,-0.073,-0.071,-0.069,-0.067,-0.065,-0.063,-0.061,& -0.059,-0.057,-0.055,-0.053,-0.051,-0.049,-0.047,-0.046,-0.044,& -0.042,-0.040,-0.038,-0.036,-0.034,-0.032,-0.030,-0.028,-0.026,& -0.024,-0.022,-0.019,-0.017,-0.015,-0.013,-0.011,-0.009,-0.007,& -0.005,-0.003,-0.001, 0.001, 0.003, 0.005, 0.007, 0.009, 0.011,& 0.013, 0.015, 0.017, 0.019, 0.021, 0.023, 0.025, 0.027, 0.029,& 0.031, 0.033, 0.035, 0.037, 0.039, 0.041, 0.043, 0.045, 0.047,& 0.049, 0.050, 0.052, 0.054, 0.056, 0.058, 0.060, 0.062, 0.064,& 0.066, 0.068, 0.070, 0.072, 0.074, 0.076, 0.078, 0.080, 0.082,& 0.084, 0.086, 0.088, 0.090, 0.091, 0.093, 0.095, 0.097, 0.099,& 0.101, 0.103, 0.105, 0.107, 0.109, 0.111, 0.113, 0.114, 0.116,& 0.118, 0.120, 0.122, 0.124, 0.126, 0.128, 0.130, 0.131, 0.133,& 0.135, 0.137, 0.139, 0.141, 0.143, 0.145, 0.146, 0.148, 0.150,& 0.152, 0.154, 0.156, 0.158, 0.159, 0.161, 0.163, 0.165, 0.167,& 0.169, 0.170, 0.172, 0.174, 0.176, 0.178, 0.180, 0.181, 0.183,& 0.185, 0.187, 0.189, 0.190, 0.192, 0.194, 0.196, 0.198, 0.199,& 0.201, 0.203, 0.205, 0.206, 0.208, 0.210, 0.212, 0.214, 0.215,& 0.217, 0.219, 0.221, 0.222, 0.224, 0.226, 0.228, 0.229, 0.231,& 0.233, 0.235, 0.236, 0.238, 0.240, 0.242, 0.243, 0.245, 0.247,& 0.248, 0.250, 0.252, 0.254, 0.255, 0.257, 0.259, 0.260, 0.262,& 0.264, 0.265, 0.267, 0.269, 0.271, 0.272, 0.274, 0.276, 0.277,& 0.279, 0.281, 0.282, 0.284, 0.286, 0.287, 0.289, 0.291, 0.292,& 0.294, 0.296, 0.297, 0.299, 0.301, 0.302, 0.304, 0.305, 0.307,& 0.309, 0.310, 0.312, 0.314, 0.315, 0.317, 0.318, 0.320, 0.322,& 0.323, 0.325, 0.327, 0.328, 0.330, 0.331, 0.333, 0.335, 0.336,& 0.338, 0.339, 0.341, 0.343, 0.344, 0.346, 0.347, 0.349, 0.350,& 0.352, 0.354, 0.355, 0.357, 0.358, 0.360, 0.361, 0.363, 0.364,& 0.366, 0.368, 0.369, 0.371, 0.372, 0.374, 0.375, 0.377, 0.378,& 0.380, 0.381, 0.383, 0.384, 0.386, 0.388, 0.389, 0.391, 0.392,& 0.394, 0.395, 0.397, 0.398, 0.400, 0.401, 0.403, 0.404, 0.406,& 0.407, 0.409, 0.410, 0.412, 0.413, 0.415, 0.416, 0.418, 0.419,& 0.421, 0.422, 0.423, 0.425, 0.426, 0.428, 0.429, 0.431, 0.432,& 0.434, 0.435, 0.437, 0.438, 0.440, 0.441, 0.442, 0.444, 0.445,& 0.447, 0.448, 0.450, 0.451, 0.466, 0.480, 0.494, 0.508, 0.522,& 0.535, 0.548, 0.561, 0.574, 0.586, 0.599, 0.611, 0.624, 0.636,& 0.648, 0.659, 0.671, 0.683, 0.694, 0.705, 0.716, 0.727, 0.738,& 0.749, 0.760, 0.770, 0.781, 0.791, 0.801, 0.811, 0.821, 0.831,& 0.841, 0.851, 0.861, 0.870, 0.879, 0.889, 0.898, 0.907, 0.916,& 0.925, 0.934, 0.943, 0.952, 0.961, 0.969, 0.978, 0.986, 0.995,& 1.003, 1.011, 1.019, 1.028, 1.036, 1.044, 1.051, 1.059, 1.067,& 1.075, 1.082, 1.090, 1.098, 1.105, 1.113, 1.120, 1.127, 1.135,& 1.142, 1.149, 1.156, 1.163, 1.170, 1.177, 1.184, 1.191, 1.198,& 1.204, 1.211, 1.218, 1.224, 1.231, 1.237, 1.244, 1.250, 1.257,& 1.263, 1.269, 1.276, 1.282, 1.288, 1.294, 1.300, 1.307, 1.313,& 1.319, 1.325, 1.330, 1.336, 1.342, 1.348, 1.354, 1.360, 1.365,& 1.371, 1.377, 1.382, 1.388, 1.393, 1.399, 1.404, 1.410, 1.415,& 1.421, 1.426, 1.431, 1.437, 1.442, 1.447, 1.453, 1.458, 1.463,& 1.468, 1.473, 1.478, 1.483, 1.488, 1.493, 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6.257, 6.278, 6.298, 6.319, 6.339, 6.359, 6.380, 6.400,& 6.419, 6.439, 6.459, 6.478, 6.498, 6.517, 6.536, 6.555, 6.574,& 6.593, 6.612, 6.631, 6.649, 6.668, 6.686, 6.705, 6.723, 6.741,& 6.759, 6.777, 6.795, 6.812, 6.830, 6.848, 6.865, 6.882, 6.900,& 6.917, 6.934, 6.951, 6.968, 6.985, 7.002, 7.018, 7.035, 7.052,& 7.068, 7.084, 7.101, 7.117, 7.133, 7.149, 7.165, 7.181, 7.197,& 7.213, 7.229, 7.244 & / !C !C ** NH4HSO4 !C DATA BNC09M/ & -0.046,-0.097,-0.122,-0.138,-0.151,-0.162,-0.170,-0.177,-0.184,& -0.189,-0.194,-0.198,-0.202,-0.206,-0.209,-0.212,-0.214,-0.216,& -0.218,-0.220,-0.222,-0.223,-0.224,-0.225,-0.226,-0.227,-0.227,& -0.228,-0.228,-0.228,-0.228,-0.228,-0.228,-0.228,-0.228,-0.227,& -0.227,-0.226,-0.225,-0.225,-0.224,-0.223,-0.222,-0.221,-0.220,& -0.219,-0.218,-0.216,-0.215,-0.214,-0.212,-0.211,-0.209,-0.208,& -0.206,-0.204,-0.203,-0.201,-0.199,-0.197,-0.195,-0.193,-0.192,& -0.190,-0.188,-0.185,-0.183,-0.181,-0.179,-0.177,-0.175,-0.173,& 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0.552, 0.554, 0.556, 0.558, 0.560, 0.562, 0.564, 0.566, 0.568,& 0.570, 0.572, 0.574, 0.576, 0.578, 0.580, 0.582, 0.584, 0.586,& 0.588, 0.590, 0.592, 0.593, 0.595, 0.597, 0.599, 0.601, 0.603,& 0.605, 0.607, 0.609, 0.611, 0.613, 0.615, 0.617, 0.619, 0.620,& 0.622, 0.624, 0.626, 0.628, 0.630, 0.632, 0.634, 0.636, 0.637,& 0.639, 0.641, 0.643, 0.645, 0.665, 0.683, 0.701, 0.719, 0.736,& 0.753, 0.770, 0.787, 0.803, 0.820, 0.836, 0.852, 0.867, 0.883,& 0.898, 0.913, 0.928, 0.942, 0.957, 0.971, 0.985, 0.999, 1.013,& 1.027, 1.040, 1.053, 1.067, 1.080, 1.093, 1.105, 1.118, 1.131,& 1.143, 1.155, 1.167, 1.179, 1.191, 1.203, 1.215, 1.226, 1.238,& 1.249, 1.260, 1.271, 1.283, 1.293, 1.304, 1.315, 1.326, 1.336,& 1.347, 1.357, 1.367, 1.377, 1.388, 1.398, 1.408, 1.417, 1.427,& 1.437, 1.446, 1.456, 1.466, 1.475, 1.484, 1.493, 1.503, 1.512,& 1.521, 1.530, 1.539, 1.548, 1.556, 1.565, 1.574, 1.582, 1.591,& 1.599, 1.608, 1.616, 1.624, 1.633, 1.641, 1.649, 1.657, 1.665,& 1.673, 1.681, 1.689, 1.697, 1.704, 1.712, 1.720, 1.727, 1.735,& 1.742, 1.750, 1.757, 1.765, 1.772, 1.779, 1.787, 1.794, 1.801,& 1.808, 1.815, 1.822, 1.829, 1.836, 1.843, 1.850, 1.857, 1.864,& 1.870, 1.877, 1.884, 1.890, 1.897, 1.904, 1.910, 1.917, 1.923,& 1.930, 1.936, 1.942, 1.949, 1.955, 1.961, 1.968, 1.974, 1.980,& 1.986, 1.992, 1.998, 2.004, 2.010, 2.016, 2.022, 2.028, 2.034,& 2.040, 2.046, 2.052, 2.058, 2.063, 2.069, 2.075, 2.080, 2.086,& 2.092, 2.097, 2.103, 2.108, 2.114, 2.119, 2.125, 2.130, 2.136,& 2.141, 2.147, 2.152 & / !C !C ** (H,NO3) !C DATA BNC10M/ & -0.045,-0.094,-0.116,-0.130,-0.140,-0.147,-0.153,-0.158,-0.162,& -0.165,-0.167,-0.169,-0.171,-0.172,-0.173,-0.173,-0.174,-0.174,& -0.174,-0.173,-0.173,-0.172,-0.172,-0.171,-0.170,-0.169,-0.168,& -0.167,-0.166,-0.165,-0.163,-0.162,-0.161,-0.159,-0.158,-0.156,& -0.155,-0.153,-0.152,-0.150,-0.148,-0.147,-0.145,-0.143,-0.142,& -0.140,-0.138,-0.136,-0.135,-0.133,-0.131,-0.129,-0.127,-0.126,& -0.124,-0.122,-0.120,-0.118,-0.117,-0.115,-0.113,-0.111,-0.109,& 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0.215, 0.217, 0.220, 0.222,& 0.224, 0.226, 0.229, 0.231, 0.233, 0.235, 0.238, 0.240, 0.242,& 0.244, 0.247, 0.249, 0.251, 0.253, 0.256, 0.258, 0.260, 0.262,& 0.264, 0.267, 0.269, 0.271, 0.273, 0.275, 0.278, 0.280, 0.282,& 0.284, 0.286, 0.288, 0.291, 0.293, 0.295, 0.297, 0.299, 0.301,& 0.304, 0.306, 0.308, 0.310, 0.312, 0.314, 0.317, 0.319, 0.321,& 0.323, 0.325, 0.327, 0.329, 0.331, 0.333, 0.336, 0.338, 0.340,& 0.342, 0.344, 0.346, 0.348, 0.350, 0.352, 0.354, 0.356, 0.359,& 0.361, 0.363, 0.365, 0.367, 0.369, 0.371, 0.373, 0.375, 0.377,& 0.379, 0.381, 0.383, 0.385, 0.387, 0.389, 0.391, 0.393, 0.395,& 0.397, 0.399, 0.401, 0.403, 0.405, 0.407, 0.409, 0.411, 0.413,& 0.415, 0.417, 0.419, 0.421, 0.423, 0.425, 0.427, 0.429, 0.431,& 0.433, 0.435, 0.437, 0.439, 0.441, 0.443, 0.445, 0.447, 0.449,& 0.451, 0.453, 0.455, 0.456, 0.458, 0.460, 0.462, 0.464, 0.466,& 0.468, 0.470, 0.472, 0.474, 0.476, 0.477, 0.479, 0.481, 0.483,& 0.485, 0.487, 0.489, 0.491, 0.493, 0.494, 0.496, 0.498, 0.500,& 0.502, 0.504, 0.506, 0.507, 0.509, 0.511, 0.513, 0.515, 0.517,& 0.518, 0.520, 0.522, 0.524, 0.526, 0.528, 0.529, 0.531, 0.533,& 0.535, 0.537, 0.539, 0.540, 0.542, 0.544, 0.546, 0.547, 0.549,& 0.551, 0.553, 0.555, 0.556, 0.558, 0.560, 0.562, 0.564, 0.565,& 0.567, 0.569, 0.571, 0.572, 0.574, 0.576, 0.578, 0.579, 0.581,& 0.583, 0.585, 0.586, 0.588, 0.590, 0.592, 0.593, 0.595, 0.597,& 0.598, 0.600, 0.602, 0.604, 0.622, 0.639, 0.655, 0.672, 0.688,& 0.704, 0.719, 0.735, 0.750, 0.765, 0.780, 0.795, 0.809, 0.824,& 0.838, 0.852, 0.866, 0.879, 0.893, 0.906, 0.919, 0.932, 0.945,& 0.958, 0.971, 0.983, 0.996, 1.008, 1.020, 1.032, 1.044, 1.055,& 1.067, 1.079, 1.090, 1.101, 1.112, 1.123, 1.134, 1.145, 1.156,& 1.167, 1.177, 1.188, 1.198, 1.208, 1.218, 1.228, 1.238, 1.248,& 1.258, 1.268, 1.278, 1.287, 1.297, 1.306, 1.315, 1.325, 1.334,& 1.343, 1.352, 1.361, 1.370, 1.379, 1.387, 1.396, 1.405, 1.413,& 1.422, 1.430, 1.438, 1.447, 1.455, 1.463, 1.471, 1.479, 1.487,& 1.495, 1.503, 1.511, 1.519, 1.527, 1.534, 1.542, 1.550, 1.557,& 1.565, 1.572, 1.579, 1.587, 1.594, 1.601, 1.608, 1.616, 1.623,& 1.630, 1.637, 1.644, 1.651, 1.657, 1.664, 1.671, 1.678, 1.685,& 1.691, 1.698, 1.704, 1.711, 1.718, 1.724, 1.730, 1.737, 1.743,& 1.750, 1.756, 1.762, 1.768, 1.775, 1.781, 1.787, 1.793, 1.799,& 1.805, 1.811, 1.817, 1.823, 1.829, 1.835, 1.841, 1.846, 1.852,& 1.858, 1.864, 1.869, 1.875, 1.881, 1.886, 1.892, 1.897, 1.903,& 1.908, 1.914, 1.919, 1.925, 1.930, 1.936, 1.941, 1.946, 1.952,& 1.957, 1.962, 1.967, 1.972, 1.978, 1.983, 1.988, 1.993, 1.998,& 2.003, 2.008, 2.013 & / !C !C ** (H,Cl) !C DATA BNC11M/ & -0.044,-0.089,-0.107,-0.118,-0.125,-0.130,-0.133,-0.135,-0.136,& -0.136,-0.136,-0.135,-0.134,-0.132,-0.130,-0.128,-0.125,-0.122,& -0.119,-0.116,-0.113,-0.109,-0.105,-0.102,-0.098,-0.094,-0.089,& -0.085,-0.081,-0.076,-0.072,-0.067,-0.062,-0.057,-0.053,-0.048,& -0.043,-0.038,-0.033,-0.028,-0.022,-0.017,-0.012,-0.007,-0.001,& 0.004, 0.009, 0.015, 0.020, 0.025, 0.031, 0.036, 0.042, 0.047,& 0.053, 0.058, 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1.718, 1.722, 1.727, 1.732, 1.736, 1.741,& 1.746, 1.750, 1.755, 1.760, 1.764, 1.769, 1.774, 1.778, 1.783,& 1.787, 1.792, 1.797, 1.801, 1.806, 1.810, 1.815, 1.819, 1.824,& 1.828, 1.833, 1.838, 1.842, 1.847, 1.851, 1.855, 1.860, 1.864,& 1.869, 1.873, 1.878, 1.882, 1.887, 1.891, 1.895, 1.900, 1.904,& 1.909, 1.913, 1.917, 1.922, 1.926, 1.931, 1.935, 1.939, 1.944,& 1.948, 1.952, 1.957, 1.961, 1.965, 1.969, 1.974, 1.978, 1.982,& 1.987, 1.991, 1.995, 1.999, 2.045, 2.086, 2.127, 2.167, 2.206,& 2.245, 2.284, 2.322, 2.359, 2.396, 2.432, 2.468, 2.503, 2.538,& 2.572, 2.606, 2.639, 2.672, 2.705, 2.737, 2.769, 2.800, 2.831,& 2.862, 2.892, 2.922, 2.952, 2.981, 3.010, 3.039, 3.067, 3.095,& 3.123, 3.150, 3.178, 3.204, 3.231, 3.257, 3.283, 3.309, 3.335,& 3.360, 3.385, 3.410, 3.435, 3.459, 3.483, 3.507, 3.531, 3.554,& 3.577, 3.600, 3.623, 3.646, 3.668, 3.691, 3.713, 3.735, 3.756,& 3.778, 3.799, 3.820, 3.841, 3.862, 3.883, 3.903, 3.924, 3.944,& 3.964, 3.984, 4.003, 4.023, 4.043, 4.062, 4.081, 4.100, 4.119,& 4.138, 4.156, 4.175, 4.193, 4.211, 4.229, 4.247, 4.265, 4.283,& 4.300, 4.318, 4.335, 4.352, 4.369, 4.386, 4.403, 4.420, 4.437,& 4.453, 4.470, 4.486, 4.503, 4.519, 4.535, 4.551, 4.567, 4.582,& 4.598, 4.614, 4.629, 4.644, 4.660, 4.675, 4.690, 4.705, 4.720,& 4.735, 4.750, 4.764, 4.779, 4.794, 4.808, 4.822, 4.837, 4.851,& 4.865, 4.879, 4.893, 4.907, 4.921, 4.935, 4.948, 4.962, 4.975,& 4.989, 5.002, 5.016, 5.029, 5.042, 5.055, 5.068, 5.081, 5.094,& 5.107, 5.120, 5.133, 5.145, 5.158, 5.171, 5.183, 5.196, 5.208,& 5.220, 5.233, 5.245, 5.257, 5.269, 5.281, 5.293, 5.305, 5.317,& 5.329, 5.340, 5.352 & / !C !C ** NaHSO4 !C DATA BNC12M/ & -0.045,-0.094,-0.116,-0.130,-0.140,-0.148,-0.155,-0.160,-0.164,& -0.168,-0.170,-0.173,-0.174,-0.176,-0.177,-0.178,-0.178,-0.179,& -0.179,-0.178,-0.178,-0.177,-0.177,-0.176,-0.175,-0.174,-0.172,& -0.171,-0.170,-0.168,-0.166,-0.164,-0.162,-0.160,-0.158,-0.156,& -0.154,-0.152,-0.149,-0.147,-0.144,-0.142,-0.139,-0.136,-0.134,& 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0.982, 0.985, 0.988, 0.991, 0.995, 0.998, 1.001, 1.004,& 1.008, 1.011, 1.014, 1.017, 1.020, 1.024, 1.027, 1.030, 1.033,& 1.036, 1.039, 1.043, 1.046, 1.049, 1.052, 1.055, 1.058, 1.061,& 1.065, 1.068, 1.071, 1.074, 1.077, 1.080, 1.083, 1.086, 1.089,& 1.092, 1.096, 1.099, 1.102, 1.105, 1.108, 1.111, 1.114, 1.117,& 1.120, 1.123, 1.126, 1.129, 1.132, 1.135, 1.138, 1.141, 1.144,& 1.147, 1.150, 1.153, 1.156, 1.159, 1.162, 1.165, 1.168, 1.171,& 1.174, 1.177, 1.180, 1.183, 1.185, 1.188, 1.191, 1.194, 1.197,& 1.200, 1.203, 1.206, 1.209, 1.240, 1.268, 1.296, 1.323, 1.350,& 1.377, 1.403, 1.429, 1.454, 1.480, 1.505, 1.529, 1.553, 1.577,& 1.601, 1.624, 1.647, 1.670, 1.692, 1.715, 1.737, 1.758, 1.780,& 1.801, 1.822, 1.843, 1.863, 1.883, 1.903, 1.923, 1.943, 1.962,& 1.981, 2.000, 2.019, 2.038, 2.056, 2.075, 2.093, 2.111, 2.128,& 2.146, 2.163, 2.181, 2.198, 2.215, 2.231, 2.248, 2.264, 2.281,& 2.297, 2.313, 2.329, 2.345, 2.360, 2.376, 2.391, 2.406, 2.422,& 2.437, 2.451, 2.466, 2.481, 2.495, 2.510, 2.524, 2.538, 2.552,& 2.566, 2.580, 2.594, 2.608, 2.621, 2.635, 2.648, 2.661, 2.674,& 2.687, 2.700, 2.713, 2.726, 2.739, 2.751, 2.764, 2.776, 2.789,& 2.801, 2.813, 2.825, 2.838, 2.850, 2.861, 2.873, 2.885, 2.897,& 2.908, 2.920, 2.931, 2.943, 2.954, 2.965, 2.976, 2.987, 2.998,& 3.009, 3.020, 3.031, 3.042, 3.053, 3.063, 3.074, 3.084, 3.095,& 3.105, 3.116, 3.126, 3.136, 3.146, 3.156, 3.166, 3.176, 3.186,& 3.196, 3.206, 3.216, 3.226, 3.235, 3.245, 3.255, 3.264, 3.274,& 3.283, 3.292, 3.302, 3.311, 3.320, 3.330, 3.339, 3.348, 3.357,& 3.366, 3.375, 3.384, 3.393, 3.402, 3.410, 3.419, 3.428, 3.437,& 3.445, 3.454, 3.462, 3.471, 3.479, 3.488, 3.496, 3.505, 3.513,& 3.521, 3.529, 3.538 & / !C !C ** (NH4)3H(SO4)2 !C DATA BNC13M/ & -0.074,-0.160,-0.203,-0.233,-0.256,-0.275,-0.291,-0.306,-0.318,& -0.329,-0.339,-0.349,-0.357,-0.365,-0.372,-0.379,-0.386,-0.392,& -0.397,-0.402,-0.407,-0.412,-0.417,-0.421,-0.425,-0.429,-0.433,& -0.436,-0.439,-0.443,-0.446,-0.448,-0.451,-0.454,-0.456,-0.459,& 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1.484, 1.508, 1.531, 1.554, 1.577,& 1.600, 1.622, 1.644, 1.666, 1.687, 1.709, 1.730, 1.751, 1.772,& 1.792, 1.812, 1.832, 1.852, 1.872, 1.892, 1.911, 1.930, 1.949,& 1.968, 1.987, 2.005, 2.023, 2.042, 2.060, 2.077, 2.095, 2.113,& 2.130, 2.147, 2.164, 2.181, 2.198, 2.215, 2.231, 2.248, 2.264,& 2.280, 2.296, 2.312, 2.328, 2.343, 2.359, 2.374, 2.389, 2.405,& 2.420, 2.435, 2.449, 2.464, 2.479, 2.493, 2.508, 2.522, 2.536,& 2.550, 2.564, 2.578, 2.592, 2.606, 2.619, 2.633, 2.646, 2.660,& 2.673, 2.686, 2.699, 2.712, 2.725, 2.738, 2.751, 2.763, 2.776,& 2.788, 2.801, 2.813, 2.826, 2.838, 2.850, 2.862, 2.874, 2.886,& 2.898, 2.910, 2.921, 2.933, 2.945, 2.956, 2.967, 2.979, 2.990,& 3.001, 3.013, 3.024, 3.035, 3.046, 3.057, 3.068, 3.079, 3.089,& 3.100, 3.111, 3.121, 3.132, 3.142, 3.153, 3.163, 3.173, 3.184,& 3.194, 3.204, 3.214, 3.224, 3.234, 3.244, 3.254, 3.264, 3.274,& 3.284, 3.293, 3.303, 3.313, 3.322, 3.332, 3.341, 3.351, 3.360,& 3.370, 3.379, 3.388, 3.397, 3.407, 3.416, 3.425, 3.434, 3.443,& 3.452, 3.461, 3.470 & / !C !C ** MGCL2 !C DATA BNC23M/ & -0.090,-0.186,-0.229,-0.256,-0.276,-0.290,-0.302,-0.310,-0.317,& -0.322,-0.327,-0.330,-0.332,-0.333,-0.334,-0.335,-0.335,-0.334,& -0.333,-0.332,-0.331,-0.329,-0.327,-0.325,-0.322,-0.320,-0.317,& -0.314,-0.311,-0.308,-0.305,-0.301,-0.298,-0.294,-0.291,-0.287,& -0.283,-0.279,-0.275,-0.272,-0.268,-0.264,-0.260,-0.255,-0.251,& -0.247,-0.243,-0.239,-0.235,-0.231,-0.226,-0.222,-0.218,-0.214,& -0.209,-0.205,-0.201,-0.196,-0.192,-0.188,-0.184,-0.179,-0.175,& -0.170,-0.166,-0.162,-0.157,-0.153,-0.148,-0.144,-0.139,-0.135,& -0.130,-0.126,-0.121,-0.117,-0.112,-0.107,-0.103,-0.098,-0.093,& -0.089,-0.084,-0.079,-0.074,-0.069,-0.065,-0.060,-0.055,-0.050,& -0.045,-0.040,-0.034,-0.029,-0.024,-0.019,-0.014,-0.009,-0.003,& 0.002, 0.007, 0.013, 0.018, 0.023, 0.029, 0.034, 0.040, 0.045,& 0.050, 0.056, 0.061, 0.067, 0.073, 0.078, 0.084, 0.089, 0.095,& 0.100, 0.106, 0.112, 0.117, 0.123, 0.128, 0.134, 0.140, 0.145,& 0.151, 0.157, 0.162, 0.168, 0.174, 0.179, 0.185, 0.190, 0.196,& 0.202, 0.207, 0.213, 0.219, 0.224, 0.230, 0.235, 0.241, 0.247,& 0.252, 0.258, 0.263, 0.269, 0.275, 0.280, 0.286, 0.291, 0.297,& 0.302, 0.308, 0.313, 0.319, 0.325, 0.330, 0.336, 0.341, 0.347,& 0.352, 0.358, 0.363, 0.369, 0.374, 0.380, 0.385, 0.390, 0.396,& 0.401, 0.407, 0.412, 0.418, 0.423, 0.428, 0.434, 0.439, 0.445,& 0.450, 0.455, 0.461, 0.466, 0.471, 0.477, 0.482, 0.487, 0.493,& 0.498, 0.503, 0.509, 0.514, 0.519, 0.525, 0.530, 0.535, 0.540,& 0.546, 0.551, 0.556, 0.561, 0.567, 0.572, 0.577, 0.582, 0.587,& 0.593, 0.598, 0.603, 0.608, 0.613, 0.618, 0.624, 0.629, 0.634,& 0.639, 0.644, 0.649, 0.654, 0.659, 0.664, 0.669, 0.675, 0.680,& 0.685, 0.690, 0.695, 0.700, 0.705, 0.710, 0.715, 0.720, 0.725,& 0.730, 0.735, 0.740, 0.745, 0.750, 0.755, 0.759, 0.764, 0.769,& 0.774, 0.779, 0.784, 0.789, 0.794, 0.799, 0.804, 0.808, 0.813,& 0.818, 0.823, 0.828, 0.833, 0.837, 0.842, 0.847, 0.852, 0.857,& 0.861, 0.866, 0.871, 0.876, 0.880, 0.885, 0.890, 0.895, 0.899,& 0.904, 0.909, 0.914, 0.918, 0.923, 0.928, 0.932, 0.937, 0.942,& 0.946, 0.951, 0.955, 0.960, 0.965, 0.969, 0.974, 0.979, 0.983,& 0.988, 0.992, 0.997, 1.001, 1.006, 1.011, 1.015, 1.020, 1.024,& 1.029, 1.033, 1.038, 1.042, 1.047, 1.051, 1.056, 1.060, 1.065,& 1.069, 1.073, 1.078, 1.082, 1.087, 1.091, 1.096, 1.100, 1.104,& 1.109, 1.113, 1.118, 1.122, 1.126, 1.131, 1.135, 1.139, 1.144,& 1.148, 1.152, 1.157, 1.161, 1.165, 1.170, 1.174, 1.178, 1.183,& 1.187, 1.191, 1.195, 1.200, 1.204, 1.208, 1.212, 1.217, 1.221,& 1.225, 1.229, 1.234, 1.238, 1.242, 1.246, 1.250, 1.255, 1.259,& 1.263, 1.267, 1.271, 1.275, 1.279, 1.284, 1.288, 1.292, 1.296,& 1.300, 1.304, 1.308, 1.312, 1.316, 1.321, 1.325, 1.329, 1.333,& 1.337, 1.341, 1.345, 1.349, 1.353, 1.357, 1.361, 1.365, 1.369,& 1.373, 1.377, 1.381, 1.385, 1.389, 1.393, 1.397, 1.401, 1.405,& 1.409, 1.413, 1.417, 1.421, 1.425, 1.428, 1.432, 1.436, 1.440,& 1.444, 1.448, 1.452, 1.456, 1.497, 1.535, 1.573, 1.610, 1.646,& 1.682, 1.717, 1.752, 1.787, 1.821, 1.854, 1.888, 1.920, 1.953,& 1.985, 2.016, 2.048, 2.078, 2.109, 2.139, 2.169, 2.198, 2.227,& 2.256, 2.285, 2.313, 2.341, 2.368, 2.395, 2.422, 2.449, 2.475,& 2.501, 2.527, 2.553, 2.578, 2.603, 2.628, 2.653, 2.677, 2.701,& 2.725, 2.749, 2.772, 2.796, 2.819, 2.841, 2.864, 2.887, 2.909,& 2.931, 2.953, 2.974, 2.996, 3.017, 3.038, 3.059, 3.080, 3.100,& 3.121, 3.141, 3.161, 3.181, 3.201, 3.221, 3.240, 3.259, 3.279,& 3.298, 3.317, 3.335, 3.354, 3.372, 3.391, 3.409, 3.427, 3.445,& 3.463, 3.480, 3.498, 3.516, 3.533, 3.550, 3.567, 3.584, 3.601,& 3.618, 3.634, 3.651, 3.667, 3.684, 3.700, 3.716, 3.732, 3.748,& 3.764, 3.779, 3.795, 3.810, 3.826, 3.841, 3.856, 3.872, 3.887,& 3.902, 3.916, 3.931, 3.946, 3.961, 3.975, 3.989, 4.004, 4.018,& 4.032, 4.046, 4.060, 4.074, 4.088, 4.102, 4.116, 4.129, 4.143,& 4.157, 4.170, 4.183, 4.197, 4.210, 4.223, 4.236, 4.249, 4.262,& 4.275, 4.288, 4.300, 4.313, 4.326, 4.338, 4.351, 4.363, 4.376,& 4.388, 4.400, 4.412, 4.424, 4.436, 4.449, 4.460, 4.472, 4.484,& 4.496, 4.508, 4.519, 4.531, 4.543, 4.554, 4.566, 4.577, 4.588,& 4.600, 4.611, 4.622 & / END !C !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE KM323 !C *** CALCULATES BINARY ACTIVITY COEFFICIENTS BY KUSIK-MEISSNER METHOD. !C THE COMPUTATIONS HAVE BEEN PERFORMED AND THE RESULTS ARE STORED IN !C LOOKUP TABLES. THE IONIC ACTIVITY 'IN' IS INPUT, AND THE ARRAY !C 'BINARR' IS RETURNED WITH THE BINARY COEFFICIENTS. !C !C TEMPERATURE IS 323K !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE KM3232p1 (IONIC, BINARR) !C !C *** Common block definition !C COMMON /KMC3232p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) REAL Binarr (23), Ionic !C !C *** Find position in arrays for bincoef !C IF (Ionic.LE. 0.200000E+02) THEN ipos = MIN(NINT( 0.200000E+02*Ionic) + 1, 400) ELSE ipos = 400+NINT( 0.200000E+01*Ionic- 0.400000E+02) ENDIF ipos = min(ipos, 561) !C !C *** Assign values to return array !C Binarr(01) = BNC01M(ipos) Binarr(02) = BNC02M(ipos) Binarr(03) = BNC03M(ipos) Binarr(04) = BNC04M(ipos) Binarr(05) = BNC05M(ipos) Binarr(06) = BNC06M(ipos) Binarr(07) = BNC07M(ipos) Binarr(08) = BNC08M(ipos) Binarr(09) = BNC09M(ipos) Binarr(10) = BNC10M(ipos) Binarr(11) = BNC11M(ipos) Binarr(12) = BNC12M(ipos) Binarr(13) = BNC13M(ipos) Binarr(14) = BNC14M(ipos) Binarr(15) = BNC15M(ipos) Binarr(16) = BNC16M(ipos) Binarr(17) = BNC17M(ipos) Binarr(18) = BNC18M(ipos) Binarr(19) = BNC19M(ipos) Binarr(20) = BNC20M(ipos) Binarr(21) = BNC21M(ipos) Binarr(22) = BNC22M(ipos) Binarr(23) = BNC23M(ipos) !C !C *** Return point ; End of subroutine !C RETURN END BLOCK DATA KMCF3232p1 !C !C *** Common block definition !C COMMON /KMC3232p1/ & BNC01M( 561),BNC02M( 561),BNC03M( 561),BNC04M( 561),& BNC05M( 561),BNC06M( 561),BNC07M( 561),BNC08M( 561),& BNC09M( 561),BNC10M( 561),BNC11M( 561),BNC12M( 561),& BNC13M( 561),BNC14M( 561),BNC15M( 561),BNC16M( 561),& BNC17M( 561),BNC18M( 561),BNC19M( 561),BNC20M( 561),& BNC21M( 561),BNC22M( 561),BNC23M( 561) !C !C *** NaCl !C DATA BNC01M/ & -0.044,-0.092,-0.114,-0.129,-0.139,-0.147,-0.154,-0.159,-0.163,& -0.167,-0.170,-0.172,-0.174,-0.176,-0.177,-0.178,-0.179,-0.180,& -0.180,-0.181,-0.181,-0.181,-0.181,-0.180,-0.180,-0.180,-0.179,& -0.179,-0.178,-0.177,-0.177,-0.176,-0.175,-0.174,-0.173,-0.172,& -0.171,-0.170,-0.169,-0.168,-0.167,-0.166,-0.165,-0.163,-0.162,& -0.161,-0.160,-0.159,-0.157,-0.156,-0.155,-0.153,-0.152,-0.151,& -0.150,-0.148,-0.147,-0.146,-0.144,-0.143,-0.142,-0.140,-0.139,& -0.137,-0.136,-0.135,-0.133,-0.132,-0.130,-0.129,-0.127,-0.126,& -0.125,-0.123,-0.122,-0.120,-0.119,-0.117,-0.116,-0.114,-0.113,& -0.111,-0.109,-0.108,-0.106,-0.105,-0.103,-0.101,-0.100,-0.098,& -0.096,-0.095,-0.093,-0.091,-0.090,-0.088,-0.086,-0.084,-0.083,& -0.081,-0.079,-0.077,-0.076,-0.074,-0.072,-0.070,-0.068,-0.066,& -0.065,-0.063,-0.061,-0.059,-0.057,-0.055,-0.053,-0.052,-0.050,& -0.048,-0.046,-0.044,-0.042,-0.040,-0.038,-0.036,-0.035,-0.033,& -0.031,-0.029,-0.027,-0.025,-0.023,-0.021,-0.019,-0.017,-0.015,& -0.013,-0.012,-0.010,-0.008,-0.006,-0.004,-0.002, 0.000, 0.002,& 0.004, 0.006, 0.008, 0.009, 0.011, 0.013, 0.015, 0.017, 0.019,& 0.021, 0.023, 0.025, 0.027, 0.028, 0.030, 0.032, 0.034, 0.036,& 0.038, 0.040, 0.042, 0.044, 0.045, 0.047, 0.049, 0.051, 0.053,& 0.055, 0.057, 0.059, 0.060, 0.062, 0.064, 0.066, 0.068, 0.070,& 0.072, 0.074, 0.075, 0.077, 0.079, 0.081, 0.083, 0.085, 0.086,& 0.088, 0.090, 0.092, 0.094, 0.096, 0.097, 0.099, 0.101, 0.103,& 0.105, 0.107, 0.108, 0.110, 0.112, 0.114, 0.116, 0.117, 0.119,& 0.121, 0.123, 0.125, 0.127, 0.128, 0.130, 0.132, 0.134, 0.135,& 0.137, 0.139, 0.141, 0.143, 0.144, 0.146, 0.148, 0.150, 0.151,& 0.153, 0.155, 0.157, 0.159, 0.160, 0.162, 0.164, 0.166, 0.167,& 0.169, 0.171, 0.173, 0.174, 0.176, 0.178, 0.180, 0.181, 0.183,& 0.185, 0.186, 0.188, 0.190, 0.192, 0.193, 0.195, 0.197, 0.198,& 0.200, 0.202, 0.204, 0.205, 0.207, 0.209, 0.210, 0.212, 0.214,& 0.215, 0.217, 0.219, 0.221, 0.222, 0.224, 0.226, 0.227, 0.229,& 0.231, 0.232, 0.234, 0.236, 0.237, 0.239, 0.241, 0.242, 0.244,& 0.246, 0.247, 0.249, 0.250, 0.252, 0.254, 0.255, 0.257, 0.259,& 0.260, 0.262, 0.264, 0.265, 0.267, 0.268, 0.270, 0.272, 0.273,& 0.275, 0.276, 0.278, 0.280, 0.281, 0.283, 0.285, 0.286, 0.288,& 0.289, 0.291, 0.293, 0.294, 0.296, 0.297, 0.299, 0.300, 0.302,& 0.304, 0.305, 0.307, 0.308, 0.310, 0.311, 0.313, 0.315, 0.316,& 0.318, 0.319, 0.321, 0.322, 0.324, 0.325, 0.327, 0.329, 0.330,& 0.332, 0.333, 0.335, 0.336, 0.338, 0.339, 0.341, 0.342, 0.344,& 0.345, 0.347, 0.349, 0.350, 0.352, 0.353, 0.355, 0.356, 0.358,& 0.359, 0.361, 0.362, 0.364, 0.365, 0.367, 0.368, 0.370, 0.371,& 0.373, 0.374, 0.376, 0.377, 0.379, 0.380, 0.382, 0.383, 0.384,& 0.386, 0.387, 0.389, 0.390, 0.392, 0.393, 0.395, 0.396, 0.398,& 0.399, 0.401, 0.402, 0.404, 0.405, 0.406, 0.408, 0.409, 0.411,& 0.412, 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1.554, 1.560, 1.565,& 1.571, 1.577, 1.583, 1.589, 1.594, 1.600, 1.606, 1.612, 1.617,& 1.623, 1.629, 1.634, 1.640, 1.645, 1.651, 1.656, 1.662, 1.667,& 1.673, 1.678, 1.684, 1.689, 1.695, 1.700, 1.705, 1.711, 1.716,& 1.721, 1.727, 1.732 & / !C !C ** Na2SO4 !C DATA BNC02M/ & -0.091,-0.196,-0.249,-0.285,-0.314,-0.337,-0.358,-0.375,-0.390,& -0.404,-0.417,-0.428,-0.439,-0.449,-0.458,-0.466,-0.475,-0.482,& -0.489,-0.496,-0.502,-0.508,-0.514,-0.520,-0.525,-0.530,-0.535,& -0.540,-0.544,-0.549,-0.553,-0.557,-0.561,-0.565,-0.569,-0.572,& -0.576,-0.579,-0.582,-0.585,-0.588,-0.591,-0.594,-0.597,-0.600,& -0.603,-0.605,-0.608,-0.610,-0.613,-0.615,-0.617,-0.620,-0.622,& -0.624,-0.626,-0.628,-0.630,-0.632,-0.634,-0.636,-0.638,-0.640,& -0.641,-0.643,-0.645,-0.647,-0.648,-0.650,-0.651,-0.653,-0.654,& -0.656,-0.657,-0.659,-0.660,-0.662,-0.663,-0.665,-0.666,-0.667,& -0.669,-0.670,-0.671,-0.672,-0.674,-0.675,-0.676,-0.677,-0.678,& -0.679,-0.681,-0.682,-0.683,-0.684,-0.685,-0.686,-0.687,-0.688,& 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1.513, 1.521, 1.529, 1.537,& 1.546, 1.554, 1.562, 1.570, 1.578, 1.586, 1.593, 1.601, 1.609,& 1.617, 1.624, 1.632, 1.640, 1.647, 1.655, 1.662, 1.670, 1.677,& 1.685, 1.692, 1.700, 1.707, 1.714, 1.721, 1.729, 1.736, 1.743,& 1.750, 1.757, 1.764, 1.771, 1.778, 1.785, 1.792, 1.799, 1.806,& 1.813, 1.820, 1.826, 1.833, 1.840, 1.847, 1.853, 1.860, 1.866,& 1.873, 1.880, 1.886, 1.893, 1.899, 1.906, 1.912, 1.918, 1.925,& 1.931, 1.938, 1.944, 1.950, 1.956, 1.963, 1.969, 1.975, 1.981,& 1.987, 1.994, 2.000, 2.006, 2.012, 2.018, 2.024, 2.030, 2.036,& 2.042, 2.048, 2.054 & / !C !C ** (H,Cl) !C DATA BNC11M/ & -0.043,-0.087,-0.106,-0.117,-0.124,-0.130,-0.133,-0.135,-0.137,& -0.138,-0.138,-0.137,-0.136,-0.135,-0.134,-0.132,-0.130,-0.127,& -0.125,-0.122,-0.119,-0.116,-0.113,-0.110,-0.107,-0.103,-0.099,& -0.096,-0.092,-0.088,-0.084,-0.080,-0.076,-0.071,-0.067,-0.063,& -0.058,-0.054,-0.049,-0.045,-0.040,-0.036,-0.031,-0.027,-0.022,& -0.017,-0.012,-0.008,-0.003, 0.002, 0.007, 0.012, 0.017, 0.022,& 0.027, 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1.523, 1.527, 1.531, 1.536, 1.540, 1.544, 1.548,& 1.553, 1.557, 1.561, 1.565, 1.570, 1.574, 1.578, 1.582, 1.587,& 1.591, 1.595, 1.599, 1.603, 1.607, 1.612, 1.616, 1.620, 1.624,& 1.628, 1.632, 1.636, 1.640, 1.645, 1.649, 1.653, 1.657, 1.661,& 1.665, 1.669, 1.673, 1.677, 1.681, 1.685, 1.689, 1.693, 1.697,& 1.701, 1.705, 1.709, 1.713, 1.717, 1.721, 1.725, 1.729, 1.733,& 1.737, 1.741, 1.745, 1.749, 1.753, 1.757, 1.761, 1.765, 1.769,& 1.772, 1.776, 1.780, 1.784, 1.826, 1.864, 1.901, 1.938, 1.974,& 2.010, 2.045, 2.080, 2.114, 2.148, 2.181, 2.214, 2.246, 2.278,& 2.310, 2.341, 2.372, 2.403, 2.433, 2.463, 2.492, 2.522, 2.550,& 2.579, 2.607, 2.635, 2.663, 2.690, 2.717, 2.744, 2.770, 2.796,& 2.822, 2.848, 2.873, 2.898, 2.923, 2.948, 2.972, 2.996, 3.020,& 3.044, 3.068, 3.091, 3.114, 3.137, 3.160, 3.182, 3.205, 3.227,& 3.249, 3.271, 3.292, 3.314, 3.335, 3.356, 3.377, 3.398, 3.418,& 3.439, 3.459, 3.479, 3.499, 3.519, 3.539, 3.558, 3.578, 3.597,& 3.616, 3.635, 3.654, 3.673, 3.691, 3.710, 3.728, 3.746, 3.765,& 3.783, 3.800, 3.818, 3.836, 3.853, 3.871, 3.888, 3.905, 3.922,& 3.939, 3.956, 3.973, 3.990, 4.006, 4.023, 4.039, 4.055, 4.071,& 4.088, 4.104, 4.119, 4.135, 4.151, 4.167, 4.182, 4.198, 4.213,& 4.228, 4.243, 4.259, 4.274, 4.289, 4.304, 4.318, 4.333, 4.348,& 4.362, 4.377, 4.391, 4.406, 4.420, 4.434, 4.448, 4.462, 4.476,& 4.490, 4.504, 4.518, 4.532, 4.545, 4.559, 4.572, 4.586, 4.599,& 4.613, 4.626, 4.639, 4.652, 4.665, 4.678, 4.691, 4.704, 4.717,& 4.730, 4.743, 4.756, 4.768, 4.781, 4.793, 4.806, 4.818, 4.831,& 4.843, 4.855, 4.867, 4.880, 4.892, 4.904, 4.916, 4.928, 4.940,& 4.952, 4.964, 4.975 & / !C !C ** NaHSO4 !C DATA BNC12M/ & -0.044,-0.092,-0.113,-0.127,-0.138,-0.146,-0.152,-0.157,-0.162,& -0.165,-0.168,-0.170,-0.172,-0.174,-0.175,-0.176,-0.176,-0.177,& -0.177,-0.177,-0.176,-0.176,-0.176,-0.175,-0.174,-0.173,-0.172,& -0.171,-0.169,-0.168,-0.167,-0.165,-0.163,-0.161,-0.160,-0.158,& -0.156,-0.154,-0.151,-0.149,-0.147,-0.145,-0.142,-0.140,-0.137,& 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0.881, 0.884, 0.887, 0.890, 0.893, 0.896, 0.899, 0.902,& 0.905, 0.908, 0.911, 0.914, 0.917, 0.920, 0.923, 0.926, 0.929,& 0.932, 0.935, 0.938, 0.941, 0.944, 0.947, 0.949, 0.952, 0.955,& 0.958, 0.961, 0.964, 0.967, 0.970, 0.973, 0.975, 0.978, 0.981,& 0.984, 0.987, 0.990, 0.993, 0.995, 0.998, 1.001, 1.004, 1.007,& 1.010, 1.012, 1.015, 1.018, 1.021, 1.024, 1.026, 1.029, 1.032,& 1.035, 1.038, 1.040, 1.043, 1.046, 1.049, 1.051, 1.054, 1.057,& 1.060, 1.062, 1.065, 1.068, 1.071, 1.073, 1.076, 1.079, 1.082,& 1.084, 1.087, 1.090, 1.092, 1.121, 1.148, 1.174, 1.199, 1.225,& 1.250, 1.274, 1.299, 1.323, 1.346, 1.370, 1.393, 1.416, 1.438,& 1.461, 1.483, 1.504, 1.526, 1.547, 1.568, 1.589, 1.610, 1.630,& 1.650, 1.670, 1.690, 1.710, 1.729, 1.748, 1.767, 1.786, 1.805,& 1.823, 1.841, 1.860, 1.878, 1.895, 1.913, 1.930, 1.948, 1.965,& 1.982, 1.999, 2.015, 2.032, 2.048, 2.065, 2.081, 2.097, 2.113,& 2.129, 2.144, 2.160, 2.175, 2.191, 2.206, 2.221, 2.236, 2.251,& 2.265, 2.280, 2.294, 2.309, 2.323, 2.337, 2.352, 2.366, 2.379,& 2.393, 2.407, 2.421, 2.434, 2.448, 2.461, 2.474, 2.488, 2.501,& 2.514, 2.527, 2.540, 2.552, 2.565, 2.578, 2.590, 2.603, 2.615,& 2.628, 2.640, 2.652, 2.664, 2.676, 2.688, 2.700, 2.712, 2.724,& 2.735, 2.747, 2.759, 2.770, 2.782, 2.793, 2.805, 2.816, 2.827,& 2.838, 2.849, 2.860, 2.871, 2.882, 2.893, 2.904, 2.915, 2.926,& 2.936, 2.947, 2.957, 2.968, 2.978, 2.989, 2.999, 3.010, 3.020,& 3.030, 3.040, 3.050, 3.060, 3.070, 3.080, 3.090, 3.100, 3.110,& 3.120, 3.130, 3.139, 3.149, 3.159, 3.168, 3.178, 3.188, 3.197,& 3.206, 3.216, 3.225, 3.235, 3.244, 3.253, 3.262, 3.272, 3.281,& 3.290, 3.299, 3.308, 3.317, 3.326, 3.335, 3.344, 3.353, 3.361,& 3.370, 3.379, 3.388 & / !C !C ** (NH4)3H(SO4)2 !C DATA BNC13M/ & -0.072,-0.156,-0.197,-0.226,-0.248,-0.266,-0.282,-0.295,-0.307,& -0.317,-0.327,-0.336,-0.344,-0.351,-0.358,-0.364,-0.370,-0.375,& -0.380,-0.385,-0.390,-0.394,-0.398,-0.402,-0.406,-0.409,-0.412,& -0.415,-0.418,-0.421,-0.424,-0.426,-0.429,-0.431,-0.433,-0.435,& 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0.567,& 0.571, 0.574, 0.578, 0.581, 0.584, 0.588, 0.591, 0.595, 0.598,& 0.601, 0.605, 0.608, 0.611, 0.615, 0.618, 0.621, 0.625, 0.628,& 0.631, 0.635, 0.638, 0.641, 0.645, 0.648, 0.651, 0.655, 0.658,& 0.661, 0.665, 0.668, 0.671, 0.674, 0.678, 0.681, 0.684, 0.687,& 0.691, 0.694, 0.697, 0.700, 0.704, 0.707, 0.710, 0.713, 0.717,& 0.720, 0.723, 0.726, 0.729, 0.733, 0.736, 0.739, 0.742, 0.745,& 0.749, 0.752, 0.755, 0.758, 0.761, 0.764, 0.768, 0.771, 0.774,& 0.777, 0.780, 0.783, 0.786, 0.790, 0.793, 0.796, 0.799, 0.802,& 0.805, 0.808, 0.811, 0.814, 0.818, 0.821, 0.824, 0.827, 0.830,& 0.833, 0.836, 0.839, 0.842, 0.845, 0.848, 0.851, 0.854, 0.857,& 0.860, 0.864, 0.867, 0.870, 0.873, 0.876, 0.879, 0.882, 0.885,& 0.888, 0.891, 0.894, 0.897, 0.900, 0.903, 0.906, 0.909, 0.912,& 0.915, 0.918, 0.921, 0.924, 0.955, 0.984, 1.013, 1.041, 1.070,& 1.097, 1.125, 1.152, 1.179, 1.205, 1.231, 1.257, 1.283, 1.308,& 1.334, 1.359, 1.383, 1.408, 1.432, 1.456, 1.479, 1.503, 1.526,& 1.549, 1.572, 1.594, 1.617, 1.639, 1.661, 1.683, 1.704, 1.726,& 1.747, 1.768, 1.789, 1.810, 1.830, 1.851, 1.871, 1.891, 1.911,& 1.930, 1.950, 1.969, 1.989, 2.008, 2.027, 2.046, 2.064, 2.083,& 2.101, 2.120, 2.138, 2.156, 2.174, 2.192, 2.209, 2.227, 2.244,& 2.262, 2.279, 2.296, 2.313, 2.330, 2.347, 2.363, 2.380, 2.396,& 2.413, 2.429, 2.445, 2.461, 2.477, 2.493, 2.509, 2.525, 2.540,& 2.556, 2.571, 2.587, 2.602, 2.617, 2.632, 2.647, 2.662, 2.677,& 2.692, 2.707, 2.721, 2.736, 2.750, 2.765, 2.779, 2.793, 2.807,& 2.822, 2.836, 2.850, 2.863, 2.877, 2.891, 2.905, 2.918, 2.932,& 2.946, 2.959, 2.972, 2.986, 2.999, 3.012, 3.025, 3.039, 3.052,& 3.065, 3.078, 3.090, 3.103, 3.116, 3.129, 3.141, 3.154, 3.167,& 3.179, 3.191, 3.204, 3.216, 3.229, 3.241, 3.253, 3.265, 3.277,& 3.289, 3.301, 3.313, 3.325, 3.337, 3.349, 3.361, 3.372, 3.384,& 3.396, 3.407, 3.419, 3.431, 3.442, 3.453, 3.465, 3.476, 3.488,& 3.499, 3.510, 3.521, 3.532, 3.544, 3.555, 3.566, 3.577, 3.588,& 3.599, 3.610, 3.621 & / !C !C ** MGCL2 !C DATA BNC23M/ & -0.088,-0.182,-0.225,-0.252,-0.271,-0.286,-0.297,-0.306,-0.313,& -0.319,-0.323,-0.327,-0.329,-0.331,-0.332,-0.333,-0.333,-0.333,& -0.333,-0.332,-0.331,-0.329,-0.328,-0.326,-0.324,-0.322,-0.319,& -0.317,-0.314,-0.312,-0.309,-0.306,-0.303,-0.300,-0.296,-0.293,& -0.290,-0.286,-0.283,-0.279,-0.276,-0.272,-0.268,-0.265,-0.261,& -0.257,-0.253,-0.250,-0.246,-0.242,-0.238,-0.234,-0.230,-0.226,& -0.223,-0.219,-0.215,-0.211,-0.207,-0.203,-0.199,-0.195,-0.191,& -0.187,-0.183,-0.179,-0.174,-0.170,-0.166,-0.162,-0.158,-0.154,& -0.150,-0.145,-0.141,-0.137,-0.133,-0.128,-0.124,-0.120,-0.115,& -0.111,-0.106,-0.102,-0.097,-0.093,-0.088,-0.084,-0.079,-0.074,& -0.070,-0.065,-0.060,-0.056,-0.051,-0.046,-0.041,-0.036,-0.031,& -0.027,-0.022,-0.017,-0.012,-0.007,-0.002, 0.003, 0.008, 0.013,& 0.019, 0.024, 0.029, 0.034, 0.039, 0.044, 0.049, 0.055, 0.060,& 0.065, 0.070, 0.075, 0.081, 0.086, 0.091, 0.096, 0.101, 0.107,& 0.112, 0.117, 0.122, 0.128, 0.133, 0.138, 0.143, 0.149, 0.154,& 0.159, 0.164, 0.170, 0.175, 0.180, 0.185, 0.190, 0.196, 0.201,& 0.206, 0.211, 0.216, 0.222, 0.227, 0.232, 0.237, 0.242, 0.248,& 0.253, 0.258, 0.263, 0.268, 0.273, 0.279, 0.284, 0.289, 0.294,& 0.299, 0.304, 0.309, 0.314, 0.320, 0.325, 0.330, 0.335, 0.340,& 0.345, 0.350, 0.355, 0.360, 0.365, 0.370, 0.375, 0.380, 0.386,& 0.391, 0.396, 0.401, 0.406, 0.411, 0.416, 0.421, 0.426, 0.431,& 0.436, 0.441, 0.446, 0.450, 0.455, 0.460, 0.465, 0.470, 0.475,& 0.480, 0.485, 0.490, 0.495, 0.500, 0.505, 0.509, 0.514, 0.519,& 0.524, 0.529, 0.534, 0.539, 0.543, 0.548, 0.553, 0.558, 0.563,& 0.568, 0.572, 0.577, 0.582, 0.587, 0.592, 0.596, 0.601, 0.606,& 0.611, 0.615, 0.620, 0.625, 0.629, 0.634, 0.639, 0.644, 0.648,& 0.653, 0.658, 0.662, 0.667, 0.672, 0.676, 0.681, 0.686, 0.690,& 0.695, 0.700, 0.704, 0.709, 0.713, 0.718, 0.723, 0.727, 0.732,& 0.736, 0.741, 0.745, 0.750, 0.754, 0.759, 0.764, 0.768, 0.773,& 0.777, 0.782, 0.786, 0.791, 0.795, 0.800, 0.804, 0.809, 0.813,& 0.817, 0.822, 0.826, 0.831, 0.835, 0.840, 0.844, 0.848, 0.853,& 0.857, 0.862, 0.866, 0.870, 0.875, 0.879, 0.884, 0.888, 0.892,& 0.897, 0.901, 0.905, 0.910, 0.914, 0.918, 0.923, 0.927, 0.931,& 0.935, 0.940, 0.944, 0.948, 0.953, 0.957, 0.961, 0.965, 0.970,& 0.974, 0.978, 0.982, 0.986, 0.991, 0.995, 0.999, 1.003, 1.007,& 1.012, 1.016, 1.020, 1.024, 1.028, 1.032, 1.037, 1.041, 1.045,& 1.049, 1.053, 1.057, 1.061, 1.065, 1.070, 1.074, 1.078, 1.082,& 1.086, 1.090, 1.094, 1.098, 1.102, 1.106, 1.110, 1.114, 1.118,& 1.122, 1.126, 1.130, 1.134, 1.138, 1.142, 1.146, 1.150, 1.154,& 1.158, 1.162, 1.166, 1.170, 1.174, 1.178, 1.182, 1.186, 1.190,& 1.194, 1.198, 1.202, 1.206, 1.210, 1.214, 1.217, 1.221, 1.225,& 1.229, 1.233, 1.237, 1.241, 1.245, 1.248, 1.252, 1.256, 1.260,& 1.264, 1.268, 1.271, 1.275, 1.279, 1.283, 1.287, 1.290, 1.294,& 1.298, 1.302, 1.306, 1.309, 1.313, 1.317, 1.321, 1.324, 1.328,& 1.332, 1.336, 1.339, 1.343, 1.383, 1.420, 1.456, 1.491, 1.527,& 1.561, 1.596, 1.630, 1.663, 1.696, 1.729, 1.761, 1.793, 1.825,& 1.856, 1.887, 1.918, 1.948, 1.978, 2.008, 2.037, 2.066, 2.095,& 2.123, 2.152, 2.180, 2.207, 2.235, 2.262, 2.289, 2.315, 2.342,& 2.368, 2.394, 2.419, 2.445, 2.470, 2.495, 2.520, 2.544, 2.569,& 2.593, 2.617, 2.641, 2.664, 2.688, 2.711, 2.734, 2.757, 2.780,& 2.802, 2.824, 2.847, 2.869, 2.890, 2.912, 2.934, 2.955, 2.976,& 2.997, 3.018, 3.039, 3.060, 3.080, 3.101, 3.121, 3.141, 3.161,& 3.181, 3.201, 3.220, 3.240, 3.259, 3.279, 3.298, 3.317, 3.336,& 3.354, 3.373, 3.392, 3.410, 3.428, 3.447, 3.465, 3.483, 3.501,& 3.519, 3.536, 3.554, 3.572, 3.589, 3.606, 3.624, 3.641, 3.658,& 3.675, 3.692, 3.709, 3.725, 3.742, 3.759, 3.775, 3.791, 3.808,& 3.824, 3.840, 3.856, 3.872, 3.888, 3.904, 3.920, 3.935, 3.951,& 3.967, 3.982, 3.997, 4.013, 4.028, 4.043, 4.058, 4.074, 4.089,& 4.103, 4.118, 4.133, 4.148, 4.163, 4.177, 4.192, 4.206, 4.221,& 4.235, 4.249, 4.264, 4.278, 4.292, 4.306, 4.320, 4.334, 4.348,& 4.362, 4.376, 4.390, 4.403, 4.417, 4.431, 4.444, 4.458, 4.471,& 4.484, 4.498, 4.511, 4.524, 4.538, 4.551, 4.564, 4.577, 4.590,& 4.603, 4.616, 4.629 & / !C !C *** END OF BLOCK DATA EXPON ****************************************** !C END !CC************************************************************************* !CC !CC TOOLBOX LIBRARY v.1.0 (May 1995) !CC !CC Program unit : SUBROUTINE CHRBLN !CC Purpose : Position of last non-blank character in a string !CC Author : Athanasios Nenes !CC !CC ======================= ARGUMENTS / USAGE ============================= !CC !CC STR is the CHARACTER variable containing the string examined !CC IBLK is a INTEGER variable containing the position of last non !CC blank character. If string is all spaces (ie ' '), then !CC the value returned is 1. !CC !CC EXAMPLE: !CC STR = 'TEST1.DAT ' !CC CALL CHRBLN (STR, IBLK) !CC !CC after execution of this code segment, "IBLK" has the value "9", which !CC is the position of the last non-blank character of "STR". !CC !CC*********************************************************************** !CC SUBROUTINE CHRBLN2p1 (STR, IBLK) !CC !CC*********************************************************************** CHARACTER*(*) STR !C IBLK = 1 ! Substring pointer (default=1) ILEN = LEN(STR) ! Length of string DO 10 i=ILEN,1,-1 IF (STR(i:i).NE.' ' .AND. STR(i:i).NE.CHAR(0)) THEN IBLK = i RETURN ENDIF 10 CONTINUE RETURN !C END !CC************************************************************************* !CC !CC TOOLBOX LIBRARY v.1.0 (May 1995) !CC !CC Program unit : SUBROUTINE SHFTRGHT !CC Purpose : RIGHT-JUSTIFICATION FUNCTION ON A STRING !CC Author : Athanasios Nenes !CC !CC ======================= ARGUMENTS / USAGE ============================= !CC !CC STRING is the CHARACTER variable with the string to be justified !CC !CC EXAMPLE: !CC STRING = 'AAAA ' !CC CALL SHFTRGHT (STRING) !CC !CC after execution of this code segment, STRING contains the value !CC ' AAAA'. !CC !CC************************************************************************* !CC SUBROUTINE SHFTRGHT2p1 (CHR) !CC !CC*********************************************************************** CHARACTER CHR*(*) !C I1 = LEN(CHR) ! Total length of string CALL CHRBLN2p1(CHR,I2) ! Position of last non-blank character IF (I2.EQ.I1) RETURN !C DO 10 I=I2,1,-1 ! Shift characters CHR(I1+I-I2:I1+I-I2) = CHR(I:I) CHR(I:I) = ' ' 10 CONTINUE RETURN !C END !CC************************************************************************* !CC !CC TOOLBOX LIBRARY v.1.0 (May 1995) !CC !CC Program unit : SUBROUTINE RPLSTR !CC Purpose : REPLACE CHARACTERS OCCURING IN A STRING !CC Author : Athanasios Nenes !CC !CC ======================= ARGUMENTS / USAGE ============================= !CC !CC STRING is the CHARACTER variable with the string to be edited !CC OLD is the old character which is to be replaced !CC NEW is the new character which OLD is to be replaced with !CC IERR is 0 if everything went well, is 1 if 'NEW' contains 'OLD'. !CC In this case, this is invalid, and no change is done. !CC !CC EXAMPLE: !CC STRING = 'AAAA' !CC OLD = 'A' !CC NEW = 'B' !CC CALL RPLSTR (STRING, OLD, NEW) !CC !CC after execution of this code segment, STRING contains the value !CC 'BBBB'. !CC !CC************************************************************************* !CC SUBROUTINE RPLSTR2p1 (STRING, OLD, NEW, IERR) !CC !CC*********************************************************************** CHARACTER STRING*(*), OLD*(*), NEW*(*) !C !C *** INITIALIZE ******************************************************** !C ILO = LEN(OLD) !C !C *** CHECK AND SEE IF 'NEW' CONTAINS 'OLD', WHICH CANNOT *************** !C IP = INDEX(NEW,OLD) IF (IP.NE.0) THEN IERR = 1 RETURN ELSE IERR = 0 ENDIF !C !C *** PROCEED WITH REPLACING ******************************************* !C 10 IP = INDEX(STRING,OLD) ! SEE IF 'OLD' EXISTS IN 'STRING' IF (IP.EQ.0) RETURN ! 'OLD' DOES NOT EXIST ; RETURN STRING(IP:IP+ILO-1) = NEW ! REPLACE SUBSTRING 'OLD' WITH 'NEW' GOTO 10 ! GO FOR NEW OCCURANCE OF 'OLD' !C END !CC************************************************************************* !CC !CC TOOLBOX LIBRARY v.1.0 (May 1995) !CC !CC Program unit : SUBROUTINE INPTD !CC Purpose : Prompts user for a value (DOUBLE). A default value !CC is provided, so if user presses , the default !CC is used. !CC Author : Athanasios Nenes !CC !CC ======================= ARGUMENTS / USAGE ============================= !CC !CC VAR is the DOUBLE PRECISION variable which value is to be saved !CC DEF is a DOUBLE PRECISION variable, with the default value of VAR. !CC PROMPT is a CHARACTER varible containing the prompt string. !CC PRFMT is a CHARACTER variable containing the FORMAT specifier !CC for the default value DEF. !CC IERR is an INTEGER error flag, and has the values: !CC 0 - No error detected. !CC 1 - Invalid FORMAT and/or Invalid default value. !CC 2 - Bad value specified by user !CC !CC EXAMPLE: !CC CALL INPTD (VAR, 1.0D0, 'Give value for A ', '*', Ierr) !CC !CC after execution of this code segment, the user is prompted for the !CC value of variable VAR. If is pressed (ie no value is specified) !CC then 1.0 is assigned to VAR. The default value is displayed in free- !CC format. The error status is specified by variable Ierr !CC !CC*********************************************************************** !CC SUBROUTINE INPTD2p1 (VAR, DEF, PROMPT, PRFMT, IERR) !CC !CC*********************************************************************** CHARACTER PROMPT*(*), PRFMT*(*), BUFFER*128 DOUBLE PRECISION DEF, VAR INTEGER IERR !C IERR = 0 !C !C *** WRITE DEFAULT VALUE TO WORK BUFFER ******************************* !C WRITE (BUFFER, FMT=PRFMT, ERR=10) DEF CALL CHRBLN2p1 (BUFFER, IEND) !C !C *** PROMPT USER FOR INPUT AND READ IT ******************************** !C WRITE (*,*) PROMPT,' [',BUFFER(1:IEND),']: ' READ (*, '(A)', ERR=20, END=20) BUFFER CALL CHRBLN2p1 (BUFFER,IEND) !C !C *** READ DATA OR SET DEFAULT ? **************************************** !C IF (IEND.EQ.1 .AND. BUFFER(1:1).EQ.' ') THEN VAR = DEF ELSE READ (BUFFER, *, ERR=20, END=20) VAR ENDIF !C !C *** RETURN POINT ****************************************************** !C 30 RETURN !C !C *** ERROR HANDLER ***************************************************** !C 10 IERR = 1 ! Bad FORMAT and/or bad default value GOTO 30 !C 20 IERR = 2 ! Bad number given by user GOTO 30 !C END !CC************************************************************************* !CC !CC TOOLBOX LIBRARY v.1.0 (May 1995) !CC !CC Program unit : SUBROUTINE Pushend !CC Purpose : Positions the pointer of a sequential file at its end !CC Simulates the ACCESS='APPEND' clause of a F77L OPEN !CC statement with Standard Fortran commands. !CC !CC ======================= ARGUMENTS / USAGE ============================= !CC !CC Iunit is a INTEGER variable, the file unit which the file is !CC connected to. !CC !CC EXAMPLE: !CC CALL PUSHEND (10) !CC !CC after execution of this code segment, the pointer of unit 10 is !CC pushed to its end. !CC !CC*********************************************************************** !CC SUBROUTINE Pushend2p1 (Iunit) !CC !CC*********************************************************************** !C LOGICAL OPNED !C !C *** INQUIRE IF Iunit CONNECTED TO FILE ******************************** !C INQUIRE (UNIT=Iunit, OPENED=OPNED) IF (.NOT.OPNED) GOTO 25 !C !C *** Iunit CONNECTED, PUSH POINTER TO END ****************************** !C 10 READ (Iunit,'()', ERR=20, END=20) GOTO 10 !C !C *** RETURN POINT ****************************************************** !C 20 BACKSPACE (Iunit) 25 RETURN END !CC************************************************************************* !CC !CC TOOLBOX LIBRARY v.1.0 (May 1995) !CC !CC Program unit : SUBROUTINE APPENDEXT !CC Purpose : Fix extension in file name string !CC !CC ======================= ARGUMENTS / USAGE ============================= !CC !CC Filename is the CHARACTER variable with the file name !CC Defext is the CHARACTER variable with extension (including '.', !CC ex. '.DAT') !CC Overwrite is a LOGICAL value, .TRUE. overwrites any existing extension !CC in "Filename" with "Defext", .FALSE. puts "Defext" only if !CC there is no extension in "Filename". !CC !CC EXAMPLE: !CC FILENAME1 = 'TEST.DAT' !CC FILENAME2 = 'TEST.DAT' !CC CALL APPENDEXT (FILENAME1, '.TXT', .FALSE.) !CC CALL APPENDEXT (FILENAME2, '.TXT', .TRUE. ) !CC !CC after execution of this code segment, "FILENAME1" has the value !CC 'TEST.DAT', while "FILENAME2" has the value 'TEST.TXT' !CC !CC*********************************************************************** !CC SUBROUTINE Appendext2p1 (Filename, Defext, Overwrite) !CC !CC*********************************************************************** CHARACTER*(*) Filename, Defext LOGICAL Overwrite !C CALL CHRBLN2p1 (Filename, Iend) IF (Filename(1:1).EQ.' ' .AND. Iend.EQ.1) RETURN ! Filename empty Idot = INDEX (Filename, '.') ! Append extension ? IF (Idot.EQ.0) Filename = Filename(1:Iend)//Defext IF (Overwrite .AND. Idot.NE.0) & Filename = Filename(:Idot-1)//Defext RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE POLY3 !C *** FINDS THE REAL ROOTS OF THE THIRD ORDER ALGEBRAIC EQUATION: !C X**3 + A1*X**2 + A2*X + A3 = 0.0 !C THE EQUATION IS SOLVED ANALYTICALLY. !C !C PARAMETERS A1, A2, A3 ARE SPECIFIED BY THE USER. THE MINIMUM !C NONEGATIVE ROOT IS RETURNED IN VARIABLE 'ROOT'. IF NO ROOT IS !C FOUND (WHICH IS GREATER THAN ZERO), ROOT HAS THE VALUE 1D30. !C AND THE FLAG ISLV HAS A VALUE GREATER THAN ZERO. !C !C SOLUTION FORMULA IS FOUND IN PAGE 32 OF: !C MATHEMATICAL HANDBOOK OF FORMULAS AND TABLES !C SCHAUM'S OUTLINE SERIES !C MURRAY SPIEGER, McGRAW-HILL, NEW YORK, 1968 !C (GREEK TRANSLATION: BY SOTIRIOS PERSIDES, ESPI, ATHENS, 1976) !C !C A SPECIAL CASE IS CONSIDERED SEPERATELY ; WHEN A3 = 0, THEN !C ONE ROOT IS X=0.0, AND THE OTHER TWO FROM THE SOLUTION OF THE !C QUADRATIC EQUATION X**2 + A1*X + A2 = 0.0 !C THIS SPECIAL CASE IS CONSIDERED BECAUSE THE ANALYTICAL FORMULA !C DOES NOT YIELD ACCURATE RESULTS (DUE TO NUMERICAL ROUNDOFF ERRORS) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE POLY32p1 (A1, A2, A3, ROOT, ISLV) !C IMPLICIT DOUBLE PRECISION (A-H, O-Z) PARAMETER (EXPON=1.D0/3.D0, ZERO=0.D0, THET1=120.D0/180.D0,& THET2=240.D0/180.D0, PI=3.14159265358932, EPS=1D-50) DOUBLE PRECISION X(3) !C !C *** SPECIAL CASE : QUADRATIC*X EQUATION ***************************** !C IF (ABS(A3).LE.EPS) THEN ISLV = 1 IX = 1 X(1) = ZERO D = A1*A1-4.D0*A2 IF (D.GE.ZERO) THEN IX = 3 SQD = SQRT(D) X(2) = 0.5*(-A1+SQD) X(3) = 0.5*(-A1-SQD) ENDIF ELSE !C !C *** NORMAL CASE : CUBIC EQUATION ************************************ !C !C DEFINE PARAMETERS Q, R, S, T, D !C ISLV= 1 Q = (3.D0*A2 - A1*A1)/9.D0 R = (9.D0*A1*A2 - 27.D0*A3 - 2.D0*A1*A1*A1)/54.D0 D = Q*Q*Q + R*R !C !C *** CALCULATE ROOTS ************************************************* !C !C D < 0, THREE REAL ROOTS !C IF (D.LT.-EPS) THEN ! D < -EPS : D < ZERO IX = 3 THET = EXPON*ACOS(R/SQRT(-Q*Q*Q)) COEF = 2.D0*SQRT(-Q) X(1) = COEF*COS(THET) - EXPON*A1 X(2) = COEF*COS(THET + THET1*PI) - EXPON*A1 X(3) = COEF*COS(THET + THET2*PI) - EXPON*A1 !C !C D = 0, THREE REAL (ONE DOUBLE) ROOTS !C ELSE IF (D.LE.EPS) THEN ! -EPS <= D <= EPS : D = ZERO IX = 2 SSIG = SIGN (1.D0, R) S = SSIG*(ABS(R))**EXPON X(1) = 2.D0*S - EXPON*A1 X(2) = -S - EXPON*A1 !C !C D > 0, ONE REAL ROOT !C ELSE ! D > EPS : D > ZERO IX = 1 SQD = SQRT(D) SSIG = SIGN (1.D0, R+SQD) ! TRANSFER SIGN TO SSIG TSIG = SIGN (1.D0, R-SQD) S = SSIG*(ABS(R+SQD))**EXPON ! EXPONENTIATE ABS() T = TSIG*(ABS(R-SQD))**EXPON X(1) = S + T - EXPON*A1 ENDIF ENDIF !C !C *** SELECT APPROPRIATE ROOT ***************************************** !C ROOT = 1.D30 DO 10 I=1,IX IF (X(I).GT.ZERO) THEN ROOT = MIN (ROOT, X(I)) ISLV = 0 ENDIF 10 CONTINUE !C !C *** END OF SUBROUTINE POLY3 ***************************************** !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE POLY3B !C *** FINDS A REAL ROOT OF THE THIRD ORDER ALGEBRAIC EQUATION: !C X**3 + A1*X**2 + A2*X + A3 = 0.0 !C THE EQUATION IS SOLVED NUMERICALLY (BISECTION). !C !C PARAMETERS A1, A2, A3 ARE SPECIFIED BY THE USER. THE MINIMUM !C NONEGATIVE ROOT IS RETURNED IN VARIABLE 'ROOT'. IF NO ROOT IS !C FOUND (WHICH IS GREATER THAN ZERO), ROOT HAS THE VALUE 1D30. !C AND THE FLAG ISLV HAS A VALUE GREATER THAN ZERO. !C !C RTLW, RTHI DEFINE THE INTERVAL WHICH THE ROOT IS LOOKED FOR. !C !C======================================================================= !C SUBROUTINE POLY3B2p1 (A1, A2, A3, RTLW, RTHI, ROOT, ISLV) !C IMPLICIT DOUBLE PRECISION (A-H, O-Z) PARAMETER (ZERO=0.D0, EPS=1D-15, MAXIT=100, NDIV=5) !C FUNC(X) = X**3.d0 + A1*X**2.0 + A2*X + A3 !C !C *** INITIAL VALUES FOR BISECTION ************************************* !C X1 = RTLW Y1 = FUNC(X1) IF (ABS(Y1).LE.EPS) THEN ! Is low a root? ROOT = RTLW GOTO 50 ENDIF !C !C *** ROOT TRACKING ; FOR THE RANGE OF HI AND LO *********************** !C DX = (RTHI-RTLW)/FLOAT(NDIV) DO 10 I=1,NDIV X2 = X1+DX Y2 = FUNC (X2) IF (SIGN(1.d0,Y1)*SIGN(1.d0,Y2) .LT. ZERO) GOTO 20 ! (Y1*Y2.LT.ZERO) X1 = X2 Y1 = Y2 10 CONTINUE !C !C *** NO SUBDIVISION WITH SOLUTION FOUND !C IF (ABS(Y2) .LT. EPS) THEN ! X2 is a root ROOT = X2 ELSE ROOT = 1.d30 ISLV = 1 ENDIF GOTO 50 !C !C *** BISECTION ******************************************************* !C 20 DO 30 I=1,MAXIT X3 = 0.5*(X1+X2) Y3 = FUNC (X3) IF (SIGN(1.d0,Y1)*SIGN(1.d0,Y3) .LE. ZERO) THEN ! (Y1*Y3 .LE. ZERO) Y2 = Y3 X2 = X3 ELSE Y1 = Y3 X1 = X3 ENDIF IF (ABS(X2-X1) .LE. EPS*X1) GOTO 40 30 CONTINUE !C !C *** CONVERGED ; RETURN *********************************************** !C 40 X3 = 0.5*(X1+X2) Y3 = FUNC (X3) ROOT = X3 ISLV = 0 !C 50 RETURN !C !C *** END OF SUBROUTINE POLY3B ***************************************** !C END !ccc PROGRAM DRIVER !ccc DOUBLE PRECISION ROOT !cccC !ccc CALL POLY3 (-1.d0, 1.d0, -1.d0, ROOT, ISLV) !ccc IF (ISLV.NE.0) STOP 'Error in POLY3' !ccc WRITE (*,*) 'Root=', ROOT !cccC !ccc CALL POLY3B (-1.d0, 1.d0, -1.d0, -10.d0, 10.d0, ROOT, ISLV) !ccc IF (ISLV.NE.0) STOP 'Error in POLY3B' !ccc WRITE (*,*) 'Root=', ROOT !cccC !ccc END !C======================================================================= !C !C *** ISORROPIA CODE !C *** FUNCTION EX10 !C *** 10^X FUNCTION ; ALTERNATE OF LIBRARY ROUTINE ; USED BECAUSE IT IS !C MUCH FASTER BUT WITHOUT GREAT LOSS IN ACCURACY. , !C MAXIMUM ERROR IS 2%, EXECUTION TIME IS 42% OF THE LIBRARY ROUTINE !C (ON A 80286/80287 MACHINE, using Lahey FORTRAN 77 v.3.0). !C !C EXPONENT RANGE IS BETWEEN -K AND K (K IS THE REAL ARGUMENT 'K') !C MAX VALUE FOR K: 9.999 !C IF X < -K, X IS SET TO -K, IF X > K, X IS SET TO K !C !C THE EXPONENT IS CALCULATED BY THE PRODUCT ADEC*AINT, WHERE ADEC !C IS THE MANTISSA AND AINT IS THE MAGNITUDE (EXPONENT). BOTH !C MANTISSA AND MAGNITUDE ARE PRE-CALCULATED AND STORED IN LOOKUP !C TABLES ; THIS LEADS TO THE INCREASED SPEED. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C FUNCTION EX102p1(X,K) REAL X, EX102p1, Y, AINT10, ADEC10, K INTEGER K1, K2 COMMON /EXPNC2p1/ AINT10(20), ADEC10(200) !C !C *** LIMIT X TO [-K, K] RANGE ***************************************** !C Y = MAX(-K, MIN(X,K)) ! MIN: -9.999, MAX: 9.999 !C !C *** GET INTEGER AND DECIMAL PART ************************************* !C K1 = INT(Y) K2 = INT(100*(Y-K1)) !C !C *** CALCULATE EXP FUNCTION ******************************************* !C EX102p1 = AINT10(K1+10)*ADEC10(K2+100) !C !C *** END OF EXP FUNCTION ********************************************** !C RETURN END !C======================================================================= !C !C *** ISORROPIA CODE !C *** BLOCK DATA EXPON !C *** CONTAINS DATA FOR EXPONENT ARRAYS NEEDED IN FUNCTION EXP10 !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C BLOCK DATA EXPON2p1 !C !C *** Common block definition !C REAL AINT10, ADEC10 COMMON /EXPNC2p1/ AINT10(20), ADEC10(200) !C !C *** Integer part !C DATA AINT10/ & 0.1000E-08, 0.1000E-07, 0.1000E-06, 0.1000E-05, 0.1000E-04,& 0.1000E-03, 0.1000E-02, 0.1000E-01, 0.1000E+00, 0.1000E+01,& 0.1000E+02, 0.1000E+03, 0.1000E+04, 0.1000E+05, 0.1000E+06,& 0.1000E+07, 0.1000E+08, 0.1000E+09, 0.1000E+10, 0.1000E+11 & / !C !C *** decimal part !C DATA (ADEC10(I),I=1,100)/ & 0.1023E+00, 0.1047E+00, 0.1072E+00, 0.1096E+00, 0.1122E+00, & 0.1148E+00, 0.1175E+00, 0.1202E+00, 0.1230E+00, 0.1259E+00, & 0.1288E+00, 0.1318E+00, 0.1349E+00, 0.1380E+00, 0.1413E+00, & 0.1445E+00, 0.1479E+00, 0.1514E+00, 0.1549E+00, 0.1585E+00, & 0.1622E+00, 0.1660E+00, 0.1698E+00, 0.1738E+00, 0.1778E+00, & 0.1820E+00, 0.1862E+00, 0.1905E+00, 0.1950E+00, 0.1995E+00, & 0.2042E+00, 0.2089E+00, 0.2138E+00, 0.2188E+00, 0.2239E+00, & 0.2291E+00, 0.2344E+00, 0.2399E+00, 0.2455E+00, 0.2512E+00, & 0.2570E+00, 0.2630E+00, 0.2692E+00, 0.2754E+00, 0.2818E+00, & 0.2884E+00, 0.2951E+00, 0.3020E+00, 0.3090E+00, 0.3162E+00, & 0.3236E+00, 0.3311E+00, 0.3388E+00, 0.3467E+00, 0.3548E+00, & 0.3631E+00, 0.3715E+00, 0.3802E+00, 0.3890E+00, 0.3981E+00, & 0.4074E+00, 0.4169E+00, 0.4266E+00, 0.4365E+00, 0.4467E+00, & 0.4571E+00, 0.4677E+00, 0.4786E+00, 0.4898E+00, 0.5012E+00, & 0.5129E+00, 0.5248E+00, 0.5370E+00, 0.5495E+00, 0.5623E+00, & 0.5754E+00, 0.5888E+00, 0.6026E+00, 0.6166E+00, 0.6310E+00, & 0.6457E+00, 0.6607E+00, 0.6761E+00, 0.6918E+00, 0.7079E+00, & 0.7244E+00, 0.7413E+00, 0.7586E+00, 0.7762E+00, 0.7943E+00, & 0.8128E+00, 0.8318E+00, 0.8511E+00, 0.8710E+00, 0.8913E+00, & 0.9120E+00, 0.9333E+00, 0.9550E+00, 0.9772E+00, 0.1000E+01/ DATA (ADEC10(I),I=101,200)/ & 0.1023E+01, 0.1047E+01, 0.1072E+01, 0.1096E+01, 0.1122E+01, & 0.1148E+01, 0.1175E+01, 0.1202E+01, 0.1230E+01, 0.1259E+01, & 0.1288E+01, 0.1318E+01, 0.1349E+01, 0.1380E+01, 0.1413E+01, & 0.1445E+01, 0.1479E+01, 0.1514E+01, 0.1549E+01, 0.1585E+01, & 0.1622E+01, 0.1660E+01, 0.1698E+01, 0.1738E+01, 0.1778E+01, & 0.1820E+01, 0.1862E+01, 0.1905E+01, 0.1950E+01, 0.1995E+01, & 0.2042E+01, 0.2089E+01, 0.2138E+01, 0.2188E+01, 0.2239E+01, & 0.2291E+01, 0.2344E+01, 0.2399E+01, 0.2455E+01, 0.2512E+01, & 0.2570E+01, 0.2630E+01, 0.2692E+01, 0.2754E+01, 0.2818E+01, & 0.2884E+01, 0.2951E+01, 0.3020E+01, 0.3090E+01, 0.3162E+01, & 0.3236E+01, 0.3311E+01, 0.3388E+01, 0.3467E+01, 0.3548E+01, & 0.3631E+01, 0.3715E+01, 0.3802E+01, 0.3890E+01, 0.3981E+01, & 0.4074E+01, 0.4169E+01, 0.4266E+01, 0.4365E+01, 0.4467E+01, & 0.4571E+01, 0.4677E+01, 0.4786E+01, 0.4898E+01, 0.5012E+01, & 0.5129E+01, 0.5248E+01, 0.5370E+01, 0.5495E+01, 0.5623E+01, & 0.5754E+01, 0.5888E+01, 0.6026E+01, 0.6166E+01, 0.6310E+01, & 0.6457E+01, 0.6607E+01, 0.6761E+01, 0.6918E+01, 0.7079E+01, & 0.7244E+01, 0.7413E+01, 0.7586E+01, 0.7762E+01, 0.7943E+01, & 0.8128E+01, 0.8318E+01, 0.8511E+01, 0.8710E+01, 0.8913E+01, & 0.9120E+01, 0.9333E+01, 0.9550E+01, 0.9772E+01, 0.1000E+02 & / !C !C *** END OF BLOCK DATA EXPON ****************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE PUSHERR !C *** THIS SUBROUTINE SAVES AN ERROR MESSAGE IN THE ERROR STACK !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE PUSHERR2p1 (IERR,ERRINF) INCLUDE 'module_isrpia_inc.F' CHARACTER ERRINF*(*) !C !C *** SAVE ERROR CODE IF THERE IS ANY SPACE *************************** !C IF (NOFER.LT.NERRMX) THEN NOFER = NOFER + 1 ERRSTK(NOFER) = IERR ERRMSG(NOFER) = ERRINF STKOFL =.FALSE. ELSE STKOFL =.TRUE. ! STACK OVERFLOW ENDIF !C !C *** END OF SUBROUTINE PUSHERR **************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE ISERRINF !C *** THIS SUBROUTINE OBTAINS A COPY OF THE ERROR STACK (& MESSAGES) !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE ISERRINF2p1 (ERRSTKI, ERRMSGI, NOFERI, STKOFLI) INCLUDE 'module_isrpia_inc.F' CHARACTER ERRMSGI*40 INTEGER ERRSTKI LOGICAL STKOFLI DIMENSION ERRMSGI(NERRMX), ERRSTKI(NERRMX) !C !C *** OBTAIN WHOLE ERROR STACK **************************************** !C DO 10 I=1,NOFER ! Error messages & codes ERRSTKI(I) = ERRSTK(I) ERRMSGI(I) = ERRMSG(I) 10 CONTINUE !C STKOFLI = STKOFL NOFERI = NOFER !C RETURN !C !C *** END OF SUBROUTINE ISERRINF *************************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE ERRSTAT !C *** THIS SUBROUTINE REPORTS ERROR MESSAGES TO UNIT 'IO' !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE ERRSTAT2p1 (IO,IERR,ERRINF) INCLUDE 'module_isrpia_inc.F' CHARACTER CER*4, NCIS*29, NCIF*27, NSIS*26, NSIF*24, ERRINF*(*) DATA NCIS /'NO CONVERGENCE IN SUBROUTINE '/, & NCIF /'NO CONVERGENCE IN FUNCTION ' /, & NSIS /'NO SOLUTION IN SUBROUTINE ' /, & NSIF /'NO SOLUTION IN FUNCTION ' / !C !C *** WRITE ERROR IN CHARACTER ***************************************** !C WRITE (CER,'(I4)') IERR CALL RPLSTR2p1 (CER, ' ', '0',IOK) ! REPLACE BLANKS WITH ZEROS CALL CHRBLN2p1 (ERRINF, IEND) ! LAST POSITION OF ERRINF CHAR !C !C *** WRITE ERROR TYPE (FATAL, WARNING ) ******************************* !C IF (IERR.EQ.0) THEN WRITE (IO,1000) 'NO ERRORS DETECTED ' GOTO 10 !C ELSE IF (IERR.LT.0) THEN WRITE (IO,1000) 'ERROR STACK EXHAUSTED ' GOTO 10 !C ELSE IF (IERR.GT.1000) THEN WRITE (IO,1100) 'FATAL',CER !C ELSE WRITE (IO,1100) 'WARNING',CER ENDIF !C !C *** WRITE ERROR MESSAGE ********************************************** !C !C FATAL MESSAGES !C IF (IERR.EQ.1001) THEN CALL CHRBLN2p1 (SCASE, IEND) WRITE (IO,1000) 'CASE NOT SUPPORTED IN CALCMR ['//SCASE(1:IEND) & //']' !C ELSEIF (IERR.EQ.1002) THEN CALL CHRBLN2p1 (SCASE, IEND) WRITE (IO,1000) 'CASE NOT SUPPORTED ['//SCASE(1:IEND)//']' !C !C WARNING MESSAGES !C ELSEIF (IERR.EQ.0001) THEN WRITE (IO,1000) NSIS,ERRINF !C ELSEIF (IERR.EQ.0002) THEN WRITE (IO,1000) NCIS,ERRINF !C ELSEIF (IERR.EQ.0003) THEN WRITE (IO,1000) NSIF,ERRINF !C ELSEIF (IERR.EQ.0004) THEN WRITE (IO,1000) NCIF,ERRINF !C ELSE IF (IERR.EQ.0019) THEN WRITE (IO,1000) 'HNO3(aq) AFFECTS H+, WHICH '// & 'MIGHT AFFECT SO4/HSO4 RATIO' WRITE (IO,1000) 'DIRECT INCREASE IN H+ [',ERRINF(1:IEND),'] %' !C ELSE IF (IERR.EQ.0020) THEN IF (W(4).GT.TINY .AND. W(5).GT.TINY) THEN WRITE (IO,1000) 'HSO4-SO4 EQUILIBRIUM MIGHT AFFECT HNO3,' & //'HCL DISSOLUTION' ELSE WRITE (IO,1000) 'HSO4-SO4 EQUILIBRIUM MIGHT AFFECT NH3 ' & //'DISSOLUTION' ENDIF WRITE (IO,1000) 'DIRECT DECREASE IN H+ [',ERRINF(1:IEND),'] %' !C ELSE IF (IERR.EQ.0021) THEN WRITE (IO,1000) 'HNO3(aq),HCL(aq) AFFECT H+, WHICH '// & 'MIGHT AFFECT SO4/HSO4 RATIO' WRITE (IO,1000) 'DIRECT INCREASE IN H+ [',ERRINF(1:IEND),'] %' !C ELSE IF (IERR.EQ.0022) THEN WRITE (IO,1000) 'HCL(g) EQUILIBRIUM YIELDS NONPHYSICAL '// & 'DISSOLUTION' WRITE (IO,1000) 'A TINY AMOUNT [',ERRINF(1:IEND),'] IS '// & 'ASSUMED TO BE DISSOLVED' !C ELSEIF (IERR.EQ.0033) THEN WRITE (IO,1000) 'HCL(aq) AFFECTS H+, WHICH '// & 'MIGHT AFFECT SO4/HSO4 RATIO' WRITE (IO,1000) 'DIRECT INCREASE IN H+ [',ERRINF(1:IEND),'] %' !C ELSEIF (IERR.EQ.0050) THEN WRITE (IO,1000) 'TOO MUCH SODIUM GIVEN AS INPUT.' WRITE (IO,1000) 'REDUCED TO COMPLETELY NEUTRALIZE SO4,Cl,NO3.' WRITE (IO,1000) 'EXCESS SODIUM IS IGNORED.' !C ELSEIF (IERR.EQ.0051) THEN WRITE (IO,1000) 'TOO MUCH CALCIUM GIVEN AS INPUT.' WRITE (IO,1000) 'REDUCED TO COMPLETELY NEUTRALIZE SO4,Cl,NO3.' WRITE (IO,1000) 'EXCESS CALCIUM IS IGNORED.' !C ELSEIF (IERR.EQ.0052) THEN WRITE (IO,1000) 'TOO MUCH SODIUM (+Ca) GIVEN AS INPUT.' WRITE (IO,1000) 'REDUCED TO COMPLETELY NEUTRALIZE SO4,Cl,NO3.' WRITE (IO,1000) 'EXCESS SODIUM IS IGNORED.' !C ELSEIF (IERR.EQ.0053) THEN WRITE (IO,1000) 'TOO MUCH MAGNESIUM (+Ca,Na) GIVEN AS INPUT.' WRITE (IO,1000) 'REDUCED TO COMPLETELY NEUTRALIZE SO4,Cl,NO3.' WRITE (IO,1000) 'EXCESS MAGNESIUM IS IGNORED.' !C ELSEIF (IERR.EQ.0054) THEN WRITE (IO,1000) 'TOO MUCH POTASSIUM(+Ca,Na,Mg) GIVEN AS INPUT.' WRITE (IO,1000) 'REDUCED TO COMPLETELY NEUTRALIZE SO4,Cl,NO3.' WRITE (IO,1000) 'EXCESS POTASSIUM IS IGNORED.' !C ELSE WRITE (IO,1000) 'NO DIAGNOSTIC MESSAGE AVAILABLE' ENDIF !C 10 RETURN !C !C *** FORMAT STATEMENTS ************************************* !C 1000 FORMAT (1X,A:A:A:A:A) 1100 FORMAT (1X,A,' ERROR [',A4,']:') !C !C *** END OF SUBROUTINE ERRSTAT ***************************** !C END !C======================================================================= !C !C *** ISORROPIA CODE !C *** SUBROUTINE ISORINF !C *** THIS SUBROUTINE PROVIDES INFORMATION ABOUT ISORROPIA !C !C ======================== ARGUMENTS / USAGE =========================== !C !C OUTPUT: !C 1. [VERSI] !C CHARACTER*15 variable. !C Contains version-date information of ISORROPIA !C !C 2. [NCMP] !C INTEGER variable. !C The number of components needed in input array WI !C (or, the number of major species accounted for by ISORROPIA) !C !C 3. [NION] !C INTEGER variable !C The number of ions considered in the aqueous phase !C !C 4. [NAQGAS] !C INTEGER variable !C The number of undissociated species found in aqueous aerosol !C phase !C !C 5. [NSOL] !C INTEGER variable !C The number of solids considered in the solid aerosol phase !C !C 6. [NERR] !C INTEGER variable !C The size of the error stack (maximum number of errors that can !C be stored before the stack exhausts). !C !C 7. [TIN] !C DOUBLE PRECISION variable !C The value used for a very small number. !C !C 8. [GRT] !C DOUBLE PRECISION variable !C The value used for a very large number. !C !C *** COPYRIGHT 1996-2006, UNIVERSITY OF MIAMI, CARNEGIE MELLON UNIVERSITY, !C *** GEORGIA INSTITUTE OF TECHNOLOGY !C *** WRITTEN BY ATHANASIOS NENES !C *** UPDATED BY CHRISTOS FOUNTOUKIS !C !C======================================================================= !C SUBROUTINE ISORINF2p1 (VERSI, NCMP, NION, NAQGAS, NSOL, NERR, TIN, & GRT) INCLUDE 'module_isrpia_inc.F' CHARACTER VERSI*(*) !C !C *** ASSIGN INFO ******************************************************* !C VERSI = VERSION NCMP = NCOMP NION = NIONS NAQGAS = NGASAQ NSOL = NSLDS NERR = NERRMX TIN = TINY GRT = GREAT !C RETURN !C !C *** END OF SUBROUTINE ISORINF ******************************************* !C END